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Title: High optical transparency polymer aerogels using low refractive index monomers

Abstract

A polymer aerogel has polymerizable monomers and crosslinkers, wherein at least one of the monomers or at least one of the crosslinkers has a refractive index of less than 1.5, and the polymer aerogel has a visible transmittance of at least 20%/3 mm, a haze of 50%/3 mm or lower, and a porosity of at least 10%. A method of producing an aerogel includes dissolving precursors into a solvent, wherein the precursors include monomers, crosslinkers, a controlling agent and an initiator to form a precursor solution, wherein at least one of the monomers or at least one of the crosslinkers has a refractive index of 1.5 or lower, polymerizing the precursor solution to form a gel polymer, and removing the solvent from the gel polymer to produce an aerogel polymer.

Inventors:
; ; ; ; ; ;
Issue Date:
Research Org.:
Palo Alto Research Center Incorporated, Palo Alto, CA (United States)
Sponsoring Org.:
USDOE Advanced Research Projects Agency - Energy (ARPA-E)
OSTI Identifier:
1823921
Patent Number(s):
10995191
Application Number:
16/228,472
Assignee:
Palo Alto Research Center Incorporated (Palo Alto, CA)
DOE Contract Number:  
AR0000274
Resource Type:
Patent
Resource Relation:
Patent File Date: 12/20/2018
Country of Publication:
United States
Language:
English

Citation Formats

Bulger, Eli, Chintapalli, Mahati, Iftime, Gabriel, Van Overmeere, Quentin, Rivest, Jessica Louis Baker, Neelakantan, Ravi, and Meckler, Stephen. High optical transparency polymer aerogels using low refractive index monomers. United States: N. p., 2021. Web.
Bulger, Eli, Chintapalli, Mahati, Iftime, Gabriel, Van Overmeere, Quentin, Rivest, Jessica Louis Baker, Neelakantan, Ravi, & Meckler, Stephen. High optical transparency polymer aerogels using low refractive index monomers. United States.
Bulger, Eli, Chintapalli, Mahati, Iftime, Gabriel, Van Overmeere, Quentin, Rivest, Jessica Louis Baker, Neelakantan, Ravi, and Meckler, Stephen. Tue . "High optical transparency polymer aerogels using low refractive index monomers". United States. https://www.osti.gov/servlets/purl/1823921.
@article{osti_1823921,
title = {High optical transparency polymer aerogels using low refractive index monomers},
author = {Bulger, Eli and Chintapalli, Mahati and Iftime, Gabriel and Van Overmeere, Quentin and Rivest, Jessica Louis Baker and Neelakantan, Ravi and Meckler, Stephen},
abstractNote = {A polymer aerogel has polymerizable monomers and crosslinkers, wherein at least one of the monomers or at least one of the crosslinkers has a refractive index of less than 1.5, and the polymer aerogel has a visible transmittance of at least 20%/3 mm, a haze of 50%/3 mm or lower, and a porosity of at least 10%. A method of producing an aerogel includes dissolving precursors into a solvent, wherein the precursors include monomers, crosslinkers, a controlling agent and an initiator to form a precursor solution, wherein at least one of the monomers or at least one of the crosslinkers has a refractive index of 1.5 or lower, polymerizing the precursor solution to form a gel polymer, and removing the solvent from the gel polymer to produce an aerogel polymer.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {2021},
month = {5}
}