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Thermogravimetric studies of vapour-aerosol interactions

Abstract

Thermogravimetric analysis has been used to study the interaction of iodine vapour with cadmium, silver and manganese monoxide substrates. These studies have demonstrated the importance of time-dependence data on reaction rates. Iodine did not react with manganese monoxide (as expected from thermodynamic considerations); however, extensive reaction did occur with silver and cadmium. Two rate limiting mechanisms were observed: mass transfer of iodine molecules from the gas phase (leading to linear reaction rates) and parabolic kinetics (ie inversely proportional to the extent of reaction) when the rate was limited by a diffusion process through the reaction product. (author).
Authors:
Henshaw, J; [1]  Newland, M S; Wood, S J
  1. AEA Reactor Services, Harwell (United Kingdom)
Publication Date:
Jan 01, 1991
Product Type:
Technical Report
Report Number:
AEA-TRS-5074
Reference Number:
SCA: 400702; PA: AIX-23:024835; SN: 92000684842
Resource Relation:
Other Information: PBD: Jan 1991
Subject:
38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY; AEROSOLS; THERMAL GRAVIMETRIC ANALYSIS; FISSION PRODUCTS; CADMIUM; IODINE; MANGANESE OXIDES; REACTION KINETICS; REACTOR ACCIDENTS; SILVER; 400702; PROPERTIES OF RADIOACTIVE MATERIALS
OSTI ID:
10128060
Research Organizations:
AEA Reactor Services, Winfrith (United Kingdom)
Country of Origin:
United Kingdom
Language:
English
Other Identifying Numbers:
Other: ON: DE92619784; TRN: GB9200118024835
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
GBN
Size:
40 p.
Announcement Date:
Jul 04, 2005

Citation Formats

Henshaw, J, Newland, M S, and Wood, S J. Thermogravimetric studies of vapour-aerosol interactions. United Kingdom: N. p., 1991. Web.
Henshaw, J, Newland, M S, & Wood, S J. Thermogravimetric studies of vapour-aerosol interactions. United Kingdom.
Henshaw, J, Newland, M S, and Wood, S J. 1991. "Thermogravimetric studies of vapour-aerosol interactions." United Kingdom.
@misc{etde_10128060,
title = {Thermogravimetric studies of vapour-aerosol interactions}
author = {Henshaw, J, Newland, M S, and Wood, S J}
abstractNote = {Thermogravimetric analysis has been used to study the interaction of iodine vapour with cadmium, silver and manganese monoxide substrates. These studies have demonstrated the importance of time-dependence data on reaction rates. Iodine did not react with manganese monoxide (as expected from thermodynamic considerations); however, extensive reaction did occur with silver and cadmium. Two rate limiting mechanisms were observed: mass transfer of iodine molecules from the gas phase (leading to linear reaction rates) and parabolic kinetics (ie inversely proportional to the extent of reaction) when the rate was limited by a diffusion process through the reaction product. (author).}
place = {United Kingdom}
year = {1991}
month = {Jan}
}