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Formation, growth and decomposition of precipitates in Zircaloy-2 and -4

Abstract

The intermetallic precipitates in Zircaloy-2 are mainly Zr(Cr,Fe){sub 2} and Zr{sub 2}(Ni,Fe). Zircaloy-4 only has the former unless the nickel impurity level is high. These precipitates are based on the hcp ZrCr{sub 2} Laves phase and bct Zr{sub 2}Ni Zintl phase with Fe substituting for Cr and Ni in proportions that depend on the alloy composition. Their structure, composition and morphology are determined by the metallurgical history and can be changed by n eutron irradiation. Zr(Cr,Fe){sub 2} precipitates irradiated at 580 K are depleted in Fe and to a lesser extent Cr. Depletion below the stoichiometric value is coincident with transformation from a crystalline to an amorphous structure. The transformation starts at the surface of the precipitate and advances inwards with increasing fluence. No structural change has been observed in Zr{sub 2}(Ni,Fe) precipitates irradiated at 580 or 675 K. At irradiation temperatures {>=} 675 K there is solute depletion and dissolution of Zr(Cr,Fe){sub 2} precipitates but no crystalline-amorphous transformation has been observed. There is a distinct observable change in precipitate morphology with the formation of Fe rich precipitates at grain boundaries and in the matrix. Both the Zr(Cr,Fe){sub 2} and Zr{sub 2}(Ni,Fe) precipitates irradiated at 350 K undergo complete amorphous  More>>
Publication Date:
Sep 01, 1985
Product Type:
Technical Report
Report Number:
AECL-8852
Reference Number:
SCA: 360106; 400600; PA: AIX-23:034185; SN: 92000724874
Resource Relation:
Other Information: PBD: Sep 1985
Subject:
36 MATERIALS SCIENCE; 38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY; ALLOY-ZR98SN-2; PRECIPITATION; ALLOY-ZR98SN-4; CHEMICAL RADIATION EFFECTS; CHROMIUM; IRON; NEUTRONS; NICKEL; 360106; 400600; RADIATION EFFECTS; RADIATION CHEMISTRY
OSTI ID:
10139657
Research Organizations:
Atomic Energy of Canada Ltd., Chalk River, ON (Canada). Chalk River Nuclear Labs.
Country of Origin:
Canada
Language:
English
Other Identifying Numbers:
Other: ON: DE92625623; TRN: CA9200213034185
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
INIS
Size:
22 p.
Announcement Date:
Jul 05, 2005

Citation Formats

Griffiths, M, Gilbert, R W, and Cheadle, B A. Formation, growth and decomposition of precipitates in Zircaloy-2 and -4. Canada: N. p., 1985. Web.
Griffiths, M, Gilbert, R W, & Cheadle, B A. Formation, growth and decomposition of precipitates in Zircaloy-2 and -4. Canada.
Griffiths, M, Gilbert, R W, and Cheadle, B A. 1985. "Formation, growth and decomposition of precipitates in Zircaloy-2 and -4." Canada.
@misc{etde_10139657,
title = {Formation, growth and decomposition of precipitates in Zircaloy-2 and -4}
author = {Griffiths, M, Gilbert, R W, and Cheadle, B A}
abstractNote = {The intermetallic precipitates in Zircaloy-2 are mainly Zr(Cr,Fe){sub 2} and Zr{sub 2}(Ni,Fe). Zircaloy-4 only has the former unless the nickel impurity level is high. These precipitates are based on the hcp ZrCr{sub 2} Laves phase and bct Zr{sub 2}Ni Zintl phase with Fe substituting for Cr and Ni in proportions that depend on the alloy composition. Their structure, composition and morphology are determined by the metallurgical history and can be changed by n eutron irradiation. Zr(Cr,Fe){sub 2} precipitates irradiated at 580 K are depleted in Fe and to a lesser extent Cr. Depletion below the stoichiometric value is coincident with transformation from a crystalline to an amorphous structure. The transformation starts at the surface of the precipitate and advances inwards with increasing fluence. No structural change has been observed in Zr{sub 2}(Ni,Fe) precipitates irradiated at 580 or 675 K. At irradiation temperatures {>=} 675 K there is solute depletion and dissolution of Zr(Cr,Fe){sub 2} precipitates but no crystalline-amorphous transformation has been observed. There is a distinct observable change in precipitate morphology with the formation of Fe rich precipitates at grain boundaries and in the matrix. Both the Zr(Cr,Fe){sub 2} and Zr{sub 2}(Ni,Fe) precipitates irradiated at 350 K undergo complete amorphous transformation although solute depletion has not been observed.}
place = {Canada}
year = {1985}
month = {Sep}
}