Flow-through reactor for electrocatalytic reactions

Biener, Monika M.; Biener, Juergen; Liang, Siwei; Qi, Zhen; Stadermann, Michael; Vedharathinam, Vedasri

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Title: Flow-through reactor for electrocatalytic reactions

Abstract

A flow-through electrolysis cell includes a hierarchical nanoporous metal cathode. A method of reducing CO2 includes flowing the CO2 through the hierarchical nanoporous metal cathode of the flow-through electrolysis cell.

Inventors:: Biener, Monika M.; Biener, Juergen; Liang, Siwei; Qi, Zhen; Stadermann, Michael; Vedharathinam, Vedasri

Issue Date:: 2021-07-06

Research Org.:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1840229

Patent Number(s):: 11053597

Application Number:: 15/946,424

Assignee:: Lawrence Livermore National Security, LLC (Livermore, CA)

Patent Classifications (CPCs):: C - CHEMISTRY C25 - ELECTROLYTIC OR ELECTROPHORETIC PROCESSES C25B - ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS

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C - CHEMISTRY C25 - ELECTROLYTIC OR ELECTROPHORETIC PROCESSES C25B - ELECTROLYTIC OR ELECTROPHORETIC PROCESSES FOR THE PRODUCTION OF COMPOUNDS OR NON-METALS
C25B15/08 - Supplying or removing reactants or electrolytes

Show less

DOE Contract Number:: AC52-07NA27344

Resource Type:: Patent

Resource Relation:: Patent File Date: 04/05/2018

Country of Publication:: United States

Language:: English

Citation Formats


                    Biener, Monika M., Biener, Juergen, Liang, Siwei, Qi, Zhen, Stadermann, Michael, and Vedharathinam, Vedasri. Flow-through reactor for electrocatalytic reactions.  United States: N. p., 2021. 
        Web.

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                    Biener, Monika M., Biener, Juergen, Liang, Siwei, Qi, Zhen, Stadermann, Michael, & Vedharathinam, Vedasri. Flow-through reactor for electrocatalytic reactions.  United States.

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                    Biener, Monika M., Biener, Juergen, Liang, Siwei, Qi, Zhen, Stadermann, Michael, and Vedharathinam, Vedasri. Tue .  
        "Flow-through reactor for electrocatalytic reactions".  United States.  https://www.osti.gov/servlets/purl/1840229.

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@article{osti_1840229,

  title        = {Flow-through reactor for electrocatalytic reactions},

  author       = {Biener, Monika M. and Biener, Juergen and Liang, Siwei and Qi, Zhen and Stadermann, Michael and Vedharathinam, Vedasri},

  abstractNote = {A flow-through electrolysis cell includes a hierarchical nanoporous metal cathode. A method of reducing CO2 includes flowing the CO2 through the hierarchical nanoporous metal cathode of the flow-through electrolysis cell.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2021},

  month        = {7}

}

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Patent:

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Similar Records

Title: Flow-through reactor for electrocatalytic reactions

Abstract

Citation Formats

Electrochemical conversion of CO2 to useful chemicals: current status, remaining challenges, and future opportunities journal, May 2013

The importance of surface morphology in controlling the selectivity of polycrystalline copper for CO2 electroreduction journal, January 2012

Nanostructured nonprecious metal catalysts for electrochemical reduction of carbon dioxide journal, June 2016

Effect of solid polymer electrolyte on electrochemical reduction of CO2 journal, June 2012

High Selectivity for Ethylene from Carbon Dioxide Reduction over Copper Nanocube Electrocatalysts journal, February 2015

Apparatus for Preparing Hydrogen Water patent-application, March 2016

Advanced carbon aerogels for energy applications journal, January 2011

Nanoporous Gold: Understanding the Origin of the Reactivity of a 21st Century Catalyst Made by Pre-Columbian Technology journal, September 2015

Method and Apparatus for the Electrochemical Reduction of Carbon Dioxide patent-application, July 2013

Nanoporous Plasmonic Metamaterials journal, March 2008

Monolithic nanoporous copper by dealloying Mn–Cu journal, October 2006

Flow-through electrode capacitive deionization cell patent-application, May 2019

Electrolytic production of high purity alkali metal hydroxide patent, October 1981

Three-dimensional porous hollow fibre copper electrodes for efficient and high-rate electrochemical carbon dioxide reduction journal, February 2016

Nanoporous Metals Fabricated through Electrochemical Dealloying of Ag-Au-Pt with Systematic Variation of Au:Pt Ratio journal, October 2013

Method and system for electrochemical reduction of carbon dioxide employing a gas diffusion electrode patent, June 2019

Dimensionally Stable Anode Construction patent, December 1974

Size Effects on the Mechanical Behavior of Nanoporous Au journal, October 2006

System and High Surface Area Electrodes for the Electrochemical Reduction of Carbon Dioxide patent-application, May 2013

Continuous Co-Current Electrochemical Reduction of Carbon Dioxide patent-application, September 2008

Surface-chemistry-driven actuation in nanoporous gold journal, November 2008

Neutralization in Electro Chemical Activation Systems patent-application, December 2019

Fabrication and compression properties of bulk hierarchical nanoporous copper with fine ligament journal, July 2014

Experimental Parameters Influencing Hydrocarbon Selectivity during the Electrochemical Conversion of CO 2 journal, November 2017

Maximizing Activity and Stability by Turning Gold Catalysis Upside Down: Oxide Particles on Nanoporous Gold journal, March 2013

