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Interaction between geosphere and biosphere in lake sediments

Abstract

One main issue in the safety assessment of nuclear repositories, in which processes influence the distribution pattern of radionuclide elements in the biopshere when released radioactivity is carried with groundwater that penetrates through the bottom sediment of a lake. To be able to evaluate the transport of elements such as thorium, uranium, and rare earth elements (REE), sampling of lake sediment cores at different Swedish sites with different degrees of groundwater leakage was performed. Different lake sediment fractions have been identified. One fraction is related to aluminosilicates (clay and sand contents), while the other major fraction contains organic material. Enrichment of uranium is observed in areas of groundwater seepage, and U-contents is correlated to the levels of organic matter. Besides a higher mobility and enrichment of uranium compared to thorium is observed. Chondrite normalised REE sediment contents have been found higher in the most reducing sediments. The weathering and deposition processes are discussed in connection with the degree of mobility of elements. Elements as titanium, zirconium and hafnium are nearly insoluble in aqueous solutions. The immobility of these elements have been confirmed by this study. Hafnium is selected to study the differentiation of the sediment fraction originating from refractory and  More>>
Authors:
Sundblad, B; Puigdomenech, I; Mathiasson, L [1] 
  1. Studsvik AB, Nykoeping (Sweden)
Publication Date:
Dec 18, 1990
Product Type:
Technical Report
Report Number:
SKB-TR-91-40
Reference Number:
SCA: 540330; 052002; PA: AIX-23:038968; SN: 92000732556
Resource Relation:
Other Information: PBD: 18 Dec 1990
Subject:
54 ENVIRONMENTAL SCIENCES; 12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES; SEDIMENTS; RADIONUCLIDE MIGRATION; HAFNIUM; LAKES; RADIOACTIVE WASTE DISPOSAL; RARE EARTHS; THORIUM; URANIUM; 540330; 052002; RADIOACTIVE MATERIALS MONITORING AND TRANSPORT; WASTE DISPOSAL AND STORAGE
OSTI ID:
10142461
Research Organizations:
Swedish Nuclear Fuel and Waste Management Co., Stockholm (Sweden)
Country of Origin:
Sweden
Language:
English
Other Identifying Numbers:
Other: ON: DE92627907; TRN: SE9200085038968
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
SWDN
Size:
111 p.
Announcement Date:
Jul 05, 2005

Citation Formats

Sundblad, B, Puigdomenech, I, and Mathiasson, L. Interaction between geosphere and biosphere in lake sediments. Sweden: N. p., 1990. Web.
Sundblad, B, Puigdomenech, I, & Mathiasson, L. Interaction between geosphere and biosphere in lake sediments. Sweden.
Sundblad, B, Puigdomenech, I, and Mathiasson, L. 1990. "Interaction between geosphere and biosphere in lake sediments." Sweden.
@misc{etde_10142461,
title = {Interaction between geosphere and biosphere in lake sediments}
author = {Sundblad, B, Puigdomenech, I, and Mathiasson, L}
abstractNote = {One main issue in the safety assessment of nuclear repositories, in which processes influence the distribution pattern of radionuclide elements in the biopshere when released radioactivity is carried with groundwater that penetrates through the bottom sediment of a lake. To be able to evaluate the transport of elements such as thorium, uranium, and rare earth elements (REE), sampling of lake sediment cores at different Swedish sites with different degrees of groundwater leakage was performed. Different lake sediment fractions have been identified. One fraction is related to aluminosilicates (clay and sand contents), while the other major fraction contains organic material. Enrichment of uranium is observed in areas of groundwater seepage, and U-contents is correlated to the levels of organic matter. Besides a higher mobility and enrichment of uranium compared to thorium is observed. Chondrite normalised REE sediment contents have been found higher in the most reducing sediments. The weathering and deposition processes are discussed in connection with the degree of mobility of elements. Elements as titanium, zirconium and hafnium are nearly insoluble in aqueous solutions. The immobility of these elements have been confirmed by this study. Hafnium is selected to study the differentiation of the sediment fraction originating from refractory and other physically weathered minerals. (au) (33 refs., 45 figs., 30 tbls.).}
place = {Sweden}
year = {1990}
month = {Dec}
}