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Feasibility study of the dissolution rates of uranium ore dust, uranium concentrates and uranium compounds in simulated lung fluid

Abstract

A flow-through apparatus has been devised to study the dissolution in simulated lung fluid of aerosol materials associated with the Canadian uranium industry. The apparatus has been experimentally applied over 16 day extraction periods to approximately 2g samples of < 38um and 53-75um particle-size fractions of both Elliot Lake and Mid-Western uranium ores. The extraction of uranium-238 was in the range 24-60% for these samples. The corresponding range for radium-226 was 8-26%. Thorium-230, lead-210, polonium-210, and thorium-232 were not significantly extracted. It was incidentally found that the elemental composition of the ores studied varies significantly with particle size, the radionuclide-containing minerals and several extractable stable elements being concentrated in the smaller size fraction. Samples of the refined compounds uranium dioxide and uranium trioxide were submitted to similar 16 day extraction experiments. Approximately 0.5% of the uranium was extracted from a 0.258g sample of unsintered (fluid bed) uranium dioxide of particle size < 38um. The corresponding figure for a 0.292g sample of uranium trioxide was 97%. Two aerosol samples on filters were also studied. Of the 88ug uranium initially measured on stage 2 of a cascade impactor sample collected from the yellow cake packing area of an Elliot Lake mill, essentially  More>>
Authors:
Robertson, R [1] 
  1. Becquerel Laboratories Inc., (Canada)
Publication Date:
Jul 30, 1986
Product Type:
Technical Report
Report Number:
INFO-0205
Reference Number:
SCA: 560161; PA: AIX-23:035101; SN: 92000725304
Resource Relation:
Other Information: PBD: 30 Jul 1986
Subject:
63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTANT EFFECTS ON LIVING ORGS. AND BIOL. MAT.; DUSTS; LUNGS; URANIUM ORES; DISSOLUTION; AEROSOLS; URANIUM OXIDES; 560161; MAN
OSTI ID:
10147579
Research Organizations:
Atomic Energy Control Board, Ottawa, ON (Canada)
Country of Origin:
Canada
Language:
English
Other Identifying Numbers:
Other: ON: DE92626052; TRN: CA9200194035101
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
INIS
Size:
99 p.
Announcement Date:
Jul 05, 2005

Citation Formats

Robertson, R. Feasibility study of the dissolution rates of uranium ore dust, uranium concentrates and uranium compounds in simulated lung fluid. Canada: N. p., 1986. Web.
Robertson, R. Feasibility study of the dissolution rates of uranium ore dust, uranium concentrates and uranium compounds in simulated lung fluid. Canada.
Robertson, R. 1986. "Feasibility study of the dissolution rates of uranium ore dust, uranium concentrates and uranium compounds in simulated lung fluid." Canada.
@misc{etde_10147579,
title = {Feasibility study of the dissolution rates of uranium ore dust, uranium concentrates and uranium compounds in simulated lung fluid}
author = {Robertson, R}
abstractNote = {A flow-through apparatus has been devised to study the dissolution in simulated lung fluid of aerosol materials associated with the Canadian uranium industry. The apparatus has been experimentally applied over 16 day extraction periods to approximately 2g samples of < 38um and 53-75um particle-size fractions of both Elliot Lake and Mid-Western uranium ores. The extraction of uranium-238 was in the range 24-60% for these samples. The corresponding range for radium-226 was 8-26%. Thorium-230, lead-210, polonium-210, and thorium-232 were not significantly extracted. It was incidentally found that the elemental composition of the ores studied varies significantly with particle size, the radionuclide-containing minerals and several extractable stable elements being concentrated in the smaller size fraction. Samples of the refined compounds uranium dioxide and uranium trioxide were submitted to similar 16 day extraction experiments. Approximately 0.5% of the uranium was extracted from a 0.258g sample of unsintered (fluid bed) uranium dioxide of particle size < 38um. The corresponding figure for a 0.292g sample of uranium trioxide was 97%. Two aerosol samples on filters were also studied. Of the 88ug uranium initially measured on stage 2 of a cascade impactor sample collected from the yellow cake packing area of an Elliot Lake mill, essentially 100% was extracted over a 16 day period. The corresponding figure for an open face filter sample collected in a fuel fabrication plant and initially measured at 288ug uranium was approximately 3%. Recommendations are made with regard to further work of a research nature which would be useful in this area. Recommendations are also made on sampling methods, analytical methods and extraction conditions for various aerosols of interest which are to be studied in a work of broader scope designed to yield meaningful data in connection with lung dosimetry calculations.}
place = {Canada}
year = {1986}
month = {Jul}
}