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Catalysis in non aqueous ionic medium. Metathesis of olefins by tungsten complexes

Abstract

Room-temperature molten salts have been studied as electrolytes for batteries or as solvents for electrochemical reactions (example: metal coating). They can also be used as solvents for transition metal catalytic cationic complexes (examples: nickel complexes for olefin dimerization, Ziegler-Natta titanium complexes for ethylene polymerization). They are particularly interesting because of their non-miscibility with non functionalized olefins and in consequence they can be used in two-phase catalysis. For this purpose, the properties expected from these media as well as their compositions are different from those expected for electrochemistry. We have studied mixtures of dialkylimidazolium chloride with ethylaluminium chloride compounds like Et{sub x}AlCl{sub (3-x)} (with x = 0, 1, 2 or 3). The catalytic reaction we were interested in is the olefin metathesis by tungsten complexes.
Publication Date:
Jan 01, 1994
Product Type:
Thesis/Dissertation
Report Number:
IFP-41151
Reference Number:
SCA: 023000; PA: FRC-94:002335; NTS-94:018484; EDB-94:079546; ERA-19:020785; SN: 94001210197
Resource Relation:
Other Information: TH: These (D. es Sc.); PBD: Jan 1994
Subject:
02 PETROLEUM; NONAQUEOUS SOLVENTS; ALKENES; TUNGSTEN; CATALYSIS; ZIEGLER CATALYST; LEWIS ACIDS; CHEMICAL REACTIONS; NICKEL COMPLEXES; TITANIUM COMPLEXES; 023000; PROPERTIES AND COMPOSITION
OSTI ID:
10155909
Research Organizations:
Institut Francais du Petrole (IFP), 92 - Rueil-Malmaison (France); Ecole Nationale Superieure du Petrole et des Moteurs (ENSPM), 92 - Rueil-Malmaison (France); Paris-6 Univ., 75 (France)
Country of Origin:
France
Language:
French
Other Identifying Numbers:
Other: ON: DE94769951; TRN: FR9402335
Availability:
OSTI; NTIS (US Sales Only)
Submitting Site:
FR
Size:
272 p.
Announcement Date:
Jul 06, 2005

Citation Formats

Di Marco-van-Tiggelen, F. Catalysis in non aqueous ionic medium. Metathesis of olefins by tungsten complexes. France: N. p., 1994. Web.
Di Marco-van-Tiggelen, F. Catalysis in non aqueous ionic medium. Metathesis of olefins by tungsten complexes. France.
Di Marco-van-Tiggelen, F. 1994. "Catalysis in non aqueous ionic medium. Metathesis of olefins by tungsten complexes." France.
@misc{etde_10155909,
title = {Catalysis in non aqueous ionic medium. Metathesis of olefins by tungsten complexes}
author = {Di Marco-van-Tiggelen, F}
abstractNote = {Room-temperature molten salts have been studied as electrolytes for batteries or as solvents for electrochemical reactions (example: metal coating). They can also be used as solvents for transition metal catalytic cationic complexes (examples: nickel complexes for olefin dimerization, Ziegler-Natta titanium complexes for ethylene polymerization). They are particularly interesting because of their non-miscibility with non functionalized olefins and in consequence they can be used in two-phase catalysis. For this purpose, the properties expected from these media as well as their compositions are different from those expected for electrochemistry. We have studied mixtures of dialkylimidazolium chloride with ethylaluminium chloride compounds like Et{sub x}AlCl{sub (3-x)} (with x = 0, 1, 2 or 3). The catalytic reaction we were interested in is the olefin metathesis by tungsten complexes.}
place = {France}
year = {1994}
month = {Jan}
}