Method for fabrication of superlattices and aperiodic layered structures using solution deposition
Abstract
A method for forming inorganic structures includes (a) transferring nanocrystals to a polar protic solvent using at least one chalcogenide precursor to produce a negatively-charged chalcogen-rich nanocrystal surface, (b) removing excess anions of the chalcogenide precursor, (c) introducing a metal salt to bind a divalent metal cation to the negatively-charged chalcogen-rich nanocrystal surface to regenerate a positively-charged metal-rich nanocrystal surface, and (d) removing excess divalent metal cations of the metal acetate salt.
- Inventors:
- Issue Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1495349
- Patent Number(s):
- 10138134
- Application Number:
- 15/644,602
- Assignee:
- UChicago Argonne, LLC (Chicago, IL)
- Patent Classifications (CPCs):
-
C - CHEMISTRY C01 - INORGANIC CHEMISTRY C01B - NON-METALLIC ELEMENTS
C - CHEMISTRY C01 - INORGANIC CHEMISTRY C01G - COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
- DOE Contract Number:
- AC02-06CH11357
- Resource Type:
- Patent
- Resource Relation:
- Patent File Date: 2017 Jul 07
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Diroll, Benjamin, and Schaller, Richard D. Method for fabrication of superlattices and aperiodic layered structures using solution deposition. United States: N. p., 2018.
Web.
Diroll, Benjamin, & Schaller, Richard D. Method for fabrication of superlattices and aperiodic layered structures using solution deposition. United States.
Diroll, Benjamin, and Schaller, Richard D. Tue .
"Method for fabrication of superlattices and aperiodic layered structures using solution deposition". United States. https://www.osti.gov/servlets/purl/1495349.
@article{osti_1495349,
title = {Method for fabrication of superlattices and aperiodic layered structures using solution deposition},
author = {Diroll, Benjamin and Schaller, Richard D.},
abstractNote = {A method for forming inorganic structures includes (a) transferring nanocrystals to a polar protic solvent using at least one chalcogenide precursor to produce a negatively-charged chalcogen-rich nanocrystal surface, (b) removing excess anions of the chalcogenide precursor, (c) introducing a metal salt to bind a divalent metal cation to the negatively-charged chalcogen-rich nanocrystal surface to regenerate a positively-charged metal-rich nanocrystal surface, and (d) removing excess divalent metal cations of the metal acetate salt.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {2018},
month = {11}
}
Works referenced in this record:
Cation Exchange Reactions in Ionic Nanocrystals
journal, November 2004
- Son, Dong Hee; Hughes, Steven M.; Yin, Yadong
- Science, Vol. 306, Issue 5698, p. 1009-1012
Spontaneous Superlattice Formation in Nanorods Through Partial Cation Exchange
journal, July 2007
- Robinson, R. D.; Sadtler, B.; Demchenko, D. O.
- Science, Vol. 317, Issue 5836, p. 355-358
Multidimensional quantum well laser and temperature dependence of its threshold current
journal, June 1982
- Arakawa, Y.; Sakaki, H.
- Applied Physics Letters, Vol. 40, Issue 11
Quantum Well Optical Devices and Materials
journal, August 1993
- Bhattacharya, P. K.; Dutta, N. K.
- Annual Review of Materials Science, Vol. 23, Issue 1
Structure and growth of crystalline superlattices: From monolayer to superlattice
journal, March 1986
- Bauer, E.; van der Merwe, Jan H.
- Physical Review B, Vol. 33, Issue 6
Synthesis of Highly Luminescent and Photo-Stable, Graded Shell CdSe/Cd x Zn 1– x S Nanoparticles by In Situ Alloying
journal, November 2013
- Boldt, Klaus; Kirkwood, Nicholas; Beane, Gary A.
- Chemistry of Materials, Vol. 25, Issue 23
CdSe Clusters: At the Interface of Small Molecules and Quantum Dots
journal, June 2011
- Cossairt, Brandi M.; Owen, Jonathan S.
- Chemistry of Materials, Vol. 23, Issue 12
Ultrafast Photoluminescence from the Core and the Shell in CdSe/CdS Dot-in-Rod Heterostructures
journal, November 2015
- Diroll, Benjamin T.; Turk, Michael E.; Gogotsi, Natalie
- ChemPhysChem, Vol. 17, Issue 5
Colloidal CdSe Quantum Rings
journal, July 2016
- Fedin, Igor; Talapin, Dmitri V.
- Journal of the American Chemical Society, Vol. 138, Issue 31
Colossal Ionic Conductivity at Interfaces of Epitaxial ZrO2:Y2O3/SrTiO3 Heterostructures
journal, August 2008
- Garcia-Barriocanal, J.; Rivera-Calzada, A.; Varela, M.
