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Competitive and successive reactions in the position cluster and energy state of positronium in the liquids; Reactions competitives et successives dans la grappe du positon et etat energetique du positonium dans les liquides

Abstract

By combining two independent positron annihilation techniques, it is shown that, in polar solvents, the halogenated compounds inhibit positronium formation by quasi-free electron scavenging followed by positron capture. This sequence occurs before halide detachment intervenes. Studying mixtures of solutes allows both to confirm the existence of these successive reactions and to stress the influence, towards positronium formation, of the trap depth for the electron captured by nitrates, whether ion associated or not, in methanol. Finally, experiments in the presence of a magnetic field allow to conclude that the formed positronium is very rapidly thermalized, then localised in a potential well in the liquids, the so-called bubble.
Authors:
Publication Date:
Oct 01, 1991
Product Type:
Thesis/Dissertation
Report Number:
CRN-CPR-91-05
Reference Number:
SCA: 664300; 664500; PA: FRD-92:000967; SN: 92000757222
Resource Relation:
Other Information: TH: These (D. es Sc.); PBD: Oct 1991
Subject:
74 ATOMIC AND MOLECULAR PHYSICS; POSITRONS; ANNIHILATION; POSITRONIUM; ENERGY LEVELS; ELECTRON CAPTURE; INHIBITION; PARTICLE PROPERTIES; MAGNETIC FIELDS; CLUSTER MODEL; SOLVENTS; LIQUIDS; SODIUM 22; CHEMICAL REACTIONS; HALIDES; NITRATES; 664300; 664500; COLLISION PHENOMENA; SPECIAL ATOMS AND MOLECULES
OSTI ID:
10149546
Research Organizations:
Strasbourg-1 Univ., 67 (France). Centre de Recherches Nucleaires; Strasbourg-1 Univ., 67 (France)
Country of Origin:
France
Language:
French
Other Identifying Numbers:
Other: ON: DE92526927; TRN: FR9200967
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
FRN
Size:
175 p.
Announcement Date:
Jul 05, 2005

Citation Formats

Didierjean, F. Competitive and successive reactions in the position cluster and energy state of positronium in the liquids; Reactions competitives et successives dans la grappe du positon et etat energetique du positonium dans les liquides. France: N. p., 1991. Web.
Didierjean, F. Competitive and successive reactions in the position cluster and energy state of positronium in the liquids; Reactions competitives et successives dans la grappe du positon et etat energetique du positonium dans les liquides. France.
Didierjean, F. 1991. "Competitive and successive reactions in the position cluster and energy state of positronium in the liquids; Reactions competitives et successives dans la grappe du positon et etat energetique du positonium dans les liquides." France.
@misc{etde_10149546,
title = {Competitive and successive reactions in the position cluster and energy state of positronium in the liquids; Reactions competitives et successives dans la grappe du positon et etat energetique du positonium dans les liquides}
author = {Didierjean, F}
abstractNote = {By combining two independent positron annihilation techniques, it is shown that, in polar solvents, the halogenated compounds inhibit positronium formation by quasi-free electron scavenging followed by positron capture. This sequence occurs before halide detachment intervenes. Studying mixtures of solutes allows both to confirm the existence of these successive reactions and to stress the influence, towards positronium formation, of the trap depth for the electron captured by nitrates, whether ion associated or not, in methanol. Finally, experiments in the presence of a magnetic field allow to conclude that the formed positronium is very rapidly thermalized, then localised in a potential well in the liquids, the so-called bubble.}
place = {France}
year = {1991}
month = {Oct}
}