Composition of a nickelate composite cathode for a fuel cell

Jung, Hwa Young; Jung, Minjae; Liu, Zhien; Goettler, Rich

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Title: Composition of a nickelate composite cathode for a fuel cell

Abstract

In some embodiments, a solid oxide fuel cell comprising an anode, an electrolyte, cathode barrier layer, a nickelate composite cathode separated from the electrolyte by the cathode barrier layer, and a cathode current collector layer is provided. The nickelate composite cathode includes a nickelate compound and second oxide material, which may be an ion conductor. The composite may further comprise a third oxide material. The composite may have the general formula (Ln_uM1_vM2_s)_n+1(Ni_1-tN_t)_nO_3n+1-A_1-xB_xO_y--C._wD_zCe_(1-w-z)O_2-δ, wherein A and B may be rare earth metals excluding ceria.

Inventors:: Jung, Hwa Young; Jung, Minjae; Liu, Zhien; Goettler, Rich

Issue Date:: 2018-10-30

Research Org.:: LG FUEL CELL SYSTEMS INC., North Canton, OH (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1492020

Patent Number(s):: 10115973

Application Number:: 15/175,913

Assignee:: LG FUEL CELL SYSTEMS INC. (North Canton, OH)

Patent Classifications (CPCs):: H - ELECTRICITY H01 - BASIC ELECTRIC ELEMENTS H01M - PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY

Y - NEW / CROSS SECTIONAL TECHNOLOGIES Y02 - TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE Y02E - REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION

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H - ELECTRICITY H01 - BASIC ELECTRIC ELEMENTS H01M - PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
H01M2004/8689 - {Positive electrodes}
H01M2008/1293 - {Fuel cells with solid oxide electrolytes}
H01M4/8652 - {as mixture}
H01M4/8657 - {layered}
H01M4/8663 - {Selection of inactive substances as ingredients for catalytic active masses, e.g. binders, fillers}
H01M4/8673 - {Electrically conductive fillers}
H01M4/8817 - {Treatment of supports before application of the catalytic active composition
H01M4/9016 - {Oxides, hydroxides or oxygenated metallic salts}
H01M4/9033 - {Complex oxides, optionally doped, of the type M1MeO3, M1 being an alkaline earth metal or a rare earth, Me being a metal, e.g. perovskites}
H01M8/12 - operating at high temperature, e.g. with stabilised ZrO2 electrolyte

Y - NEW / CROSS SECTIONAL TECHNOLOGIES Y02 - TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE Y02E - REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
Y02E60/50 - Fuel cells

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DOE Contract Number:: FE0000303; FE0012077

Resource Type:: Patent

Resource Relation:: Patent File Date: 2016 Jun 07

Country of Publication:: United States

Language:: English

Subject:: 25 ENERGY STORAGE

Citation Formats


                    Jung, Hwa Young, Jung, Minjae, Liu, Zhien, and Goettler, Rich. Composition of a nickelate composite cathode for a fuel cell.  United States: N. p., 2018. 
        Web.

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                    Jung, Hwa Young, Jung, Minjae, Liu, Zhien, & Goettler, Rich. Composition of a nickelate composite cathode for a fuel cell.  United States.

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                    Jung, Hwa Young, Jung, Minjae, Liu, Zhien, and Goettler, Rich. Tue .  
        "Composition of a nickelate composite cathode for a fuel cell".  United States.  https://www.osti.gov/servlets/purl/1492020.