Gold-containing catalyst with porous structure patent-application, September 2007

A three-dimensional tin-coated nanoporous copper for lithium-ion battery anodes journal, August 2011

Capacitive desalination with flow-through electrodes journal, January 2012

Nanoporous Gold Catalysts for Selective Gas-Phase Oxidative Coupling of Methanol at Low Temperature journal, January 2010

Swimming pool chlorinator system patent, December 1978

Electrochemical membrane reactors for the utilisation of carbon dioxide journal, December 2016

Axial flow electrolytic cell patent, August 1976

Ultra-strong and Low-Density Nanotubular Bulk Materials with Tunable Feature Sizes journal, May 2014

Quantitative Phase Composition of TiO 2 -Coated Nanoporous Au Monoliths by X-ray Absorption Spectroscopy and Correlations to Catalytic Behavior journal, February 2014

ALD Functionalized Nanoporous Gold: Thermal Stability, Mechanical Properties, and Catalytic Activity journal, August 2011

Defining the Nanostructured Morphology of Triblock Copolymers Using Resonant Soft X-ray Scattering journal, September 2011

Battery/supercapacitor hybrid via non-covalent functionalization of graphene macro-assemblies journal, January 2014

Materials and Methods for Electrochemical Reduction of Carbon Dioxide patent-application, March 2018

Hierarchical nested-network porous copper fabricated by one-step dealloying for glucose sensing journal, October 2016

Electrochemical conversion of CO2 to useful chemicals: current status, remaining challenges, and future opportunities
journal, May 2013

The importance of surface morphology in controlling the selectivity of polycrystalline copper for CO2 electroreduction
journal, January 2012

Nanostructured nonprecious metal catalysts for electrochemical reduction of carbon dioxide
journal, June 2016

Effect of solid polymer electrolyte on electrochemical reduction of CO₂
journal, June 2012

High Selectivity for Ethylene from Carbon Dioxide Reduction over Copper Nanocube Electrocatalysts
journal, February 2015

Apparatus for Preparing Hydrogen Water
patent-application, March 2016

Advanced carbon aerogels for energy applications
journal, January 2011

Nanoporous Gold: Understanding the Origin of the Reactivity of a 21st Century Catalyst Made by Pre-Columbian Technology
journal, September 2015

Method and Apparatus for the Electrochemical Reduction of Carbon Dioxide
patent-application, July 2013

Nanoporous Plasmonic Metamaterials
journal, March 2008

Monolithic nanoporous copper by dealloying Mn–Cu
journal, October 2006

Flow-through electrode capacitive deionization cell
patent-application, May 2019

Electrolytic production of high purity alkali metal hydroxide
patent, October 1981

Three-dimensional porous hollow fibre copper electrodes for efficient and high-rate electrochemical carbon dioxide reduction
journal, February 2016

Nanoporous Metals Fabricated through Electrochemical Dealloying of Ag-Au-Pt with Systematic Variation of Au:Pt Ratio
journal, October 2013

Method and system for electrochemical reduction of carbon dioxide employing a gas diffusion electrode
patent, June 2019

Dimensionally Stable Anode Construction
patent, December 1974

Size Effects on the Mechanical Behavior of Nanoporous Au
journal, October 2006

System and High Surface Area Electrodes for the Electrochemical Reduction of Carbon Dioxide
patent-application, May 2013

Continuous Co-Current Electrochemical Reduction of Carbon Dioxide
patent-application, September 2008

Surface-chemistry-driven actuation in nanoporous gold
journal, November 2008

Neutralization in Electro Chemical Activation Systems
patent-application, December 2019

Fabrication and compression properties of bulk hierarchical nanoporous copper with fine ligament
journal, July 2014

Experimental Parameters Influencing Hydrocarbon Selectivity during the Electrochemical Conversion of CO ₂
journal, November 2017

Maximizing Activity and Stability by Turning Gold Catalysis Upside Down: Oxide Particles on Nanoporous Gold
journal, March 2013

Gold-containing catalyst with porous structure
patent-application, September 2007

A three-dimensional tin-coated nanoporous copper for lithium-ion battery anodes
journal, August 2011

Capacitive desalination with flow-through electrodes
journal, January 2012

Nanoporous Gold Catalysts for Selective Gas-Phase Oxidative Coupling of Methanol at Low Temperature
journal, January 2010

Swimming pool chlorinator system
patent, December 1978

Electrochemical membrane reactors for the utilisation of carbon dioxide
journal, December 2016

Axial flow electrolytic cell
patent, August 1976

Ultra-strong and Low-Density Nanotubular Bulk Materials with Tunable Feature Sizes
journal, May 2014

Quantitative Phase Composition of TiO ₂ -Coated Nanoporous Au Monoliths by X-ray Absorption Spectroscopy and Correlations to Catalytic Behavior
journal, February 2014

ALD Functionalized Nanoporous Gold: Thermal Stability, Mechanical Properties, and Catalytic Activity
journal, August 2011

Defining the Nanostructured Morphology of Triblock Copolymers Using Resonant Soft X-ray Scattering
journal, September 2011

Battery/supercapacitor hybrid via non-covalent functionalization of graphene macro-assemblies
journal, January 2014

Materials and Methods for Electrochemical Reduction of Carbon Dioxide
patent-application, March 2018

Hierarchical nested-network porous copper fabricated by one-step dealloying for glucose sensing
journal, October 2016