Systems and processes for conversion of ethylene feedstocks to hydrocarbon fuels

Lilga, Michael A.; Hallen, Richard T.; Albrecht, Karl O.; Cooper, Alan R.; Frye, John G.; Ramasamy, Karthikeyan Kallupalayam

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Title: Systems and processes for conversion of ethylene feedstocks to hydrocarbon fuels

Abstract

Systems, processes, and catalysts are disclosed for obtaining fuel and fuel blends containing selected ratios of open-chain and closed-chain fuel-range hydrocarbons suitable for production of alternate fuels including gasolines, jet fuels, and diesel fuels. Fuel-range hydrocarbons may be derived from ethylene-containing feedstocks and ethanol-containing feedstocks.

Inventors:: Lilga, Michael A.; Hallen, Richard T.; Albrecht, Karl O.; Cooper, Alan R.; Frye, John G.; Ramasamy, Karthikeyan Kallupalayam

Issue Date:: 2018-04-03

Research Org.:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1433367

Patent Number(s):: 9932531

Application Number:: 15/494,758

Assignee:: Battelle Memorial Institute (Richland, WA)

Patent Classifications (CPCs):: B - PERFORMING OPERATIONS B01 - PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL B01J - CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY

C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07C - ACYCLIC OR CARBOCYCLIC COMPOUNDS

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B - PERFORMING OPERATIONS B01 - PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL B01J - CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY
B01J21/04 - Alumina
B01J21/12 - Silica and alumina
B01J2208/02 - with stationary particles
B01J2208/027 - Beds
B01J23/42 - Platinum
B01J23/755 - Nickel
B01J29/072 - Iron group metals or copper
B01J29/084 - {Y-type faujasite}
B01J29/40 - of the pentasil type, e.g. types ZSM-5, ZSM-8 or ZSM-11, as exemplified by patent documents US3702886, GB1334243 and US3709979, respectively
B01J29/7007 - {Zeolite Beta}
B01J29/7615 - {Zeolite Beta}
B01J29/90 - Regeneration or reactivation
B01J35/0006 - {Catalysts containing parts with different compositions}
B01J37/0201 - {Impregnation}
B01J38/02 - Heat treatment
B01J8/04 - the fluid passing successively through two or more beds

C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07C - ACYCLIC OR CARBOCYCLIC COMPOUNDS
C07C1/20 - starting from organic compounds containing only oxygen atoms as heteroatoms
C07C1/24 - by elimination of water
C07C11/02 - Alkenes
C07C11/04 - Ethylene
C07C2/12 - with crystalline alumino-silicates {or with catalysts comprising} molecular sieves
C07C2/24 - with metals
C07C2521/12 - Silica and alumina
C07C2523/755 - Nickel
C07C2529/06 - Crystalline aluminosilicate zeolites
C07C2529/072 - Iron group metals or copper
C07C2529/14 - Iron group metals or copper
C07C2529/24 - Iron group metals or copper
C07C2529/46 - Iron group metals or copper
C07C2529/68 - Iron group metals or copper
C07C2529/70 - of types characterised by their specific structure not provided for in groups C07C2529/08 - C07C2529/65
C07C2529/76 - Iron group metals or copper
C07C2529/85 - Silicoaluminophosphates
C07C5/03 - of non-aromatic carbon-to-carbon double bonds

C - CHEMISTRY C10 - PETROLEUM, GAS OR COKE INDUSTRIES C10G - CRACKING HYDROCARBON OILS
C10G2300/1092 - C2-C4 olefins
C10G2300/4081 - Recycling aspects
C10G2400/02 - Gasoline
C10G2400/04 - Diesel oil
C10G2400/08 - Jet fuel
C10G3/00 - Production of liquid hydrocarbon mixtures from oxygen-containing or organic materials, e.g. fatty oils, fatty acids
C10G45/00 - Refining of hydrocarbon oils using hydrogen or hydrogen-generating compounds
C10G50/00 - Production of liquid hydrocarbon mixtures from lower carbon number hydrocarbons, e.g. by oligomerisation
C10G69/126 - {polymerisation, e.g. oligomerisation}

Y - NEW / CROSS SECTIONAL TECHNOLOGIES Y02 - TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE Y02P - CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
Y02P20/52 - using catalysts, e.g. selective catalysts
Y02P20/584 - of catalysts
Y02P30/20 - Bio-feedstock
Y02P30/40 - Ethylene production

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DOE Contract Number:: AC05-76RLO1830

Resource Type:: Patent

Resource Relation:: Patent File Date: 2017 Apr 24

Country of Publication:: United States

Language:: English

Subject:: 09 BIOMASS FUELS

Citation Formats


                    Lilga, Michael A., Hallen, Richard T., Albrecht, Karl O., Cooper, Alan R., Frye, John G., and Ramasamy, Karthikeyan Kallupalayam. Systems and processes for conversion of ethylene feedstocks to hydrocarbon fuels.  United States: N. p., 2018. 
        Web.

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                    Lilga, Michael A., Hallen, Richard T., Albrecht, Karl O., Cooper, Alan R., Frye, John G., & Ramasamy, Karthikeyan Kallupalayam. Systems and processes for conversion of ethylene feedstocks to hydrocarbon fuels.  United States.

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                    Lilga, Michael A., Hallen, Richard T., Albrecht, Karl O., Cooper, Alan R., Frye, John G., and Ramasamy, Karthikeyan Kallupalayam. Tue .  
        "Systems and processes for conversion of ethylene feedstocks to hydrocarbon fuels".  United States.  https://www.osti.gov/servlets/purl/1433367.

