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Measurements of atmospheric trace gas concentrations during the field campaign in Juelich 1988

Abstract

Our current understanding of the gas phase chemistry of the lower troposphere is based on measurements of trace gas concentrations in the atmosphere, laboratory studies of gas phase reactions and model calculations of the relevant chemical processes. The ultimate validation of a reaction scheme can only be derived from a comparison of model results with experimental data from measurements in the atmosphere. In order to establish an extended and reliable experimental data set on which such a comparison could be based the Institut fuer Atmosphaerische Chemie of the Forschungszentrum Juelich (KFA) has been conducting field campaigns for a number of years. One such campaign took place in Juelich from May 9 - June 10 in 1988. Many of the relevant trace species were measured on a continuous basis together with photolysis frequencies and meteorological parameters. All measurements were ground based and included OH, O{sub 3}, NO, and NO{sub 2}, NO{sub y}, HCHO, SO{sub 2}, CH{sub 4}, CO, non methane hydrocarbons up to C{sub 5}, peroxyacetylnitrate, and aldehydes. The photolysis frequencies of O{sub 3} and NO{sub 2} were also monitored, as were atmospheric temperature, relative humidity, wind speed, and wind direction. All quantities were measured in-situ except OH and SO{sub 2},  More>>
Publication Date:
Feb 01, 1993
Product Type:
Technical Report
Report Number:
Juel-2731
Reference Number:
SCA: 540120; PA: DE-94:0G2001; EDB-94:039591; NTS-94:011778; ERA-19:010306; SN: 94001157220
Resource Relation:
Other Information: PBD: Feb 1993
Subject:
54 ENVIRONMENTAL SCIENCES; ATMOSPHERIC CHEMISTRY; MEASURING METHODS; NITROGEN OXIDES; OZONE; FORMALDEHYDE; SULFUR DIOXIDE; CARBON MONOXIDE; METHANE; FIELD TESTS; BENCH-SCALE EXPERIMENTS; 540120; CHEMICALS MONITORING AND TRANSPORT
OSTI ID:
10130087
Research Organizations:
Forschungszentrum Juelich GmbH (Germany). Inst. fuer Chemie und Dynamik der Geosphaere 3: Atmosphaerische Chemie
Country of Origin:
Germany
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0366-0885; Other: ON: DE94746032; TRN: DE94G2001
Availability:
OSTI; NTIS (US Sales Only)
Submitting Site:
DE
Size:
170 p.
Announcement Date:
Jul 04, 2005

Citation Formats

Poppe, D, Bauer, R, Brauers, T, Bruening, D, Callies, J, Dorn, H P, Hofzumahaus, A, Johnen, F J, Khedim, A, Koppmann, R, London, H, Mueller, K P, Neuroth, R, Plass-Duelmer, C, Platt, U, Rohrer, F, Rudolph, J, Schmidt, U, Wallasch, M, and Ehhalt, D H. Measurements of atmospheric trace gas concentrations during the field campaign in Juelich 1988. Germany: N. p., 1993. Web.
Poppe, D, Bauer, R, Brauers, T, Bruening, D, Callies, J, Dorn, H P, Hofzumahaus, A, Johnen, F J, Khedim, A, Koppmann, R, London, H, Mueller, K P, Neuroth, R, Plass-Duelmer, C, Platt, U, Rohrer, F, Rudolph, J, Schmidt, U, Wallasch, M, & Ehhalt, D H. Measurements of atmospheric trace gas concentrations during the field campaign in Juelich 1988. Germany.
Poppe, D, Bauer, R, Brauers, T, Bruening, D, Callies, J, Dorn, H P, Hofzumahaus, A, Johnen, F J, Khedim, A, Koppmann, R, London, H, Mueller, K P, Neuroth, R, Plass-Duelmer, C, Platt, U, Rohrer, F, Rudolph, J, Schmidt, U, Wallasch, M, and Ehhalt, D H. 1993. "Measurements of atmospheric trace gas concentrations during the field campaign in Juelich 1988." Germany.
@misc{etde_10130087,
title = {Measurements of atmospheric trace gas concentrations during the field campaign in Juelich 1988}
author = {Poppe, D, Bauer, R, Brauers, T, Bruening, D, Callies, J, Dorn, H P, Hofzumahaus, A, Johnen, F J, Khedim, A, Koppmann, R, London, H, Mueller, K P, Neuroth, R, Plass-Duelmer, C, Platt, U, Rohrer, F, Rudolph, J, Schmidt, U, Wallasch, M, and Ehhalt, D H}
abstractNote = {Our current understanding of the gas phase chemistry of the lower troposphere is based on measurements of trace gas concentrations in the atmosphere, laboratory studies of gas phase reactions and model calculations of the relevant chemical processes. The ultimate validation of a reaction scheme can only be derived from a comparison of model results with experimental data from measurements in the atmosphere. In order to establish an extended and reliable experimental data set on which such a comparison could be based the Institut fuer Atmosphaerische Chemie of the Forschungszentrum Juelich (KFA) has been conducting field campaigns for a number of years. One such campaign took place in Juelich from May 9 - June 10 in 1988. Many of the relevant trace species were measured on a continuous basis together with photolysis frequencies and meteorological parameters. All measurements were ground based and included OH, O{sub 3}, NO, and NO{sub 2}, NO{sub y}, HCHO, SO{sub 2}, CH{sub 4}, CO, non methane hydrocarbons up to C{sub 5}, peroxyacetylnitrate, and aldehydes. The photolysis frequencies of O{sub 3} and NO{sub 2} were also monitored, as were atmospheric temperature, relative humidity, wind speed, and wind direction. All quantities were measured in-situ except OH and SO{sub 2}, which were exclusively measured by a long path differential optical absorption technique. HCHO, NO{sub 2}, and O{sub 3} were determined by in-situ and also by long-path-absorption methods for intercomparison. (orig./EF)}
place = {Germany}
year = {1993}
month = {Feb}
}