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Pretreatment of phosphoric acid of Annaba; Pretraitement de l`acide phosphorique de Annaba

Abstract

The most important step in the process of uranium recovery from phosphoric acid is the pretreatment operation. In this study, the adsorption of organic matters on activated carbon was carried out in a batch process and in a fixed bed column. First, the chemical and physical characterization of phosphoric acid, activated carbon and gypsum were performed. In addition, the organic matters were qualitatively analysed and a new and original quantitative method was experimented. Next, the various operating parameters such as agitation speed, granulometry, temperature, solid/liquid ratio, initial concentration, acid flowrate, and bed height were optimized. The experimental equilibrium isotherm was compared to the Langmuir, Freundlich, and Redlich-Peterson theoretical isotherms. It was noticed that the three models did not fit the experimental isotherm in the total concentration range. Thus, an original bilinear model was proposed. The influence of the operating conditions on the adsorption kinetics was also investigated. As a result of that, a new mathematical model was proposed to determine both the liquid and solid phases mass transfer and the solid phase diffusion coefficient. Finally, adsorption of organic matters on a fixed bed process allowed computation of the number of transfer units (NTU), the height of adsorption zone and the  More>>
Authors:
Publication Date:
Mar 01, 1990
Product Type:
Technical Report
Report Number:
INIS-mf-13094
Reference Number:
SCA: 050400; PA: AIX-23:018571; SN: 92000664411
Resource Relation:
Other Information: PBD: Mar 1990
Subject:
11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS; ACTIVATED CARBON; SORPTIVE PROPERTIES; PHOSPHORIC ACID; URANIUM PHOSPHATES; SEPARATION PROCESSES; ORGANIC COMPOUNDS; ADSORPTION; URANIUM; RECOVERY; ALGERIA; VAN DER WAALS FORCES; GYPSUM; KINETICS; ADSORPTION ISOTHERMS; MATHEMATICAL MODELS; 050400; FEED PROCESSING
OSTI ID:
10121148
Research Organizations:
Centre de Developpement des Materiaux, Algiers (Algeria). Lab. d`Analyse
Country of Origin:
Algeria
Language:
French
Other Identifying Numbers:
Other: ON: DE92617629; TRN: DZ9100072018571
Availability:
OSTI; NTIS (US Sales Only); INIS
Submitting Site:
INIS
Size:
85 p.
Announcement Date:
Jun 30, 2005

Citation Formats

Kada, R. Pretreatment of phosphoric acid of Annaba; Pretraitement de l`acide phosphorique de Annaba. Algeria: N. p., 1990. Web.
Kada, R. Pretreatment of phosphoric acid of Annaba; Pretraitement de l`acide phosphorique de Annaba. Algeria.
Kada, R. 1990. "Pretreatment of phosphoric acid of Annaba; Pretraitement de l`acide phosphorique de Annaba." Algeria.
@misc{etde_10121148,
title = {Pretreatment of phosphoric acid of Annaba; Pretraitement de l`acide phosphorique de Annaba}
author = {Kada, R}
abstractNote = {The most important step in the process of uranium recovery from phosphoric acid is the pretreatment operation. In this study, the adsorption of organic matters on activated carbon was carried out in a batch process and in a fixed bed column. First, the chemical and physical characterization of phosphoric acid, activated carbon and gypsum were performed. In addition, the organic matters were qualitatively analysed and a new and original quantitative method was experimented. Next, the various operating parameters such as agitation speed, granulometry, temperature, solid/liquid ratio, initial concentration, acid flowrate, and bed height were optimized. The experimental equilibrium isotherm was compared to the Langmuir, Freundlich, and Redlich-Peterson theoretical isotherms. It was noticed that the three models did not fit the experimental isotherm in the total concentration range. Thus, an original bilinear model was proposed. The influence of the operating conditions on the adsorption kinetics was also investigated. As a result of that, a new mathematical model was proposed to determine both the liquid and solid phases mass transfer and the solid phase diffusion coefficient. Finally, adsorption of organic matters on a fixed bed process allowed computation of the number of transfer units (NTU), the height of adsorption zone and the degree of saturation of activated carbon.}
place = {Algeria}
year = {1990}
month = {Mar}
}