Production of isotopes using high power proton beams

Nolen, Jerry A.; Gomes, Itacil C.

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Title: Production of isotopes using high power proton beams

Abstract

The invention provides for a method for producing isotopes using a beam of particles from an accelerator, whereby the beam is maintained at between about 70 to 2000 MeV; and contacting a thorium-containing target with the particles. The medically important isotope .sup.225Ac is produced via the nuclear reaction (p,2p6n), whereby an energetic proton causes the ejection of 2 protons and 6 neutrons from a .sup.232Th target nucleus. Another medically important isotope .sup.213Bi is then available as a decay product. The production of highly purified .sup.211At is also provided.

Inventors:: Nolen, Jr., Jerry A.; Gomes, Itacil C.

Issue Date:: Tue Apr 02 00:00:00 EDT 2019

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1568155

Patent Number(s):: 10249399

Application Number:: 14/949,665

Assignee:: UChicago Argonne, LLC (Chicago, IL)

Patent Classifications (CPCs):: G - PHYSICS G21 - NUCLEAR PHYSICS G21G - CONVERSION OF CHEMICAL ELEMENTS

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G - PHYSICS G21 - NUCLEAR PHYSICS G21G - CONVERSION OF CHEMICAL ELEMENTS
G21G1/001 - {Recovery of specific isotopes from irradiated targets}
G21G1/10 - by bombardment with electrically charged particles
G21G2001/0084 - {Bismuth}
G21G2001/0089 - {Actinium}
G21G2001/0094 - {Other isotopes not provided for in the groups listed above}

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DOE Contract Number:: AC02-06CH11357

Resource Type:: Patent

Resource Relation:: Patent File Date: 11/23/2015

Country of Publication:: United States

Language:: English

Citation Formats


                    Nolen, Jr., Jerry A., and Gomes, Itacil C. Production of isotopes using high power proton beams.  United States: N. p., 2019. 
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                    Nolen, Jr., Jerry A., & Gomes, Itacil C. Production of isotopes using high power proton beams.  United States.

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                    Nolen, Jr., Jerry A., and Gomes, Itacil C. Tue .  
        "Production of isotopes using high power proton beams".  United States.  https://www.osti.gov/servlets/purl/1568155.

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@article{osti_1568155,

  title        = {Production of isotopes using high power proton beams},

  author       = {Nolen, Jr., Jerry A. and Gomes, Itacil C.},

  abstractNote = {The invention provides for a method for producing isotopes using a beam of particles from an accelerator, whereby the beam is maintained at between about 70 to 2000 MeV; and contacting a thorium-containing target with the particles. The medically important isotope .sup.225Ac is produced via the nuclear reaction (p,2p6n), whereby an energetic proton causes the ejection of 2 protons and 6 neutrons from a .sup.232Th target nucleus. Another medically important isotope .sup.213Bi is then available as a decay product. The production of highly purified .sup.211At is also provided.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {Tue Apr 02 00:00:00 EDT 2019},

  month        = {Tue Apr 02 00:00:00 EDT 2019}

}

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Works referenced in this record:

Actinium-225 complexes and conjugates for targeted radiotherapy
patent, December 2003

Frank, R. Keith; Kiefer, Garry E.; Simon, Jaime
US Patent Document 6,670,456
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6670456

Method for Production of Radioisotope Preparations and Their Use in Life Science, Research, Medical Application and Industry
patent-application, June 2009

Ravn, Helge Leif; Beyer, Gerd Juergen; Koester, Ulli
US Patent Application 11/814035; 20090162278
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20090162278

Method for the simultaneous preparation of Radon-211, Xenon-125, Xenon-123, Astatine-211, Iodine-125 and Iodine-123
patent, May 1987

Mirzadeh, Saed; Lambrecht, Richard M.
US Patent Document 4,664,869
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/4664869

Process for producing astatine-211 for radiopharmaceutical use
patent, July 1987

Mirzadeh, Saed; Lambrecht, Richard M.
US Patent Document 4,681,727
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/4681727

Transmutable radiotherapy device
patent, September 2001

Sioshansi, Piran; Bricault, Raymond J.
US Patent Document 6,293,899
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6293899

Spallation device for producing neutrons
patent, May 2005

Ritter, Guillaume
US Patent Document 6,895,064
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6895064

Actinium radioisotope products of enhanced purity
patent, June 2010

Meikrantz, David H.; Todd, Terry A.; Tranter, Troy J.
US Patent Document 7,736,610
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7736610

Method for producing Ac-225 by irradiation of Ra-226 with protons
patent, October 2001

Apostolidis, Christos; Janssens, Willem; Koch, Lothar
US Patent Document 6,299,666
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6299666