- Science, Vol. 321, Issue 5889
Quasi 2D Colloidal CdSe Platelets with Thicknesses Controlled at the Atomic Level
journal, December 2008
- Ithurria, Sandrine; Dubertret, Benoit
- Journal of the American Chemical Society, Vol. 130, Issue 49
Colloidal Atomic Layer Deposition (c-ALD) using Self-Limiting Reactions at Nanocrystal Surface Coupled to Phase Transfer between Polar and Nonpolar Media
journal, November 2012
- Ithurria, Sandrine; Talapin, Dmitri V.
- Journal of the American Chemical Society, Vol. 134, Issue 45
Colloidal nanoplatelets with two-dimensional electronic structure
journal, October 2011
- Ithurria, S.; Tessier, M. D.; Mahler, B.
- Nature Materials, Vol. 10, Issue 12
Attempt to Design a Strong Solid
journal, July 1970
- Koehler, J. S.
- Physical Review B, Vol. 2, Issue 2
Retardation of Dislocation Generation and Motion in Thin-Layered Metal Laminates
journal, December 1978
- Lehoczky, S. L.
- Physical Review Letters, Vol. 41, Issue 26
Large-Scale Synthesis of Nearly Monodisperse CdSe/CdS Core/Shell Nanocrystals Using Air-Stable Reagents via Successive Ion Layer Adsorption and Reaction
journal, October 2003
- Li, J. Jack; Wang, Y. Andrew; Guo, Wenzhuo
- Journal of the American Chemical Society, Vol. 125, Issue 41, p. 12567-12575
Organization of Artificial Superlattices Utilizing Nanosheets as a Building Block and Exploration of Their Advanced Functions
journal, July 2015
- Ma, Renzhi; Sasaki, Takayoshi
- Annual Review of Materials Research, Vol. 45, Issue 1
Self-Organization of CdSe Nanocrystallites into Three-Dimensional Quantum Dot Superlattices
journal, November 1995
- Murray, C. B.; Kagan, C. R.; Bawendi, M. G.
- Science, Vol. 270, Issue 5240
Metal-free Inorganic Ligands for Colloidal Nanocrystals: S2–, HS–, Se2–, HSe–, Te2–, HTe–, TeS32–, OH–, and NH2– as Surface Ligands
journal, July 2011
- Nag, Angshuman; Kovalenko, Maksym V.; Lee, Jong-Soo
- Journal of the American Chemical Society, Vol. 133, Issue 27, p. 10612-10620
High-Brightness InGaN Blue, Green and Yellow Light-Emitting Diodes with Quantum Well Structures
journal, July 1995
- Nakamura, Shuji; Senoh, Masayuki; Iwasa, Naruhito
- Japanese Journal of Applied Physics, Vol. 34, Issue Part 2, No. 7A
Optimized Synthesis of CdTe Nanoplatelets and Photoresponse of CdTe Nanoplatelets Films
journal, June 2013
- Pedetti, Silvia; Nadal, Brice; Lhuillier, Emmanuel
- Chemistry of Materials, Vol. 25, Issue 12
Colloidal Synthesis of Monodisperse Semiconductor Nanocrystals through Saturated Ionic Layer Adsorption
journal, April 2016
- Razgoniaeva, Natalia; Carrillo, Luis; Burchfield, Douglas
- Chemistry of Materials, Vol. 28, Issue 8
PbS/CdS Core/Shell Quantum Dots by Additive, Layer-by-Layer Shell Growth
journal, September 2016
- Sagar, Laxmi Kishore; Walravens, Willem; Zhao, Qiang
- Chemistry of Materials, Vol. 28, Issue 19
Low-Threshold Stimulated Emission Using Colloidal Quantum Wells
journal, April 2014
- She, Chunxing; Fedin, Igor; Dolzhnikov, Dmitriy S.
- Nano Letters, Vol. 14, Issue 5
Efficient Exciton Concentrators Built from Colloidal Core/Crown CdSe/CdS Semiconductor Nanoplatelets
journal, December 2013
- Tessier, Mickaël D.; Spinicelli, Piernicola; Dupont, Dorian
- Nano Letters, Vol. 14, Issue 1
Quantum‐well infrared photodetectors
journal, October 1993
- Levine, B. F.
- Journal of Applied Physics, Vol. 74, Issue 8
Chemical Transformations in Ultrathin Chalcogenide Nanowires
journal, March 2010
- Moon, Geon Dae; Ko, Sungwook; Xia, Younan
- ACS Nano, Vol. 4, Issue 4
Synthesis of PbS Nanorods and Other Ionic Nanocrystals of Complex Morphology by Sequential Cation Exchange Reactions
journal, November 2009
- Luther, Joseph M.; Zheng, Haimei; Sadtler, Bryce
- Journal of the American Chemical Society, Vol. 131, Issue 46