System and method for collecting and isolating radiosotopes

Brown, Michael A.; Gelis, Artem; Rotsch, David; Nolen, Jerry A.; Youker, Amanda J.

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Title: System and method for collecting and isolating radiosotopes

Abstract

A method for obtaining ²²⁵AC from ²²⁵Ra having the steps of assembling a column having an inorganic stationary phase; priming the column to immobilize ²²⁶Ra ²²⁵Ra and natural decay products therefrom; immobilizing the ²²⁶Ra, ²²⁵Ra, ²²⁴Ra, and natural decay products therefrom onto a stationary phase within the column; and eluting the column containing the ²²⁵Ra with an aqueous sulfate solution to obtain a milking effluent that contains ²²⁵AC. Also provided is a method for obtaining pure ²²⁵AC from its isotope parents, the method comprising assembling a column having a stationary phase comprising an inorganic material; priming the column with the isotope parents to immobilize ²²⁵Ac, and natural decay products of ²²⁵AC; immobilizing the ²²⁵Ac, and natural decay products therefrom onto the stationary phase within the column ²²⁶Ra, ²²⁵Ra, ²²⁴Ra; and eluting the column containing the ²²⁵AC to obtain an effluent that contains the isotope parents.

Inventors:: Brown, Michael A.; Gelis, Artem; Rotsch, David; Nolen, Jr., Jerry A.; Youker, Amanda J.

Issue Date:: 2023-10-24

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 2293770

Patent Number(s):: 11798702

Application Number:: 16/554,048

Assignee:: UChicago Argonne, LLC (Chicago, IL)

DOE Contract Number:: AC02-06CH11357

Resource Type:: Patent

Resource Relation:: Patent File Date: 08/28/2019

Country of Publication:: United States

Language:: English

Citation Formats


                    Brown, Michael A., Gelis, Artem, Rotsch, David, Nolen, Jr., Jerry A., and Youker, Amanda J. System and method for collecting and isolating radiosotopes.  United States: N. p., 2023. 
        Web.

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                    Brown, Michael A., Gelis, Artem, Rotsch, David, Nolen, Jr., Jerry A., & Youker, Amanda J. System and method for collecting and isolating radiosotopes.  United States.

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                    Brown, Michael A., Gelis, Artem, Rotsch, David, Nolen, Jr., Jerry A., and Youker, Amanda J. Tue .  
        "System and method for collecting and isolating radiosotopes".  United States.  https://www.osti.gov/servlets/purl/2293770.

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@article{osti_2293770,

  title        = {System and method for collecting and isolating radiosotopes},

  author       = {Brown, Michael A. and Gelis, Artem and Rotsch, David and Nolen, Jr., Jerry A. and Youker, Amanda J.},

  abstractNote = {A method for obtaining 225AC from 225Ra having the steps of assembling a column having an inorganic stationary phase; priming the column to immobilize 226Ra 225Ra and natural decay products therefrom; immobilizing the 226Ra, 225Ra, 224Ra, and natural decay products therefrom onto a stationary phase within the column; and eluting the column containing the 225Ra with an aqueous sulfate solution to obtain a milking effluent that contains 225AC. Also provided is a method for obtaining pure 225AC from its isotope parents, the method comprising assembling a column having a stationary phase comprising an inorganic material; priming the column with the isotope parents to immobilize 225Ac, and natural decay products of 225AC; immobilizing the 225Ac, and natural decay products therefrom onto the stationary phase within the column 226Ra, 225Ra, 224Ra; and eluting the column containing the 225AC to obtain an effluent that contains the isotope parents.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2023},

  month        = {10}

}

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Works referenced in this record:

Anion-exchange Studies. XI. Lead(II) and Bismuth(III) in Chloride and Nitrate Solutions ^1,2
journal, December 1954

Nelson, Frederick; Kraus, Kurt A.
Journal of the American Chemical Society, Vol. 76, Issue 23
https://doi.org/10.1021/ja01652a006

Preparation of 225Ac and 228Ac generators using a cryptomelane manganese dioxide sorbent
journal, January 2003

Wlodzimirska, B.; Bartoś, B.; Bilewicz, A.
Radiochimica Acta, Vol. 91, Issue 9
https://doi.org/10.1524/ract.91.9.553.19996

The feasibility of 225 Ac as a source of ??-particles in radioimmunotherapy
journal, January 1993

Geerlings, M. W.; Kaspersen, F. M.; Apostolidis, C.
Nuclear Medicine Communications, Vol. 14, Issue 2
https://doi.org/10.1097/00006231-199302000-00009

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Similar Records

Title: System and method for collecting and isolating radiosotopes

Abstract

Citation Formats

Anion-exchange Studies. XI. Lead(II) and Bismuth(III) in Chloride and Nitrate Solutions 1,2 journal, December 1954

Preparation of 225Ac and 228Ac generators using a cryptomelane manganese dioxide sorbent journal, January 2003

The feasibility of 225 Ac as a source of ??-particles in radioimmunotherapy journal, January 1993

Anion-exchange Studies. XI. Lead(II) and Bismuth(III) in Chloride and Nitrate Solutions ^1,2
journal, December 1954

Preparation of 225Ac and 228Ac generators using a cryptomelane manganese dioxide sorbent
journal, January 2003

The feasibility of 225 Ac as a source of ??-particles in radioimmunotherapy
journal, January 1993