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Title: ANION EXCHANGE METHOD FOR SEPARATION OF METAL VALUES

Abstract

A method is described for selectively separating radium, bismuth, poloniums and lead values from a metallic mixture of thc same. The mixture is dissolved in aqueous hydrochloric acid and the acidity is adjusted to between 1 to 2M in hydrochloric acid to form the anionic polychloro complexes of polonium and bismuth. The solution is contacted with a first anion exchange resin such as strong base quaternary ammonia type to selectively absorb the polonium and bismuth leaving the radium and lead in the effluent. The effluent, after treatment in hydrochloric acid to increase the hydrochloric acid concentration to 6M is contacted with a second anion exchange iesin of the same type as the above to selectively adsorb the lead leaving the radium in the effluent. Radium is separately recovered from the effluent from the second exchange column. Lead is stripped from the loaded resin of the second column by treatment with 3M hydrochloric acid solution. The loaded resin of the first column is washed with 8M hydrochloric acid solution to recover bismuth and then treated with strong nitric acid solution to recover polonium.

Inventors:
;
Issue Date:
Research Org.:
Originating Research Org. not identified
OSTI Identifier:
4261330
Patent Number(s):
2873170
Assignee:
U.S. Atomic Energy Commission
Patent Classifications (CPCs):
B - PERFORMING OPERATIONS B01 - PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL B01J - CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY
Y - NEW / CROSS SECTIONAL TECHNOLOGIES Y10 - TECHNICAL SUBJECTS COVERED BY FORMER USPC Y10S - TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
NSA Number:
NSA-13-013323
Resource Type:
Patent
Resource Relation:
Other Information: Orig. Receipt Date: 31-DEC-59
Country of Publication:
United States
Language:
English
Subject:
CHEMISTRY; ABSORPTION; ADSORPTION; AMMONIA; ANIONS; BISMUTH; BISMUTH COMPLEXES; EXTRACTION COLUMNS; HYDROCHLORIC ACID; ION EXCHANGE MATERIALS; IONIZATION; LEAD; MIXING; NITRIC ACID; OPERATION; ORGANIC CHLORINE COMPOUNDS; POLONIUM; POLONIUM COMPLEXES; QUANTITY RATIO; RADIUM; RESINS; SEPARATION PROCESSES; SOLUTIONS; STRIPPING

Citation Formats

Hyde, E K, and Raby, B A. ANION EXCHANGE METHOD FOR SEPARATION OF METAL VALUES. United States: N. p., 1959. Web.
Hyde, E K, & Raby, B A. ANION EXCHANGE METHOD FOR SEPARATION OF METAL VALUES. United States.
Hyde, E K, and Raby, B A. Tue . "ANION EXCHANGE METHOD FOR SEPARATION OF METAL VALUES". United States.
@article{osti_4261330,
title = {ANION EXCHANGE METHOD FOR SEPARATION OF METAL VALUES},
author = {Hyde, E K and Raby, B A},
abstractNote = {A method is described for selectively separating radium, bismuth, poloniums and lead values from a metallic mixture of thc same. The mixture is dissolved in aqueous hydrochloric acid and the acidity is adjusted to between 1 to 2M in hydrochloric acid to form the anionic polychloro complexes of polonium and bismuth. The solution is contacted with a first anion exchange resin such as strong base quaternary ammonia type to selectively absorb the polonium and bismuth leaving the radium and lead in the effluent. The effluent, after treatment in hydrochloric acid to increase the hydrochloric acid concentration to 6M is contacted with a second anion exchange iesin of the same type as the above to selectively adsorb the lead leaving the radium in the effluent. Radium is separately recovered from the effluent from the second exchange column. Lead is stripped from the loaded resin of the second column by treatment with 3M hydrochloric acid solution. The loaded resin of the first column is washed with 8M hydrochloric acid solution to recover bismuth and then treated with strong nitric acid solution to recover polonium.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {1959},
month = {2}
}

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