Compositions and methods for carbon dioxide capture

Lu, Yongqi; Du, Yang; Ye, Qing

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Title: Compositions and methods for carbon dioxide capture

Abstract

An aqueous solvent composition is provided, comprising a nucleophilic component having one or more sterically unhindered primary or secondary amine moieties, a Brønsted base component having one or more basic nitrogen moieties, a water-soluble organic solvent, and water. A biphasic composition is provided, comprising one or more carbamate compounds, one or more conjugate acids of Brønsted base, a water-soluble organic solvent, and water. A biphasic CO2 absorption process is also provided, utilizing the biphasic solvent composition.

Inventors:: Lu, Yongqi; Du, Yang; Ye, Qing

Issue Date:: 2022-08-02

Research Org.:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1924933

Patent Number(s):: 11400410

Application Number:: 16/374,471

Assignee:: The Board of Trustees of the University of Illinois (Urbana, IL)

Patent Classifications (CPCs):: B - PERFORMING OPERATIONS B01 - PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL B01D - SEPARATION

C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07C - ACYCLIC OR CARBOCYCLIC COMPOUNDS

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B - PERFORMING OPERATIONS B01 - PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL B01D - SEPARATION
B01D2252/20405 - Monoamines
B01D2252/2041 - Diamines
B01D2252/20415 - Tri- or polyamines
B01D2252/20421 - Primary amines
B01D2252/20426 - Secondary amines
B01D2252/20431 - Tertiary amines
B01D2252/20442 - containing a piperidine-ring
B01D2252/20447 - containing a piperazine-ring
B01D2252/20473 - containing an imidazole-ring
B01D2252/20484 - with one hydroxyl group
B01D2252/504 - Mixtures of two or more absorbents
B01D2257/504 - Carbon dioxide
B01D2258/0283 - Flue gases
B01D53/1425 - {Regeneration of liquid absorbents}
B01D53/1475 - {Removing carbon dioxide}
B01D53/1493 - {Selection of liquid materials for use as absorbents}
B01D53/62 - Carbon oxides
B01D53/78 - with gas-liquid contact
B01D53/96 - Regeneration, reactivation or recycling of reactants

C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07C - ACYCLIC OR CARBOCYCLIC COMPOUNDS
C07C211/03 - Monoamines
C07C211/06 - containing only n- or iso-propyl groups
C07C211/11 - Diaminopropanes
C07C211/13 - Amines containing three or more amino groups bound to the carbon skeleton
C07C211/17 - containing only non-condensed rings

C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07D - HETEROCYCLIC COMPOUNDS
C07D213/16 - containing only one pyridine ring
C07D221/00 - Heterocyclic compounds containing six-membered rings having one nitrogen atom as the only ring hetero atom, not provided for by groups C07D211/00 - C07D219/00
C07D223/04 - with only hydrogen atoms, halogen atoms, hydrocarbon or substituted hydrocarbon radicals, directly attached to ring carbon atoms
C07D235/00 - Heterocyclic compounds containing 1,3-diazole or hydrogenated 1,3-diazole rings, condensed with other rings
C07D241/04 - having no double bonds between ring members or between ring members and non-ring members
C07D265/30 - not condensed with other rings

Y - NEW / CROSS SECTIONAL TECHNOLOGIES Y02 - TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE Y02P - CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
Y02P20/151 - Reduction of greenhouse gas [GHG] emissions

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DOE Contract Number:: FE0004360; FE0026434

Resource Type:: Patent

Resource Relation:: Patent File Date: 04/03/2019

Country of Publication:: United States

Language:: English

Citation Formats


                    Lu, Yongqi, Du, Yang, and Ye, Qing. Compositions and methods for carbon dioxide capture.  United States: N. p., 2022. 
        Web.

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                    Lu, Yongqi, Du, Yang, & Ye, Qing. Compositions and methods for carbon dioxide capture.  United States.

