Oxygen carrying materials with surface modification for redox-based catalysis and methods of making and uses thereof

Li, Fanxing; Neal, Luke Michael; Gao, Yunfei; Yusuf, Seif; Dudek, Ryan

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Title: Oxygen carrying materials with surface modification for redox-based catalysis and methods of making and uses thereof

Abstract

Redox catalysts having surface medication, methods of making redox catalysts with surface modification, and uses of the surface modified redox catalysts are provided. In some aspects, the redox catalysts include a core oxygen carrier region such as CaMnO₃, BaMnO_3−δ, SrMnO_3−δ, Mn₂SiO₄, Mn₂MgO_4−δ, La_0.8Sr_0.2O_3−δ, La_0.8Sr_0.2FeO_3−δ, Ca₉Ti_0.1Mn_0.9O_3−δ, Pr₆O_11−δ, manganese ore, or a combination thereof; and an outer shell having an average thickness of about 1-100 monolayers surrounding the outer surface of the core region. The outer shell can include, for example a salt selected such as Li₂WO₄, Na₂WO₄, K₂WO₄, SrWO₄, Li₂MoO₄, Na₂MoO₄, K₂MoO₄, CsMoO₄, Li₂CO₃, Na₂CO₃, K₂CO₃, or a combination thereof.

Inventors:: Li, Fanxing; Neal, Luke Michael; Gao, Yunfei; Yusuf, Seif; Dudek, Ryan

Issue Date:: Tue Nov 14 00:00:00 EST 2023

Research Org.:: North Carolina State University, Raleigh, NC (United States)

Sponsoring Org.:: USDOE Advanced Research Projects Agency - Energy (ARPA-E); National Science Foundation (NSF)

OSTI Identifier:: 2293854

Patent Number(s):: 11813592

Application Number:: 16/622,627

Assignee:: North Carolina State University (Raleigh, NC)

DOE Contract Number:: AR0000327; 1254351

Resource Type:: Patent

Resource Relation:: Patent File Date: 06/14/2018

Country of Publication:: United States

Language:: English

Citation Formats


                    Li, Fanxing, Neal, Luke Michael, Gao, Yunfei, Yusuf, Seif, and Dudek, Ryan. Oxygen carrying materials with surface modification for redox-based catalysis and methods of making and uses thereof.  United States: N. p., 2023. 
        Web.

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                    Li, Fanxing, Neal, Luke Michael, Gao, Yunfei, Yusuf, Seif, & Dudek, Ryan. Oxygen carrying materials with surface modification for redox-based catalysis and methods of making and uses thereof.  United States.

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                    Li, Fanxing, Neal, Luke Michael, Gao, Yunfei, Yusuf, Seif, and Dudek, Ryan. Tue .  
        "Oxygen carrying materials with surface modification for redox-based catalysis and methods of making and uses thereof".  United States.  https://www.osti.gov/servlets/purl/2293854.

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@article{osti_2293854,

  title        = {Oxygen carrying materials with surface modification for redox-based catalysis and methods of making and uses thereof},

  author       = {Li, Fanxing and Neal, Luke Michael and Gao, Yunfei and Yusuf, Seif and Dudek, Ryan},

  abstractNote = {Redox catalysts having surface medication, methods of making redox catalysts with surface modification, and uses of the surface modified redox catalysts are provided. In some aspects, the redox catalysts include a core oxygen carrier region such as CaMnO3, BaMnO3−δ, SrMnO3−δ, Mn2SiO4, Mn2MgO4−δ, La0.8Sr0.2O3−δ, La0.8Sr0.2FeO3−δ, Ca9Ti0.1Mn0.9O3−δ, Pr6O11−δ, manganese ore, or a combination thereof; and an outer shell having an average thickness of about 1-100 monolayers surrounding the outer surface of the core region. The outer shell can include, for example a salt selected such as Li2WO4, Na2WO4, K2WO4, SrWO4, Li2MoO4, Na2MoO4, K2MoO4, CsMoO4, Li2CO3, Na2CO3, K2CO3, or a combination thereof.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {Tue Nov 14 00:00:00 EST 2023},

  month        = {Tue Nov 14 00:00:00 EST 2023}

}

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Similar Records

Title: Oxygen carrying materials with surface modification for redox-based catalysis and methods of making and uses thereof

