You need JavaScript to view this

The solubility of uranium in cementitious near-field chemical conditions

Abstract

Tetravalent and hexavalent uranium solubilities have been measured in cement-equilibriated water for pH values from 4 to 13. Tetravalent uranium solubilities at pH 12 have been measured by three experimental techniques: oversaturation, undersaturation and by the use of an electrochemical cell which controlled the redox conditions. The experimentally obtained data have been simulated using the thermodynamic equilibrium program HARPHRQ in conjunction with three different sets of thermodynamic data for uranium. In each case, differences were found between the predicted and measured uranium behaviour. For hexavalent uranium at high pH values the model suggested the formation of anionic hydrolysis products which led to the prediction of uranium solubilities significantly higher than those observed. Refinement of the thermodynamic data used in the model enabled the derivation of maximum values for the formation constants of these species under cementitious conditions. Similarly, the experimental data have been used to refine a model of tetravalent uranium solubility under cementitious near-field conditions. (author).
Authors:
Baston, G M.N.; Brownsword, M; Cross, J E; Hobley, J; Moreton, A D; Smith-Briggs, J L; Thomason, H P [1] 
  1. AEA Decommissioning and Waste Management, Harwell (United Kingdom)
Publication Date:
May 01, 1993
Product Type:
Technical Report
Report Number:
NSS/R-222
Reference Number:
SCA: 540330; PA: AIX-25:009100; EDB-94:039912; ERA-19:010440; NTS-94:015168; SN: 94001151409
Resource Relation:
Other Information: PBD: May 1993
Subject:
54 ENVIRONMENTAL SCIENCES; RADIOACTIVE WASTE DISPOSAL; THERMODYNAMIC MODEL; URANIUM; SOLUBILITY; CHEMICAL STATE; ENVIRONMENTAL IMPACTS; H CODES; PH VALUE; REDOX POTENTIAL; 540330; RADIOACTIVE MATERIALS MONITORING AND TRANSPORT
OSTI ID:
10126962
Research Organizations:
United Kingdom Nirex Ltd., Harwell (United Kingdom)
Country of Origin:
United Kingdom
Language:
English
Other Identifying Numbers:
Other: ON: DE94613175; TRN: GB9303784009100
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
GBN
Size:
28 p.
Announcement Date:
Jul 04, 2005

Citation Formats

Baston, G M.N., Brownsword, M, Cross, J E, Hobley, J, Moreton, A D, Smith-Briggs, J L, and Thomason, H P. The solubility of uranium in cementitious near-field chemical conditions. United Kingdom: N. p., 1993. Web.
Baston, G M.N., Brownsword, M, Cross, J E, Hobley, J, Moreton, A D, Smith-Briggs, J L, & Thomason, H P. The solubility of uranium in cementitious near-field chemical conditions. United Kingdom.
Baston, G M.N., Brownsword, M, Cross, J E, Hobley, J, Moreton, A D, Smith-Briggs, J L, and Thomason, H P. 1993. "The solubility of uranium in cementitious near-field chemical conditions." United Kingdom.
@misc{etde_10126962,
title = {The solubility of uranium in cementitious near-field chemical conditions}
author = {Baston, G M.N., Brownsword, M, Cross, J E, Hobley, J, Moreton, A D, Smith-Briggs, J L, and Thomason, H P}
abstractNote = {Tetravalent and hexavalent uranium solubilities have been measured in cement-equilibriated water for pH values from 4 to 13. Tetravalent uranium solubilities at pH 12 have been measured by three experimental techniques: oversaturation, undersaturation and by the use of an electrochemical cell which controlled the redox conditions. The experimentally obtained data have been simulated using the thermodynamic equilibrium program HARPHRQ in conjunction with three different sets of thermodynamic data for uranium. In each case, differences were found between the predicted and measured uranium behaviour. For hexavalent uranium at high pH values the model suggested the formation of anionic hydrolysis products which led to the prediction of uranium solubilities significantly higher than those observed. Refinement of the thermodynamic data used in the model enabled the derivation of maximum values for the formation constants of these species under cementitious conditions. Similarly, the experimental data have been used to refine a model of tetravalent uranium solubility under cementitious near-field conditions. (author).}
place = {United Kingdom}
year = {1993}
month = {May}
}