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                    Lu, Yongqi, Du, Yang, and Ye, Qing. Tue .  
        "Compositions and methods for carbon dioxide capture".  United States.  https://www.osti.gov/servlets/purl/1924933.

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@article{osti_1924933,

  title        = {Compositions and methods for carbon dioxide capture},

  author       = {Lu, Yongqi and Du, Yang and Ye, Qing},

  abstractNote = {An aqueous solvent composition is provided, comprising a nucleophilic component having one or more sterically unhindered primary or secondary amine moieties, a Brønsted base component having one or more basic nitrogen moieties, a water-soluble organic solvent, and water. A biphasic composition is provided, comprising one or more carbamate compounds, one or more conjugate acids of Brønsted base, a water-soluble organic solvent, and water. A biphasic CO2 absorption process is also provided, utilizing the biphasic solvent composition.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2022},

  month        = {8}

}

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Works referenced in this record:

CO2 absorption by biphasic solvents: Mixtures of 1,4-Butanediamine and 2-(Diethylamino)-ethanol
journal, August 2013

Xu, Zhicheng; Wang, Shujuan; Chen, Changhe
International Journal of Greenhouse Gas Control, Vol. 16
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Self-concentrating absorbent for acid gas separation
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Hu, Liang
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Development of an Energy-efficient CO2 Capture Process Using Thermomorphic Biphasic Solvents
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Zhang, Jiafei; Qiao, Yu; Wang, Wanzhong
Energy Procedia, Vol. 37
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Novel Thermomorphic Biphasic Amine Solvents for CO2 Absorption and Low-Temperature Extractive Regeneration
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Zhang, J.; Misch, R.; Tan, Y.
Chemical Engineering & Technology, Vol. 34, Issue 9
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Phase transitional absorption method
patent, June 2009

Hu, Liang
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Carbon dioxide absorption using a phase transitional alkanolamine–alcohol mixture
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Kim, Young Eun; Park, Jung Hwan; Yun, Soung Hee
Journal of Industrial and Engineering Chemistry, Vol. 20, Issue 4
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Experimental Investigation and Thermodynamic Modeling of Phase Transition and Equilibria in a Biphasic Solvent System for CO₂ Capture
journal, June 2018

Ye, Qing; Wang, Xinlei; Lu, Yongqi
Industrial & Engineering Chemistry Research, Vol. 57, Issue 29
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Kinetics of CO2 absorption in aqueous blends of N,N-diethylethanolamine (DEEA) and N-methyl-1,3-propane-diamine (MAPA)
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Monteiro, Juliana G. M. -S.; Majeed, Hammad; Knuutila, Hanna
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Study on potential biphasic solvents: Absorption capacity, CO2 loading and reaction rate
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Zhicheng, Xu; Shujuan, Wang; Bo, Zhao
Energy Procedia, Vol. 37
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Phase separation characteristics in biphasic solvents based on mutually miscible amines for energy efficient CO2 capture
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Lee, Jun; Hong, Yeon Ki; You, Jong Kyun
Korean Journal of Chemical Engineering, Vol. 34, Issue 6
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Thermal degradation of amines for CO2 capture
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Rochelle, Gary T.
Current Opinion in Chemical Engineering, Vol. 1, Issue 2
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Mixed amine and non-nucleophilic base CO2 scrubbing process for improved adsorption at increased temperatures
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Kortunov, Pavel; Baugh, Lisa Saunders; Calabro, David C.
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Co2 mass transfer enhancement of aqueous amine solvents by particle additives
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Widger, Leland R.; Qi, Guojie; Liu, Kun
US Patent Application 15/423042; 20170216763
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Journal of Medicinal Chemistry, Vol. 58, Issue 7
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Non-Aqueous Amine Scrubbing for Removal of Carbon Dioxide
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Capturing CO₂ into the Precipitate of a Phase-Changing Solvent after Absorption
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Environmental Science & Technology, Vol. 48, Issue 15
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Similar Records

