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Accelerated remediation of pesticide-contaminated soil with zerovalent iron

Abstract

High pesticide concentrations in soil from spills or discharges can result in point-source contamination of ground and surface waters. Cost-effective technologies are needed for on-site treatment that meet clean-up goals and restore soil function. Remediation is particularly challenging when a mixture of pesticides is present. Zerovalent iron (Fe{sup 0}) has been shown to promote reductive dechlorination and nitro group reduction of a wide range of contaminants in soil and water. We employed Fe{sup 0} for on-site treatment of soil containing >1000 mg metolachlor, >55 mg alachlor, >64 mg atrazine, >35 mg pendimethalin, and >10 mg chlorpyrifos kg{sup -1}. While concentrations were highly variable within the windrowed soil, treatment with 5% (w/w) Fe{sup 0} resulted in >60% destruction of the five pesticides within 90 d and increased to >90% when 2% (w/w) Al{sub 2}(SO{sub 4}){sub 3} was added to the Fe{sup 0}. GC/MS analysis confirmed dechlorination of metolachlor and alachlor during treatment. Our observations support the use of Fe{sup 0} for ex situ treatment of pesticide-contaminated soil. - Capsule: Zerovalent iron promotes pesticide degradation in highly contaminated soil.
Authors:
Shea, P J; [1]  Machacek, T A; [1]  Comfort, S D [1] 
  1. University of Nebraska-Lincoln, Lincoln, NE 68583-0915 (United States)
Publication Date:
Nov 01, 2004
Product Type:
Journal Article
Resource Relation:
Journal Name: Environmental Pollution (1987); Journal Volume: 132; Journal Issue: 2; Other Information: DOI: 10.1016/j.envpol.2004.05.003; PII: S0269-7491(04)00187-3; Copyright (c) 2004 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved; Country of input: International Atomic Energy Agency (IAEA); PBD: Nov 2004
Subject:
54 ENVIRONMENTAL SCIENCES; ALUMINIUM SULFATES; COST; DECHLORINATION; GAS CHROMATOGRAPHY; IRON; LAND POLLUTION; MASS SPECTROSCOPY; PESTICIDES; POINT SOURCES; REMEDIAL ACTION; SOILS; SURFACE WATERS; WATER
OSTI ID:
20617959
Country of Origin:
United Kingdom
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0269-7491; ENPOEK; TRN: GB05R2489061457
Submitting Site:
GBN
Size:
page(s) 183-188
Announcement Date:
Aug 21, 2005

Citation Formats

Shea, P J, Machacek, T A, and Comfort, S D. Accelerated remediation of pesticide-contaminated soil with zerovalent iron. United Kingdom: N. p., 2004. Web. doi:10.1016/j.envpol.2004.05.003.
Shea, P J, Machacek, T A, & Comfort, S D. Accelerated remediation of pesticide-contaminated soil with zerovalent iron. United Kingdom. https://doi.org/10.1016/j.envpol.2004.05.003
Shea, P J, Machacek, T A, and Comfort, S D. 2004. "Accelerated remediation of pesticide-contaminated soil with zerovalent iron." United Kingdom. https://doi.org/10.1016/j.envpol.2004.05.003.
@misc{etde_20617959,
title = {Accelerated remediation of pesticide-contaminated soil with zerovalent iron}
author = {Shea, P J, Machacek, T A, and Comfort, S D}
abstractNote = {High pesticide concentrations in soil from spills or discharges can result in point-source contamination of ground and surface waters. Cost-effective technologies are needed for on-site treatment that meet clean-up goals and restore soil function. Remediation is particularly challenging when a mixture of pesticides is present. Zerovalent iron (Fe{sup 0}) has been shown to promote reductive dechlorination and nitro group reduction of a wide range of contaminants in soil and water. We employed Fe{sup 0} for on-site treatment of soil containing >1000 mg metolachlor, >55 mg alachlor, >64 mg atrazine, >35 mg pendimethalin, and >10 mg chlorpyrifos kg{sup -1}. While concentrations were highly variable within the windrowed soil, treatment with 5% (w/w) Fe{sup 0} resulted in >60% destruction of the five pesticides within 90 d and increased to >90% when 2% (w/w) Al{sub 2}(SO{sub 4}){sub 3} was added to the Fe{sup 0}. GC/MS analysis confirmed dechlorination of metolachlor and alachlor during treatment. Our observations support the use of Fe{sup 0} for ex situ treatment of pesticide-contaminated soil. - Capsule: Zerovalent iron promotes pesticide degradation in highly contaminated soil.}
doi = {10.1016/j.envpol.2004.05.003}
journal = []
issue = {2}
volume = {132}
journal type = {AC}
place = {United Kingdom}
year = {2004}
month = {Nov}
}