Abstract

Citation Formats

Effects of Sodium and Tungsten Promoters on Mg 6 MnO 8 -Based Core–Shell Redox Catalysts for Chemical Looping—Oxidative Dehydrogenation of Ethane journal, February 2019

Intensification of Ethylene Production from Naphtha via a Redox Oxy-Cracking Scheme: Process Simulations and Analysis journal, October 2018

Oxidative dehydrogenation of ethane under a cyclic redox scheme – Process simulations and analysis journal, January 2017

Molten LiCl Layer Supported on MgO: Its Possible Role in Enhancing the Oxidative Dehydrogenation of Ethane journal, April 2015

Mixed iron-manganese oxides as redox catalysts for chemical looping–oxidative dehydrogenation of ethane with tailorable heat of reactions journal, November 2019

Methane conversion patent, February 1985

Comparison of LaFeO3, La0.8Sr0.2FeO3, and La0.8Sr0.2Fe0.9Co0.1O3 perovskite oxides as oxygen carrier for partial oxidation of methane journal, December 2008

Screening of different manganese ores for chemical-looping combustion (CLC) and chemical-looping with oxygen uncoupling (CLOU) journal, December 2015

Alkali promoted manganese oxide compositions containing zirconium patent, September 1988

Methane conversion process patent, June 1985

Methane conversion patent, October 1985

Ca1−A MnO3 (A = Sr and Ba) perovskite based oxygen carriers for chemical looping with oxygen uncoupling (CLOU) journal, November 2015

Oxidative Dehydrogenation of Ethane: A Chemical Looping Approach journal, June 2016

Oxygen transfer agents for the oxidative dehydrogenation of hydrocarbons and systems and processes using the same patent, November 2018

Combined oxides as oxygen-carrier material for chemical-looping with oxygen uncoupling journal, January 2014

Effect of Promoters on Manganese-Containing Mixed Metal Oxides for Oxidative Dehydrogenation of Ethane via a Cyclic Redox Scheme journal, July 2017

Oxidative dehydrogenation of ethane using MoO3/Fe2O3 catalysts in a cyclic redox mode journal, November 2018

Intensified Ethylene Production via Chemical Looping through an Exergetically Efficient Redox Scheme journal, September 2019

Modular‐scale ethane to liquids via chemical looping oxidative dehydrogenation: Redox catalyst performance and process analysis journal, February 2019

Effect of promoter in the oxidative coupling of methane over synthesized Mn/SiO2 nanocatalysts via incipient wetness impregnation journal, November 2010

Alkali promoted manganese oxide compositions containing silica and/or alkaline earth oxides patent, December 1986

Manganese-containing redox catalysts for selective hydrogen combustion under a cyclic redox scheme journal, April 2018

Li-Promoted La x Sr 2– x FeO 4−δ Core–Shell Redox Catalysts for Oxidative Dehydrogenation of Ethane under a Cyclic Redox Scheme journal, September 2016

Chemical looping capabilities of olivine, used as a catalyst in indirect biomass gasification journal, February 2014

Manganese silicate based redox catalysts for greener ethylene production via chemical looping – oxidative dehydrogenation of ethane journal, September 2018

Shell catalyst, in particular for oxidation of methanol to formaldehyde, and also method for production thereof patent, September 2010

Alkali Metal-Promoted La x Sr 2– x FeO 4−δ Redox Catalysts for Chemical Looping Oxidative Dehydrogenation of Ethane journal, January 2018