Title: Compositions and methods for carbon dioxide capture

Abstract

Citation Formats

CO2 absorption by biphasic solvents: Mixtures of 1,4-Butanediamine and 2-(Diethylamino)-ethanol journal, August 2013

Self-concentrating absorbent for acid gas separation patent, December 2010

Development of an Energy-efficient CO2 Capture Process Using Thermomorphic Biphasic Solvents journal, January 2013

Novel Thermomorphic Biphasic Amine Solvents for CO2 Absorption and Low-Temperature Extractive Regeneration journal, August 2011

Phase transitional absorption method patent, June 2009

Carbon dioxide absorption using a phase transitional alkanolamine–alcohol mixture journal, July 2014

Experimental Investigation and Thermodynamic Modeling of Phase Transition and Equilibria in a Biphasic Solvent System for CO2 Capture journal, June 2018

Kinetics of CO2 absorption in aqueous blends of N,N-diethylethanolamine (DEEA) and N-methyl-1,3-propane-diamine (MAPA) journal, June 2015

Study on potential biphasic solvents: Absorption capacity, CO2 loading and reaction rate journal, January 2013

Phase separation characteristics in biphasic solvents based on mutually miscible amines for energy efficient CO2 capture journal, April 2017

Thermal degradation of amines for CO2 capture journal, May 2012

Mixed amine and non-nucleophilic base CO2 scrubbing process for improved adsorption at increased temperatures patent, May 2014

Co2 mass transfer enhancement of aqueous amine solvents by particle additives patent-application, August 2017

Organic Carbamates in Drug Design and Medicinal Chemistry journal, January 2015

Non-Aqueous Amine Scrubbing for Removal of Carbon Dioxide patent-application, March 2012

Capturing CO2 into the Precipitate of a Phase-Changing Solvent after Absorption journal, July 2014

Absorbing Solution, Method and Device for Absorbing CO2 or H2S or Both patent-application, April 2008

Promotion of CO2 mass transfer in carbonate solutions journal, January 1981

CO2 absorption by biphasic solvents: Mixtures of 1,4-Butanediamine and 2-(Diethylamino)-ethanol
journal, August 2013

Self-concentrating absorbent for acid gas separation
patent, December 2010

Development of an Energy-efficient CO2 Capture Process Using Thermomorphic Biphasic Solvents
journal, January 2013

Novel Thermomorphic Biphasic Amine Solvents for CO2 Absorption and Low-Temperature Extractive Regeneration
journal, August 2011

Phase transitional absorption method
patent, June 2009

Carbon dioxide absorption using a phase transitional alkanolamine–alcohol mixture
journal, July 2014

Experimental Investigation and Thermodynamic Modeling of Phase Transition and Equilibria in a Biphasic Solvent System for CO₂ Capture
journal, June 2018

Kinetics of CO2 absorption in aqueous blends of N,N-diethylethanolamine (DEEA) and N-methyl-1,3-propane-diamine (MAPA)
journal, June 2015

Study on potential biphasic solvents: Absorption capacity, CO2 loading and reaction rate
journal, January 2013

Phase separation characteristics in biphasic solvents based on mutually miscible amines for energy efficient CO2 capture
journal, April 2017

Thermal degradation of amines for CO2 capture
journal, May 2012

Mixed amine and non-nucleophilic base CO2 scrubbing process for improved adsorption at increased temperatures
patent, May 2014

Co2 mass transfer enhancement of aqueous amine solvents by particle additives
patent-application, August 2017

Organic Carbamates in Drug Design and Medicinal Chemistry
journal, January 2015

Non-Aqueous Amine Scrubbing for Removal of Carbon Dioxide
patent-application, March 2012

Capturing CO₂ into the Precipitate of a Phase-Changing Solvent after Absorption
journal, July 2014

Absorbing Solution, Method and Device for Absorbing CO2 or H2S or Both
patent-application, April 2008

Promotion of CO2 mass transfer in carbonate solutions
journal, January 1981