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Electronic properties of disordered silicon carbides; Proprietes electroniques des carbures de silicium desordonnes

Abstract

The disorder effects on the electronic properties of silicon carbide were studied at the atomic or micro-structural scale. We have investigated a great variety of materials: silicon carbide fibers, carbonated amorphous silicon films, single crystals and amorphous or crystalline SiC powders. The DC and AC conductivity measurements on the SiC fibers point out the major role of their micro-structure at the nanometric scale, which leads to large dielectric constants. Hopping of polaronic carriers is the dominant conduction mechanism. An electrons spin resonance study of all the materials was performed: sp{sup 2} hybridized carbon is always present, in diluted form in the amorphous systems or as free carbon in the crystalline one. Some irradiation defects of SiC were identified: silicon or carbon vacancy and carbon complexes with sp{sup 2} hybridization. Such a carbon is responsible of the low paramagnetic stability of the silicon dangling bonds. It is believed to induce the polaronic behavior of the localized carriers. (Author). refs., figs., tabs.
Authors:
Publication Date:
May 01, 1991
Product Type:
Thesis/Dissertation
Report Number:
CEA-R-5625
Reference Number:
SCA: 360204; PA: AIX-24:035424; SN: 93000976624
Resource Relation:
Other Information: TH: These (D. es Sc.).; PBD: May 1991
Subject:
36 MATERIALS SCIENCE; SILICON CARBIDES; ELECTRIC CONDUCTIVITY; ELECTRON SPIN RESONANCE; AMORPHOUS STATE; CARBON; CERAMICS; CRYSTAL DEFECTS; ELECTRON BEAMS; FIBERS; IRRADIATION; METHANE; METHYL RADICALS; MICROSTRUCTURE; MONOCRYSTALS; PARAMAGNETISM; POWDERS; SILANES; SILICON; 360204; PHYSICAL PROPERTIES
OSTI ID:
10144599
Research Organizations:
CEA Centre d`Etudes de Saclay, 91 - Gif-sur-Yvette (France). Dept. de Technologie des Materiaux; Paris-7 Univ., 75 (France)
Country of Origin:
France
Language:
French
Other Identifying Numbers:
Other: ON: DE93622202; TRN: FR9301874035424
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
FRN
Size:
[202] p.
Announcement Date:
Jul 05, 2005

Citation Formats

Chauvet, O. Electronic properties of disordered silicon carbides; Proprietes electroniques des carbures de silicium desordonnes. France: N. p., 1991. Web.
Chauvet, O. Electronic properties of disordered silicon carbides; Proprietes electroniques des carbures de silicium desordonnes. France.
Chauvet, O. 1991. "Electronic properties of disordered silicon carbides; Proprietes electroniques des carbures de silicium desordonnes." France.
@misc{etde_10144599,
title = {Electronic properties of disordered silicon carbides; Proprietes electroniques des carbures de silicium desordonnes}
author = {Chauvet, O}
abstractNote = {The disorder effects on the electronic properties of silicon carbide were studied at the atomic or micro-structural scale. We have investigated a great variety of materials: silicon carbide fibers, carbonated amorphous silicon films, single crystals and amorphous or crystalline SiC powders. The DC and AC conductivity measurements on the SiC fibers point out the major role of their micro-structure at the nanometric scale, which leads to large dielectric constants. Hopping of polaronic carriers is the dominant conduction mechanism. An electrons spin resonance study of all the materials was performed: sp{sup 2} hybridized carbon is always present, in diluted form in the amorphous systems or as free carbon in the crystalline one. Some irradiation defects of SiC were identified: silicon or carbon vacancy and carbon complexes with sp{sup 2} hybridization. Such a carbon is responsible of the low paramagnetic stability of the silicon dangling bonds. It is believed to induce the polaronic behavior of the localized carriers. (Author). refs., figs., tabs.}
place = {France}
year = {1991}
month = {May}
}