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@article{osti_1492020,

  title        = {Composition of a nickelate composite cathode for a fuel cell},

  author       = {Jung, Hwa Young and Jung, Minjae and Liu, Zhien and Goettler, Rich},

  abstractNote = {In some embodiments, a solid oxide fuel cell comprising an anode, an electrolyte, cathode barrier layer, a nickelate composite cathode separated from the electrolyte by the cathode barrier layer, and a cathode current collector layer is provided. The nickelate composite cathode includes a nickelate compound and second oxide material, which may be an ion conductor. The composite may further comprise a third oxide material. The composite may have the general formula (LnuM1vM2s)n+1(Ni1-tNt)nO3n+1-A1-xBxOy--C.wDzCe(1-w-z)O2-δ, wherein A and B may be rare earth metals excluding ceria.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2018},

  month        = {10}

}

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Works referenced in this record:

Surface-limited oxygen transport and electrode properties of La₂Ni_0.8Cu_0.2O_4+δ
journal, January 2004

Kharton, V. V.; Tsipis, E. V.; Yaremchenko, A. A.
Solid State Ionics, Vol. 166, Issue 3-4, p. 327-337
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Crystal Structure, Diffusion Path, and Oxygen Permeability of a Pr₂NiO₄-Based Mixed Conductor (Pr_0.9La_0.1)₂(Ni_0.74Cu_0.21Ga_0.05)O_4+δ
journal, February 2010

Yashima, Masatomo; Sirikanda, Nuansaeng; Ishihara, Tatsumi
Journal of the American Chemical Society, Vol. 132, Issue 7, p. 2385-2392
https://doi.org/10.1021/ja909820h

Oxygen ion conductors
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Skinner, Stephen J.; Kilner, John A.
Materials Today, Vol. 6, Issue 3, p. 30-37
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Oxygen mobility and surface reactivity of PrNi1−xCoxO3+δ–Ce0.9Y0.1O2−δ cathode nanocomposites
journal, September 2014

Sadykov, V.; Eremeev, N.; Alikina, G.
Solid State Ionics, Vol. 262
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In situ compatibility studies of lanthanum nickelate with a ceria-based electrolyte for SOFC composite cathodes
journal, January 2012

Sayers, R.; Parker, J. E.; Tang, C. C.
Journal of Materials Chemistry, Vol. 22, Issue 8
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Oxygen ion transport in La₂NiO₄‐based ceramics
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Kharton, Vladislav V.; Viskup, Alexandre P.; Naumovich, Eugene N.
Journal of Materials Chemistry, Vol. 9, Issue 10, p. 2623-2629
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Ionic transport in oxygen-hyperstoichiometric phases with K₂NiF₄-type structure
journal, July 2001

Kharton, V. V.; Viskup, A. P.; Kovalevsky, A. V.
Solid State Ionics, Vol. 143, Issue 3-4, p. 337-353
https://doi.org/10.1016/S0167-2738(01)00876-1

Solid Oxide Fuel Cell Cathode Comprising Lanthanum Nickelate
patent-application, August 2007

Lyons, Karen Swider; Laberty, Christel; Zhao, Feng
US Patent Application 11/627485; 20070184324
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High performance praseodymium nickelate oxide cathode for low temperature solid oxide fuel cell
journal, February 2011

Ferchaud, Claire; Grenier, Jean-Claude; Zhang-Steenwinkel, Ye
Journal of Power Sources, Vol. 196, Issue 4, p. 1872-1879
https://doi.org/10.1016/j.jpowsour.2010.09.036

LNF SOFC cathodes with active layer using Pr₆O₁₁ or Pr-doped CeO₂
journal, November 2013

Taguchi, Hiroaki; Chiba, Reiichi; Komatsu, Takeshi
Journal of Power Sources, Vol. 241, p. 768-775
https://doi.org/10.1016/j.jpowsour.2013.04.141

Mechanism of oxygen transfer in layered lanthanide nickelates Ln2 − x NiO4 + δ (Ln = La, Pr) and their nanocomposites with Ce0.9Gd0.1O2 − δ and Y2(Ti0.8Zr0.2)1.6Mn0.4O7 − δ solid electrolytes
journal, July 2013

Sadykov, V. A.; Eremeev, N. F.; Usol’tsev, V. V.
Russian Journal of Electrochemistry, Vol. 49, Issue 7
https://doi.org/10.1134/S1023193513070136

Composition for Fuel Cell Electrode
patent-application, January 2016

Jung, Hwa Young; Xing, Zhengliang; Liu, Zhien
US Patent Application 14/805279; 20160020470
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20160020470