Comparing direct and indirect fluidized bed gasification: Effect of redox cycle on olivine activity journal, June 2014

Perovskite oxides for redox oxidative cracking of n-hexane under a cyclic redox scheme journal, June 2019

Effects of Sodium and Tungsten Promoters on Mg ₆ MnO ₈ -Based Core–Shell Redox Catalysts for Chemical Looping—Oxidative Dehydrogenation of Ethane
journal, February 2019

Intensification of Ethylene Production from Naphtha via a Redox Oxy-Cracking Scheme: Process Simulations and Analysis
journal, October 2018

Oxidative dehydrogenation of ethane under a cyclic redox scheme – Process simulations and analysis
journal, January 2017

Molten LiCl Layer Supported on MgO: Its Possible Role in Enhancing the Oxidative Dehydrogenation of Ethane
journal, April 2015

Mixed iron-manganese oxides as redox catalysts for chemical looping–oxidative dehydrogenation of ethane with tailorable heat of reactions
journal, November 2019

Methane conversion
patent, February 1985

Comparison of LaFeO3, La0.8Sr0.2FeO3, and La0.8Sr0.2Fe0.9Co0.1O3 perovskite oxides as oxygen carrier for partial oxidation of methane
journal, December 2008

Screening of different manganese ores for chemical-looping combustion (CLC) and chemical-looping with oxygen uncoupling (CLOU)
journal, December 2015

Alkali promoted manganese oxide compositions containing zirconium
patent, September 1988

Methane conversion process
patent, June 1985

Methane conversion
patent, October 1985

Ca1−A MnO3 (A = Sr and Ba) perovskite based oxygen carriers for chemical looping with oxygen uncoupling (CLOU)
journal, November 2015

Oxidative Dehydrogenation of Ethane: A Chemical Looping Approach
journal, June 2016

Oxygen transfer agents for the oxidative dehydrogenation of hydrocarbons and systems and processes using the same
patent, November 2018

Combined oxides as oxygen-carrier material for chemical-looping with oxygen uncoupling
journal, January 2014

Effect of Promoters on Manganese-Containing Mixed Metal Oxides for Oxidative Dehydrogenation of Ethane via a Cyclic Redox Scheme
journal, July 2017

Oxidative dehydrogenation of ethane using MoO3/Fe2O3 catalysts in a cyclic redox mode
journal, November 2018

Intensified Ethylene Production via Chemical Looping through an Exergetically Efficient Redox Scheme
journal, September 2019

Modular‐scale ethane to liquids via chemical looping oxidative dehydrogenation: Redox catalyst performance and process analysis
journal, February 2019

Effect of promoter in the oxidative coupling of methane over synthesized Mn/SiO2 nanocatalysts via incipient wetness impregnation
journal, November 2010

Alkali promoted manganese oxide compositions containing silica and/or alkaline earth oxides
patent, December 1986

Manganese-containing redox catalysts for selective hydrogen combustion under a cyclic redox scheme
journal, April 2018

Li-Promoted La _x Sr _{2– x} FeO _4−δ Core–Shell Redox Catalysts for Oxidative Dehydrogenation of Ethane under a Cyclic Redox Scheme
journal, September 2016

Chemical looping capabilities of olivine, used as a catalyst in indirect biomass gasification
journal, February 2014

Manganese silicate based redox catalysts for greener ethylene production via chemical looping – oxidative dehydrogenation of ethane
journal, September 2018

Shell catalyst, in particular for oxidation of methanol to formaldehyde, and also method for production thereof
patent, September 2010

Alkali Metal-Promoted La _x Sr _{2– x} FeO _4−δ Redox Catalysts for Chemical Looping Oxidative Dehydrogenation of Ethane
journal, January 2018

Comparing direct and indirect fluidized bed gasification: Effect of redox cycle on olivine activity
journal, June 2014

Perovskite oxides for redox oxidative cracking of n-hexane under a cyclic redox scheme
journal, June 2019