Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation

Lyons, James E

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Title: Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation

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Abstract

New compositions of matter comprising cyano-substituted metal complexes of porphyrins are catalysts for the oxidation of alkanes. The metal is iron, chromium, manganese, ruthenium, copper or cobalt. The porphyrin ring has cyano groups attached thereto in meso and/or .beta.-pyrrolic positions.

Inventors:

Ellis, Jr., Paul E. ^[1]; Lyons, James E ^[2]

(Downingtown, PA)
Wallingford, PA

Issue Date:: 1995-01-01

Research Org.:: Sun Refining and Marketing Co., Marcus Hook, PA (United States)

OSTI Identifier:: 869710

Patent Number(s):: 5382662

Assignee:: Sun Company, Inc. (R&M) (Philadelphia, PA)

Patent Classifications (CPCs):: B - PERFORMING OPERATIONS B01 - PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL B01J - CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY

C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07C - ACYCLIC OR CARBOCYCLIC COMPOUNDS

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B - PERFORMING OPERATIONS B01 - PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL B01J - CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY
B01J2531/025 - Ligands with a porphyrin ring system or analogues thereof, e.g. phthalocyanines, corroles
B01J2531/16 - Copper
B01J2531/62 - Chromium
B01J2531/72 - Manganese
B01J2531/821 - Ruthenium
B01J2531/842 - Iron
B01J2531/845 - Cobalt
B01J31/1815 - {with more than one complexing nitrogen atom, e.g. bipyridyl, 2-aminopyridine}

C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07C - ACYCLIC OR CARBOCYCLIC COMPOUNDS
C07C29/50 - with molecular oxygen only
C07C31/12 - containing four carbon atoms
C07C45/33 - of CHx-moieties
C07C45/34 - in unsaturated compounds

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DOE Contract Number:: FC21-90MC26029

Resource Type:: Patent

Country of Publication:: United States

Language:: English

Subject:: cyano-; polycyanometallo-porphyrins; catalysts; alkane; oxidation; compositions; matter; comprising; cyano-substituted; metal; complexes; porphyrins; alkanes; iron; chromium; manganese; ruthenium; copper; cobalt; porphyrin; cyano; attached; thereto; meso; beta; -pyrrolic; positions; alkane oxidation; matter comprising; attached thereto; metal complexes; metal complex; -pyrrolic positions; comprising cyano-substituted; cyano-substituted metal; /999/

Citation Formats


                    Ellis, Jr., Paul E., and Lyons, James E. Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation.  United States: N. p., 1995. 
        Web.

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                    Ellis, Jr., Paul E., & Lyons, James E. Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation.  United States.

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                    Ellis, Jr., Paul E., and Lyons, James E. Sun .  
        "Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation".  United States.  https://www.osti.gov/servlets/purl/869710.

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@article{osti_869710,

  title        = {Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation},

  author       = {Ellis, Jr., Paul E. and Lyons, James E},

  abstractNote = {New compositions of matter comprising cyano-substituted metal complexes of porphyrins are catalysts for the oxidation of alkanes. The metal is iron, chromium, manganese, ruthenium, copper or cobalt. The porphyrin ring has cyano groups attached thereto in meso and/or .beta.-pyrrolic positions.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {1995},

  month        = {1}

}

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Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation

Patent Ellis, Jr., Paul E. (Downingtown, PA); Lyons, James E [Wallingford, PA]

New compositions of matter comprising cyano-substituted metal complexes of porphyrins are catalysts for the oxidation of alkanes. The metal is iron, chromium, manganese, ruthenium, copper or cobalt. The porphyrin ring has cyano groups attached thereto in meso and/or .beta.-pyrrolic positions.
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Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation

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Cyano- and polycyanometallo-porphyrins as catalysts for alkane oxidation

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New compositions of matter comprising cyano-substituted metal complexes of porphyrins are catalysts for the oxidation of alkanes. The metal is iron, chromium, manganese, ruthenium, copper or cobalt. The porphyrin ring has cyano groups attached thereto in meso and/or [beta]-pyrrolic positions.
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Alkanes are oxidized by contact with oxygen-containing gas in the presence as catalyst of a metalloporphyrin in which hydrogen atoms in the porphyrin ring have been substituted with one or more cyano groups. Hydrogen atoms in the porphyrin ring may also be substituted with halogen atoms.
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Transition metal complexes of meso-haloalkylporphyrins, wherein the haloalkyl groups contain 2 to 8 carbon atoms have been found to be highly effective catalysts for oxidation of alkanes and for the decomposition of hydroperoxides.
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