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Ripening and annealing effects in InAs/GaAs(001) quantum dot formation

Abstract

Scanning tunneling microscopy has been used to investigate the effects of annealing and quenching on InAs/GaAs(001) quantum dots (QD) grown at a low growth rate by molecular beam epitaxy (MBE). Significant changes in QD number density, average volume (of more than one order of magnitude), wetting layer morphology, and QD volume density have been observed after in situ annealing for up to 90 s at a growth temperature of 485 deg. C providing direct evidence for a QD ripening process resembling that observed in other heteroepitaxial growth systems. Inefficient sample removal from the growth chamber and cooling (quenching) leads to unintentional annealing and ripening of the QDs and/or the appearance of clusters on the sample surface. The appearance of these clusters can have a significant impact on any statistical analysis of QD samples. Our results show that MBE-grown InAs/GaAs(001) QDs are kinetically controlled structures even at low growth rates, and underline the importance of the quench method in minimizing postgrowth changes in the characteristics of the uncapped QD array and preserving the in situ surface morphology for ex situ surface studies.
Authors:
Krzyzewski, T J; Jones, T S [1] 
  1. Centre for Electronic Materials and Devices, Department of Chemistry, Imperial College London, London SW7 2AZ (United Kingdom)
Publication Date:
Jul 01, 2004
Product Type:
Journal Article
Resource Relation:
Journal Name: Journal of Applied Physics; Journal Volume: 96; Journal Issue: 1; Other Information: DOI: 10.1063/1.1759788; (c) 2004 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA); PBD: 1 Jul 2004
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; ANNEALING; CRYSTAL GROWTH; GALLIUM ARSENIDES; INDIUM ARSENIDES; MOLECULAR BEAM EPITAXY; MORPHOLOGY; QUANTUM DOTS; QUENCHING; SCANNING TUNNELING MICROSCOPY
OSTI ID:
20619028
Country of Origin:
United States
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0021-8979; JAPIAU; TRN: US04B2018062526
Submitting Site:
INIS
Size:
page(s) 668-674
Announcement Date:
Aug 21, 2005

Citation Formats

Krzyzewski, T J, and Jones, T S. Ripening and annealing effects in InAs/GaAs(001) quantum dot formation. United States: N. p., 2004. Web. doi:10.1063/1.1759788.
Krzyzewski, T J, & Jones, T S. Ripening and annealing effects in InAs/GaAs(001) quantum dot formation. United States. https://doi.org/10.1063/1.1759788
Krzyzewski, T J, and Jones, T S. 2004. "Ripening and annealing effects in InAs/GaAs(001) quantum dot formation." United States. https://doi.org/10.1063/1.1759788.
@misc{etde_20619028,
title = {Ripening and annealing effects in InAs/GaAs(001) quantum dot formation}
author = {Krzyzewski, T J, and Jones, T S}
abstractNote = {Scanning tunneling microscopy has been used to investigate the effects of annealing and quenching on InAs/GaAs(001) quantum dots (QD) grown at a low growth rate by molecular beam epitaxy (MBE). Significant changes in QD number density, average volume (of more than one order of magnitude), wetting layer morphology, and QD volume density have been observed after in situ annealing for up to 90 s at a growth temperature of 485 deg. C providing direct evidence for a QD ripening process resembling that observed in other heteroepitaxial growth systems. Inefficient sample removal from the growth chamber and cooling (quenching) leads to unintentional annealing and ripening of the QDs and/or the appearance of clusters on the sample surface. The appearance of these clusters can have a significant impact on any statistical analysis of QD samples. Our results show that MBE-grown InAs/GaAs(001) QDs are kinetically controlled structures even at low growth rates, and underline the importance of the quench method in minimizing postgrowth changes in the characteristics of the uncapped QD array and preserving the in situ surface morphology for ex situ surface studies.}
doi = {10.1063/1.1759788}
journal = []
issue = {1}
volume = {96}
journal type = {AC}
place = {United States}
year = {2004}
month = {Jul}
}