You need JavaScript to view this

Spectroscopic study of europium(III) iminodiacelate, di-glycolate, thiodiglicolate and dipicolinate in aqueous solution

Abstract

Luminescence lifetime of Eu(III) in complexes with four dicarboxylic (imino dicarboxylic, diglicolic, thioglycolic and dipicolinic) acids having potentially liganding donor atoms have been measured in H{sub 2}O and D{sub O} solutions. Luminescence lifetimes have been used for identification of the inner-sphere interactions between Eu(III) and the ligands, providing the number of water molecules coordinated to the Eu(III) ion. On the basis of hydration numbers calculated for the complexes studied as well as analysis of the FTIR spectra of the DGA ligands and their Tb(III) complexes, the role of the donor atoms (N, O, S) in complexation of lanthanide ions is discussed. The results show that the donor atoms of nitrogen and oxygen are bonded to lanthanide ions, in tridentate - dipicolinic, diglicolic and iminodiacetic acid ligands, whereas sulfur is not bonded to these ions, thus tioglycolic acid coordinates as a bidentate ligands. (author). 10 refs, 3 figs, 2 tabs.
Authors:
Lis, S; Hnatejko, Z; Elbanowski, M [1] 
  1. Uniwersytet Adama Mickiewicza, Poznan (Poland). Inst. Chemii
Publication Date:
Dec 31, 1994
Product Type:
Journal Article
Reference Number:
SCA: 400201; PA: AIX-26:058521; EDB-95:131016; SN: 95001461675
Resource Relation:
Journal Name: Bulletin of the Polish Academy of Sciences, Chemistry; Journal Volume: 42; Journal Issue: 1; Other Information: PBD: 1994
Subject:
40 CHEMISTRY; EUROPIUM IONS; COMPLEXES; TERBIUM IONS; SPECTROSCOPY; ACETATES; AQUEOUS SOLUTIONS; CHEMICAL BONDS; COORDINATION VALENCES; GLYCOLS; LUMINESCENCE; PICOLINES; STRUCTURAL CHEMICAL ANALYSIS; TDA
OSTI ID:
101522
Country of Origin:
Poland
Language:
English
Other Identifying Numbers:
Journal ID: BPACEQ; ISSN 0239-7285; TRN: PL9500282058521
Submitting Site:
PLN
Size:
pp. 49-55
Announcement Date:
Oct 06, 1995

Citation Formats

Lis, S, Hnatejko, Z, and Elbanowski, M. Spectroscopic study of europium(III) iminodiacelate, di-glycolate, thiodiglicolate and dipicolinate in aqueous solution. Poland: N. p., 1994. Web.
Lis, S, Hnatejko, Z, & Elbanowski, M. Spectroscopic study of europium(III) iminodiacelate, di-glycolate, thiodiglicolate and dipicolinate in aqueous solution. Poland.
Lis, S, Hnatejko, Z, and Elbanowski, M. 1994. "Spectroscopic study of europium(III) iminodiacelate, di-glycolate, thiodiglicolate and dipicolinate in aqueous solution." Poland.
@misc{etde_101522,
title = {Spectroscopic study of europium(III) iminodiacelate, di-glycolate, thiodiglicolate and dipicolinate in aqueous solution}
author = {Lis, S, Hnatejko, Z, and Elbanowski, M}
abstractNote = {Luminescence lifetime of Eu(III) in complexes with four dicarboxylic (imino dicarboxylic, diglicolic, thioglycolic and dipicolinic) acids having potentially liganding donor atoms have been measured in H{sub 2}O and D{sub O} solutions. Luminescence lifetimes have been used for identification of the inner-sphere interactions between Eu(III) and the ligands, providing the number of water molecules coordinated to the Eu(III) ion. On the basis of hydration numbers calculated for the complexes studied as well as analysis of the FTIR spectra of the DGA ligands and their Tb(III) complexes, the role of the donor atoms (N, O, S) in complexation of lanthanide ions is discussed. The results show that the donor atoms of nitrogen and oxygen are bonded to lanthanide ions, in tridentate - dipicolinic, diglicolic and iminodiacetic acid ligands, whereas sulfur is not bonded to these ions, thus tioglycolic acid coordinates as a bidentate ligands. (author). 10 refs, 3 figs, 2 tabs.}
journal = []
issue = {1}
volume = {42}
journal type = {AC}
place = {Poland}
year = {1994}
month = {Dec}
}