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Comparative study of humic and fulvic substances in groundwaters. Pt. 3. Metal complexation with humic substances

Abstract

Humic and fulvic acids were extracted from large volumes of three different groundwaters. After purification they were characterised in terms of proton-binding properties, molecular weight, UV spectra and trace impurities. Conditional stability constants were measured for fulvic and humic binding with cobalt, nickel, calcium and uranium. From these, intrinsic binding constants were calculated using Humic Ion-Binding Model V which was found to describe the dependence of binding strength on pH and ionic strength reasonably well. Species distributions in the groundwaters were calculated and the effects of competition with alkali earths are discussed. All the experimental data are reported in a separate volume (Appendix A and B) so that they are available for testing other models. (author).
Authors:
Higgo, J J.W.; Davis, J; Smith, B [1] 
  1. British Geological Survey, Keyworth (United Kingdom). Fluid Processes Research Group; and others
Publication Date:
Dec 31, 1992
Product Type:
Technical Report
Report Number:
DOE-HMIP-RR-92.099
Reference Number:
SCA: 052002; PA: AIX-24:042919; SN: 93000991048
Resource Relation:
Other Information: PBD: 1992
Subject:
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES; GROUND WATER; FULVIC ACIDS; HUMIC ACIDS; RADIOACTIVE WASTE DISPOSAL; MATHEMATICAL MODELS; CHEMICAL STATE; IMPURITIES; PH VALUE; ULTRAVIOLET SPECTRA; 052002; WASTE DISPOSAL AND STORAGE
OSTI ID:
10153754
Research Organizations:
Department of the Environment, London (United Kingdom). Her Majesty`s Inspectorate of Pollution
Country of Origin:
United Kingdom
Language:
English
Other Identifying Numbers:
Other: ON: DE93626424; CNN: Contract PECD-7/9/533; WE/92/12; TRN: GB9300539042919
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
GBN
Size:
[75] p.
Announcement Date:
Jul 06, 2005

Citation Formats

Higgo, J J.W., Davis, J, and Smith, B. Comparative study of humic and fulvic substances in groundwaters. Pt. 3. Metal complexation with humic substances. United Kingdom: N. p., 1992. Web.
Higgo, J J.W., Davis, J, & Smith, B. Comparative study of humic and fulvic substances in groundwaters. Pt. 3. Metal complexation with humic substances. United Kingdom.
Higgo, J J.W., Davis, J, and Smith, B. 1992. "Comparative study of humic and fulvic substances in groundwaters. Pt. 3. Metal complexation with humic substances." United Kingdom.
@misc{etde_10153754,
title = {Comparative study of humic and fulvic substances in groundwaters. Pt. 3. Metal complexation with humic substances}
author = {Higgo, J J.W., Davis, J, and Smith, B}
abstractNote = {Humic and fulvic acids were extracted from large volumes of three different groundwaters. After purification they were characterised in terms of proton-binding properties, molecular weight, UV spectra and trace impurities. Conditional stability constants were measured for fulvic and humic binding with cobalt, nickel, calcium and uranium. From these, intrinsic binding constants were calculated using Humic Ion-Binding Model V which was found to describe the dependence of binding strength on pH and ionic strength reasonably well. Species distributions in the groundwaters were calculated and the effects of competition with alkali earths are discussed. All the experimental data are reported in a separate volume (Appendix A and B) so that they are available for testing other models. (author).}
place = {United Kingdom}
year = {1992}
month = {Dec}
}