Manganese-based oxygen reduction catalyst, metal-air electrode including said catalyst and methods for making the same
patent, September 2002

Golovin, Neal
US Patent Document 6,444,609
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Oxide material and a fuel cell electrode containing said material
patent, August 2009

Stevens, Philippe; Boehm, Emmanuelle; Basset, Jean-Marc
US Patent Document 7,572,532
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Similar Records

Title: Composition of a nickelate composite cathode for a fuel cell

Abstract

Citation Formats

Surface-limited oxygen transport and electrode properties of La2Ni0.8Cu0.2O4+δ journal, January 2004

Crystal Structure, Diffusion Path, and Oxygen Permeability of a Pr2NiO4-Based Mixed Conductor (Pr0.9La0.1)2(Ni0.74Cu0.21Ga0.05)O4+δ journal, February 2010

Oxygen ion conductors journal, March 2003

Oxygen mobility and surface reactivity of PrNi1−xCoxO3+δ–Ce0.9Y0.1O2−δ cathode nanocomposites journal, September 2014

In situ compatibility studies of lanthanum nickelate with a ceria-based electrolyte for SOFC composite cathodes journal, January 2012

Oxygen ion transport in La2NiO4‐based ceramics journal, January 1999

Ionic transport in oxygen-hyperstoichiometric phases with K2NiF4-type structure journal, July 2001

Solid Oxide Fuel Cell Cathode Comprising Lanthanum Nickelate patent-application, August 2007

High performance praseodymium nickelate oxide cathode for low temperature solid oxide fuel cell journal, February 2011

LNF SOFC cathodes with active layer using Pr6O11 or Pr-doped CeO2 journal, November 2013

Mechanism of oxygen transfer in layered lanthanide nickelates Ln2 − x NiO4 + δ (Ln = La, Pr) and their nanocomposites with Ce0.9Gd0.1O2 − δ and Y2(Ti0.8Zr0.2)1.6Mn0.4O7 − δ solid electrolytes journal, July 2013

Composition for Fuel Cell Electrode patent-application, January 2016

Manganese-based oxygen reduction catalyst, metal-air electrode including said catalyst and methods for making the same patent, September 2002

Oxide material and a fuel cell electrode containing said material patent, August 2009

Surface-limited oxygen transport and electrode properties of La₂Ni_0.8Cu_0.2O_4+δ
journal, January 2004

Crystal Structure, Diffusion Path, and Oxygen Permeability of a Pr₂NiO₄-Based Mixed Conductor (Pr_0.9La_0.1)₂(Ni_0.74Cu_0.21Ga_0.05)O_4+δ
journal, February 2010

Oxygen ion conductors
journal, March 2003

Oxygen mobility and surface reactivity of PrNi1−xCoxO3+δ–Ce0.9Y0.1O2−δ cathode nanocomposites
journal, September 2014

In situ compatibility studies of lanthanum nickelate with a ceria-based electrolyte for SOFC composite cathodes
journal, January 2012

Oxygen ion transport in La₂NiO₄‐based ceramics
journal, January 1999

Ionic transport in oxygen-hyperstoichiometric phases with K₂NiF₄-type structure
journal, July 2001

Solid Oxide Fuel Cell Cathode Comprising Lanthanum Nickelate
patent-application, August 2007

High performance praseodymium nickelate oxide cathode for low temperature solid oxide fuel cell
journal, February 2011

LNF SOFC cathodes with active layer using Pr₆O₁₁ or Pr-doped CeO₂
journal, November 2013

Mechanism of oxygen transfer in layered lanthanide nickelates Ln2 − x NiO4 + δ (Ln = La, Pr) and their nanocomposites with Ce0.9Gd0.1O2 − δ and Y2(Ti0.8Zr0.2)1.6Mn0.4O7 − δ solid electrolytes
journal, July 2013

Composition for Fuel Cell Electrode
patent-application, January 2016

Manganese-based oxygen reduction catalyst, metal-air electrode including said catalyst and methods for making the same
patent, September 2002

Oxide material and a fuel cell electrode containing said material
patent, August 2009