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@article{osti_1433367,

  title        = {Systems and processes for conversion of ethylene feedstocks to hydrocarbon fuels},

  author       = {Lilga, Michael A. and Hallen, Richard T. and Albrecht, Karl O. and Cooper, Alan R. and Frye, John G. and Ramasamy, Karthikeyan Kallupalayam},

  abstractNote = {Systems, processes, and catalysts are disclosed for obtaining fuel and fuel blends containing selected ratios of open-chain and closed-chain fuel-range hydrocarbons suitable for production of alternate fuels including gasolines, jet fuels, and diesel fuels. Fuel-range hydrocarbons may be derived from ethylene-containing feedstocks and ethanol-containing feedstocks.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2018},

  month        = {4}

}

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Works referenced in this record:

Multistage conversion of lower olefins with interreactor quenching
patent, April 1988

Garwood, William E.; Krambeck, Frederick J.; Kushnerick, John D.
US Patent Document 4,740,645
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/4740645

Renewable compositions
patent, February 2013

Gruber, Patrick R.; Peters, Matthew W.; Griffith, Josefa M.
US Patent Document 8,378,160
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/8378160

Process for the production of a fuel base from an ethylene feedstock implementing at least one oligomerization stage in the presence of a homogeneous catalytic system
patent, February 2015

Berard, Sandrine; Harry, Stephane; Touchais, Natacha
US Patent Document 8,957,270
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/8957270

Ethylene oligomerization catalyst and use thereof
patent-application, May 2011

Inoue, Koji; Muraishi, Teruo; Heng, Phala
US Patent Application 13/054550; 20110124938
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20110124938

System and method for the production of liquid fuels
patent-application, August 2012

Cantrell, Joel; Morrow, Duane; Peterson, Edward
US Patent Application 13/192396; 20120197053
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20120197053

Conversion of alcohols to distillate fuels
patent-application, April 2014

Greene, Marvin; Song, Ruozhi; Judzis, Jr., Arvids
US Patent Application 14/052972; 20140114101
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20140114101

Catalytic oligomerization of ethene over nickel-exchanged amorphous silica-aluminas; effect of the acid strength of the support
journal, January 1987

Espinoza, R. L.; Snel, R.; Korf, C. J.
Applied Catalysis, Vol. 29, Issue 2, p. 295-303
https://doi.org/10.1016/S0166-9834(00)82899-7

Catalysts and conditions for the highly efficient, selective and stable heterogeneous oligomerisation of ethylene
journal, October 1998

Heveling, J.; Nicolaides, C. P.; Scurrell, M. S.
Applied Catalysis A: General, Vol. 173, Issue 1, p. 1-9
https://doi.org/10.1016/S0926-860X(98)00147-1

Ni-exchanged AlMCM-41—An efficient bifunctional catalyst for ethylene oligomerization
journal, July 2004

Hulea, Vasile; Fajula, François
Journal of Catalysis, Vol. 225, Issue 1, p. 213-222
https://doi.org/10.1016/j.jcat.2004.04.018

Synthesis of ZSM-5 zeolite with small crystal size and its catalytic performance for ethylene oligomerization
journal, November 1994

Yamamura, Masami; Chaki, Kazutoshi; Wakatsuki, Toshiya
Zeolites, Vol. 14, Issue 8, p. 643-649
https://doi.org/10.1016/0144-2449(94)90121-X

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Similar Records

Title: Systems and processes for conversion of ethylene feedstocks to hydrocarbon fuels

Abstract

Citation Formats

Multistage conversion of lower olefins with interreactor quenching patent, April 1988

Renewable compositions patent, February 2013

Process for the production of a fuel base from an ethylene feedstock implementing at least one oligomerization stage in the presence of a homogeneous catalytic system patent, February 2015

Ethylene oligomerization catalyst and use thereof patent-application, May 2011

System and method for the production of liquid fuels patent-application, August 2012

Conversion of alcohols to distillate fuels patent-application, April 2014

Catalytic oligomerization of ethene over nickel-exchanged amorphous silica-aluminas; effect of the acid strength of the support journal, January 1987

Catalysts and conditions for the highly efficient, selective and stable heterogeneous oligomerisation of ethylene journal, October 1998

Ni-exchanged AlMCM-41—An efficient bifunctional catalyst for ethylene oligomerization journal, July 2004

Synthesis of ZSM-5 zeolite with small crystal size and its catalytic performance for ethylene oligomerization journal, November 1994

Multistage conversion of lower olefins with interreactor quenching
patent, April 1988

Renewable compositions
patent, February 2013

Process for the production of a fuel base from an ethylene feedstock implementing at least one oligomerization stage in the presence of a homogeneous catalytic system
patent, February 2015

Ethylene oligomerization catalyst and use thereof
patent-application, May 2011

System and method for the production of liquid fuels
patent-application, August 2012

Conversion of alcohols to distillate fuels
patent-application, April 2014

Catalytic oligomerization of ethene over nickel-exchanged amorphous silica-aluminas; effect of the acid strength of the support
journal, January 1987

Catalysts and conditions for the highly efficient, selective and stable heterogeneous oligomerisation of ethylene
journal, October 1998

Ni-exchanged AlMCM-41—An efficient bifunctional catalyst for ethylene oligomerization
journal, July 2004

Synthesis of ZSM-5 zeolite with small crystal size and its catalytic performance for ethylene oligomerization
journal, November 1994