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Extraction of nitric acid and perchloric acid with N,N,N`,N`-tetraalkyl 2-alkyl propane 1,3-diamides; Extractions des acides: HNO{sub 3} et HClO{sub 4} par les N,N,N`,N`-tetraalkyl-alkyl-2 propane diamides-1,3

Abstract

The N,N`-dimethyl N,N`-dibutyl tetradecylmalonamide (DMDBTDMA) with an aliphatic diluent can extract trivalent actinides from nitric solutions. Then it is useful to know extraction equilibria of nitric acid with these molecules. They are determined from partition coefficients in function of acidity and amide concentration, and determination of water in the organic phase. Aggregates of diamide molecules are formed in non-acid solutions. Structures of complexes are determined by infrared spectroscopy. The same study is carried out for perchloric acid.
Publication Date:
Dec 31, 1992
Product Type:
Conference
Report Number:
CEA-CONF-11074; CONF-9205295-
Reference Number:
SCA: 050800; 400105; PA: AIX-24:005111; SN: 93000930347
Resource Relation:
Conference: 22. CONCOORD conference,Paris (France),18-21 May 1992; Other Information: PBD: 1992
Subject:
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS; 37 INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY; NITRIC ACID; SOLVENT EXTRACTION; PERCHLORIC ACID; AGGLOMERATION; AMIDES; DISTRIBUTION FUNCTIONS; INFRARED SPECTRA; QUANTITY RATIO; REPROCESSING; 050800; 400105; SPENT FUELS REPROCESSING; SEPARATION PROCEDURES
OSTI ID:
10123435
Research Organizations:
CEA Centre d`Etudes de la Vallee du Rhone, 30 - Marcoule (France). Dept. des Procedes de Retraitement
Country of Origin:
France
Language:
French
Other Identifying Numbers:
Other: ON: DE93610898; TRN: FR9300184005111
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
FRN
Size:
[7] p.
Announcement Date:
Jul 04, 2005

Citation Formats

Nigond, L, Musikas, C, and Cuillerdier, C. Extraction of nitric acid and perchloric acid with N,N,N`,N`-tetraalkyl 2-alkyl propane 1,3-diamides; Extractions des acides: HNO{sub 3} et HClO{sub 4} par les N,N,N`,N`-tetraalkyl-alkyl-2 propane diamides-1,3. France: N. p., 1992. Web.
Nigond, L, Musikas, C, & Cuillerdier, C. Extraction of nitric acid and perchloric acid with N,N,N`,N`-tetraalkyl 2-alkyl propane 1,3-diamides; Extractions des acides: HNO{sub 3} et HClO{sub 4} par les N,N,N`,N`-tetraalkyl-alkyl-2 propane diamides-1,3. France.
Nigond, L, Musikas, C, and Cuillerdier, C. 1992. "Extraction of nitric acid and perchloric acid with N,N,N`,N`-tetraalkyl 2-alkyl propane 1,3-diamides; Extractions des acides: HNO{sub 3} et HClO{sub 4} par les N,N,N`,N`-tetraalkyl-alkyl-2 propane diamides-1,3." France.
@misc{etde_10123435,
title = {Extraction of nitric acid and perchloric acid with N,N,N`,N`-tetraalkyl 2-alkyl propane 1,3-diamides; Extractions des acides: HNO{sub 3} et HClO{sub 4} par les N,N,N`,N`-tetraalkyl-alkyl-2 propane diamides-1,3}
author = {Nigond, L, Musikas, C, and Cuillerdier, C}
abstractNote = {The N,N`-dimethyl N,N`-dibutyl tetradecylmalonamide (DMDBTDMA) with an aliphatic diluent can extract trivalent actinides from nitric solutions. Then it is useful to know extraction equilibria of nitric acid with these molecules. They are determined from partition coefficients in function of acidity and amide concentration, and determination of water in the organic phase. Aggregates of diamide molecules are formed in non-acid solutions. Structures of complexes are determined by infrared spectroscopy. The same study is carried out for perchloric acid.}
place = {France}
year = {1992}
month = {Dec}
}