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Study of point defect mobilities in zirconium during electron irradiation in a HVEM

Abstract

A high voltage electron microscope (HVEM) was used to investigate the nature of intrinsic point defects in {alpha}-Zr by direct observation of dislocation climb and cavity growth or shrinkage. The material used was Marz-grade Zr that had been pre-irradiated with neutrons at about 740 K in the Dounreay Fast Reactor. Dislocation loops of vacancy character that had been produced during the neutron irradiation were studied by further irradiation with electrons in the HVEM. Growth of the loops was observed at temperatures as low as 230 K, indicating that, under the conditions of the experiment, some vacancy-type defects were mobile in the temperature regime 230 K-300 K. The nature of these defects is unknown. One possibility is that these defects are not intrinsic in nature, but may be vacancy-Fe complexes. In addition to the climb of dislocation loops, c-component network dislocations and cavities were also studied. Basal plane climb of the network dislocations was observed at 573 K, but was not readily apparent at 320 K. This suggests that preferred climb planes (and possibly loop habit planes) are sensitive to temperature. Cavities that were already in the foil after neutron irradiation or were induced by electron irradiation grew along the c-axis  More>>
Authors:
Griffiths, M; [1]  Styles, R C; Woo, C H; [2]  Phillip, F; Frank, W [3] 
  1. Atomic Energy of Canada Ltd., Chalk River, ON (Canada). Chalk River Nuclear Labs.
  2. Atomic Energy of Canada Ltd., Pinawa, MB (Canada). Whiteshell Nuclear Research Establishment
  3. Max-Planck-Institut fuer Metallforschung, Stuttgart (Germany)
Publication Date:
Jan 01, 1993
Product Type:
Technical Report
Report Number:
AECL-10801; COG-92-40.
Reference Number:
SCA: 360102; PA: AIX-25:024869; EDB-94:052914; NTS-94:016653; SN: 94001174328
Resource Relation:
Other Information: PBD: Jan 1993
Subject:
36 MATERIALS SCIENCE; ZIRCONIUM; POINT DEFECTS; CONTRACTION; DISLOCATIONS; ELECTRON MICROSCOPES; ELONGATION; EXPERIMENTAL DATA; PHYSICAL RADIATION EFFECTS; TEMPERATURE DEPENDENCE; TEMPERATURE RANGE 0065-0273 K; TEMPERATURE RANGE 0273-0400 K; TEMPERATURE RANGE 0400-1000 K; 360102; STRUCTURE AND PHASE STUDIES
OSTI ID:
10138340
Research Organizations:
Atomic Energy of Canada Ltd., Chalk River, ON (Canada). Chalk River Nuclear Labs.
Country of Origin:
Canada
Language:
English
Other Identifying Numbers:
Other: ON: DE94619028; TRN: CA9400065024869
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
INIS
Size:
23 p.
Announcement Date:
Jul 05, 2005

Citation Formats

Griffiths, M, Styles, R C, Woo, C H, Phillip, F, and Frank, W. Study of point defect mobilities in zirconium during electron irradiation in a HVEM. Canada: N. p., 1993. Web.
Griffiths, M, Styles, R C, Woo, C H, Phillip, F, & Frank, W. Study of point defect mobilities in zirconium during electron irradiation in a HVEM. Canada.
Griffiths, M, Styles, R C, Woo, C H, Phillip, F, and Frank, W. 1993. "Study of point defect mobilities in zirconium during electron irradiation in a HVEM." Canada.
@misc{etde_10138340,
title = {Study of point defect mobilities in zirconium during electron irradiation in a HVEM}
author = {Griffiths, M, Styles, R C, Woo, C H, Phillip, F, and Frank, W}
abstractNote = {A high voltage electron microscope (HVEM) was used to investigate the nature of intrinsic point defects in {alpha}-Zr by direct observation of dislocation climb and cavity growth or shrinkage. The material used was Marz-grade Zr that had been pre-irradiated with neutrons at about 740 K in the Dounreay Fast Reactor. Dislocation loops of vacancy character that had been produced during the neutron irradiation were studied by further irradiation with electrons in the HVEM. Growth of the loops was observed at temperatures as low as 230 K, indicating that, under the conditions of the experiment, some vacancy-type defects were mobile in the temperature regime 230 K-300 K. The nature of these defects is unknown. One possibility is that these defects are not intrinsic in nature, but may be vacancy-Fe complexes. In addition to the climb of dislocation loops, c-component network dislocations and cavities were also studied. Basal plane climb of the network dislocations was observed at 573 K, but was not readily apparent at 320 K. This suggests that preferred climb planes (and possibly loop habit planes) are sensitive to temperature. Cavities that were already in the foil after neutron irradiation or were induced by electron irradiation grew along the c-axis and shrank along a-directions during electron irradiation. This radiation-induced shape change of the cavities strongly suggests the existence of a diffusional anisotropy difference between interstitials and vacancies in {alpha}-Zr. (Author) 14 figs., 22 refs.}
place = {Canada}
year = {1993}
month = {Jan}
}