Radiotherapy
patent, June 2006

Larsen, Roy H.; Henriksen, Gjermund
US Patent Document 7,056,275
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7056275

Aqueous liquid bleaching detergents which are stable during storage and washing process
patent, November 1992

Carron, Henry; Jourdan-Laforte, Eric
US Patent Document 5,160,656
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/5160656

Process and apparatus for the production of BI-213 cations
patent, December 1998

Horwitz, E. Philip; Hines, John J.; Chiarizia, Renato
US Patent Document 5,854,968
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/5854968

Separation of Actinium and Thorium from Uranium and Its Daughters
patent, March 1969

Swanson, Donald H.
US Patent Document 3434809
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/3434809

Target arrangement for spallation-neutron-sources
patent, April 1986

Bauer, Gunter
US Patent Document 4,582,667
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/4582667

Multicolumn selectivity inversion generator for production of high purity actinium for use in therapeutic nuclear medicine
patent-application, October 2002

Bond, Andrew H.; Horwitz, E. Philip; McAlister, Daniel R.
US Patent Application 10/261031; 20030194364
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20030194364

Method of producing Actinium-225 and daughters
patent, January 2004

Satz, Stanley; Schenter, Scott
US Patent Document 6,680,993
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6680993

Method for producing actinium-225 and bismuth-213
patent, October 1994

van Geel, Jacobus N. C.; Fuger, Jean J.; Koch, Lothar
US Patent Document 5,355,394
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/5355394

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The invention provides for a method for producing isotopes using a beam of particles from an accelerator, whereby the beam is maintained at between about 70 to 2000 MeV; and contacting a thorium-containing target with the particles. The medically important isotope .sup.225Ac is produced via the nuclear reaction (p,2p6n), whereby an energetic proton causes the ejection of 2 protons and 6 neutrons from a .sup.232Th target nucleus. Another medically important isotope .sup.213Bi is then available as a decay product. The production of highly purified .sup.211At is also provided.
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Similar Records

Title: Production of isotopes using high power proton beams

Abstract

Citation Formats

Actinium-225 complexes and conjugates for targeted radiotherapy patent, December 2003

Method for Production of Radioisotope Preparations and Their Use in Life Science, Research, Medical Application and Industry patent-application, June 2009

Method for the simultaneous preparation of Radon-211, Xenon-125, Xenon-123, Astatine-211, Iodine-125 and Iodine-123 patent, May 1987

Process for producing astatine-211 for radiopharmaceutical use patent, July 1987

Transmutable radiotherapy device patent, September 2001

Spallation device for producing neutrons patent, May 2005

Actinium radioisotope products of enhanced purity patent, June 2010

Method for producing Ac-225 by irradiation of Ra-226 with protons patent, October 2001

Radiotherapy patent, June 2006

Aqueous liquid bleaching detergents which are stable during storage and washing process patent, November 1992

Process and apparatus for the production of BI-213 cations patent, December 1998

Separation of Actinium and Thorium from Uranium and Its Daughters patent, March 1969

Target arrangement for spallation-neutron-sources patent, April 1986

Multicolumn selectivity inversion generator for production of high purity actinium for use in therapeutic nuclear medicine patent-application, October 2002

Method of producing Actinium-225 and daughters patent, January 2004

Method for producing actinium-225 and bismuth-213 patent, October 1994

Actinium-225 complexes and conjugates for targeted radiotherapy
patent, December 2003

Method for Production of Radioisotope Preparations and Their Use in Life Science, Research, Medical Application and Industry
patent-application, June 2009

Method for the simultaneous preparation of Radon-211, Xenon-125, Xenon-123, Astatine-211, Iodine-125 and Iodine-123
patent, May 1987

Process for producing astatine-211 for radiopharmaceutical use
patent, July 1987

Transmutable radiotherapy device
patent, September 2001

Spallation device for producing neutrons
patent, May 2005

Actinium radioisotope products of enhanced purity
patent, June 2010

Method for producing Ac-225 by irradiation of Ra-226 with protons
patent, October 2001

Radiotherapy
patent, June 2006

Aqueous liquid bleaching detergents which are stable during storage and washing process
patent, November 1992

Process and apparatus for the production of BI-213 cations
patent, December 1998

Separation of Actinium and Thorium from Uranium and Its Daughters
patent, March 1969

Target arrangement for spallation-neutron-sources
patent, April 1986

Multicolumn selectivity inversion generator for production of high purity actinium for use in therapeutic nuclear medicine
patent-application, October 2002

Method of producing Actinium-225 and daughters
patent, January 2004

Method for producing actinium-225 and bismuth-213
patent, October 1994