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Statistical interpretation of electronic energy relaxation in Ce vapor

Abstract

Experimental results obtained with a set-up designed to study the physical properties of uranium surrogate vapor are presented. Cerium is evaporated to obtain systematic data in order to better understand the underlying physical properties. By a time of flight technique, the velocity was measured on the axial streamline of Ce present in the vapor produced by an electron gun. A description of the experimental set-up is given. A brief review of the T.O.F. spectrum modelization is then developed, which allows to deduce hydrodynamic velocity and axial temperature. Within a macroscopic collisional flow model, considering kinetic layer and hydrodynamic layer, a source temperature is deduced. A significant part of the internal electronic energy relaxes into translational kinetic energy. A microscopic atomic collisional mechanism, the non resonant internal energy transfer, is used to interpret this energy relaxation. The necessary probability that such collisional process occurs is estimated in order to reproduce T.O.F. spectra.
Publication Date:
Dec 31, 1992
Product Type:
Conference
Report Number:
CEA-CONF-11206; CONF-9208222-
Reference Number:
SCA: 664200; 664300; PA: AIX-24:045958; SN: 93000989121
Resource Relation:
Conference: 3. International Workshop on Separation Phenomena in Liquids and Gases,Charlottesville, VA (United States),18 Aug 1992; Other Information: PBD: 1992
Subject:
74 ATOMIC AND MOLECULAR PHYSICS; CERIUM; ATOM-ATOM COLLISIONS; VAPORS; ENERGY-LEVEL TRANSITIONS; KINETIC ENERGY; RELAXATION; TIME-OF-FLIGHT METHOD; 664200; 664300; SPECTRA OF ATOMS AND MOLECULES AND THEIR INTERACTIONS WITH PHOTONS; COLLISION PHENOMENA
OSTI ID:
10152137
Research Organizations:
CEA Centre d`Etudes de Saclay, 91 - Gif-sur-Yvette (France). Dept. des Procedes d`Enrichissement
Country of Origin:
France
Language:
English
Other Identifying Numbers:
Other: ON: DE93624898; TRN: FR9301837045958
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
FRN
Size:
[10] p.
Announcement Date:
Jul 05, 2005

Citation Formats

Blumenfeld, L, Gonella, C, and Fleche, J L. Statistical interpretation of electronic energy relaxation in Ce vapor. France: N. p., 1992. Web.
Blumenfeld, L, Gonella, C, & Fleche, J L. Statistical interpretation of electronic energy relaxation in Ce vapor. France.
Blumenfeld, L, Gonella, C, and Fleche, J L. 1992. "Statistical interpretation of electronic energy relaxation in Ce vapor." France.
@misc{etde_10152137,
title = {Statistical interpretation of electronic energy relaxation in Ce vapor}
author = {Blumenfeld, L, Gonella, C, and Fleche, J L}
abstractNote = {Experimental results obtained with a set-up designed to study the physical properties of uranium surrogate vapor are presented. Cerium is evaporated to obtain systematic data in order to better understand the underlying physical properties. By a time of flight technique, the velocity was measured on the axial streamline of Ce present in the vapor produced by an electron gun. A description of the experimental set-up is given. A brief review of the T.O.F. spectrum modelization is then developed, which allows to deduce hydrodynamic velocity and axial temperature. Within a macroscopic collisional flow model, considering kinetic layer and hydrodynamic layer, a source temperature is deduced. A significant part of the internal electronic energy relaxes into translational kinetic energy. A microscopic atomic collisional mechanism, the non resonant internal energy transfer, is used to interpret this energy relaxation. The necessary probability that such collisional process occurs is estimated in order to reproduce T.O.F. spectra.}
place = {France}
year = {1992}
month = {Dec}
}