Silicon oxide based high capacity anode materials for lithium ion batteries

Title: Silicon oxide based high capacity anode materials for lithium ion batteries

Silicon oxide based materials, including composites with various electrical conductive compositions, are formulated into desirable anodes. The anodes can be effectively combined into lithium ion batteries with high capacity cathode materials. In some formulations, supplemental lithium can be used to stabilize cycling as well as to reduce effects of first cycle irreversible capacity loss. Batteries are described with surprisingly good cycling properties with good specific capacities with respect to both cathode active weights and anode active weights.

Inventors:: Deng, Haixia; Han, Yongbong; Masarapu, Charan; Anguchamy, Yogesh Kumar; Lopez, Herman A.; Kumar, Sujeet

Issue Date:: 2017-03-21

OSTI Identifier:: 1347561

Assignee:: Envia Systems, Inc. ARPA-E

Patent Number(s):: 9,601,228

Application Number:: 13/108,708

Contract Number:: AR0000034

Resource Relation:: Patent File Date: 2011 May 16

Research Org:: Envia Systems, Inc. Newark, CA (United States)

Sponsoring Org:: USDOE

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; 25 ENERGY STORAGE

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patent, November 2010

Kim, Han-su; Mah, Sang-kook
US Patent Document 7,833,662
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Alloy compositions for lithium ion batteries
patent, December 2010

Obrovac, Mark N.; Christensen, Leif
US Patent Document 7,851,085
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Alloy composition for lithium ion batteries
patent, January 2011

Obrovac, Mark N.; Christensen, Leif
US Patent Document 7,871,727
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Non-aqueous electrolyte secondary battery
patent, April 2011

Yamamoto, Teruaki; Ueda, Tomohiro; Waki, Shinichi
US Patent Document 7,923,150
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High Capacity, Temperature-Stable Lithium Aluminum Manganese Oxide Cathodes for Rechargeable Batteries
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Chiang, Yet-Ming; Sadoway, Donald R.; Jang, Young‐Il
Electrochemical and Solid-State Letters, Vol. 2, Issue 3, p. 107-110
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Cyclic deterioration and its improvement for Li-rich layered cathode material Li[Ni_0.17Li_0.2Co_0.07Mn_0.56]O₂
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Ito, Atsushi; Li, Decheng; Sato, Yuichi
Journal of Power Sources, Vol. 195, Issue 2, p. 567-573
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A new approach to improve the high-voltage cyclic performance of Li-rich layered cathode material by electrochemical pre-treatment
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Ito, Atsushi; Li, Decheng; Ohsawa, Yasuhiko
Journal of Power Sources, Vol. 183, Issue 1, p. 344-346
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Impedance Analysis of Silicon Nanowire Lithium Ion Battery Anodes
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Ruffo, Riccardo; Hong, Seung Sae; Chan, Candace K.
The Journal of Physical Chemistry C, Vol. 113, Issue 26, p. 11390-11398
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Lithium Insertion in Carbon-Silicon Composite Materials Produced by Mechanical Milling
journal, January 1998

Wang, C. S.; Wu, G. T.; Zhang, X. B.
Journal of The Electrochemical Society, Vol. 145, Issue 8, p. 2751-2758
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Electrochemical Behavior of Nonflammable Organo-Fluorine Compounds for Lithium Ion Batteries
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Achiha, Takashi; Nakajima, Tsuyoshi; Ohzawa, Yoshimi
Journal of The Electrochemical Society, Vol. 156, Issue 6, p. A483-A488
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High-performance lithium battery anodes using silicon nanowires
journal, December 2007

Chan, Candace K.; Peng, Hailin; Liu, Gao
Nature Nanotechnology, Vol. 3, Issue 1, p. 31-35
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Effect of fluoroethylene carbonate additive on interfacial properties of silicon thin-film electrode
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Choi, Nam-Soon; Yew, Kyoung Han; Lee, Kyu Youl
Journal of Power Sources, Vol. 161, Issue 2, p. 1254-1259
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Carbon−Silicon Core−Shell Nanowires as High Capacity Electrode for Lithium Ion Batteries
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Cui, Li-Feng; Yang, Yuan; Hsu, Ching-Mei
Nano Letters, Vol. 9, Issue 9, p. 3370-3374
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SiO_x–graphite as negative for high energy Li-ion batteries
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Guerfi, A.; Charest, P.; Dontigny, M.
Journal of Power Sources, Vol. 196, Issue 13, p. 5667-5673
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Li-Ion Battery Performance with FSI-Based Ionic Liquid Electrolyte and Fluorinated Solvent-Based Electrolyte
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Ishikawa, Masashi; Yamagata, Masaki; Sugimoto, Toshinori
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A Nanostructured SiAl_0.2O Anode Material for Lithium Batteries
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Jeong, Goojin; Kim, Young-Ugk; Krachkovskiy, Sergey A.
Chemistry of Materials, Vol. 22, Issue 19, p. 5570-5579
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Enhancing the rate capability of high capacity xLi₂MnO₃ · (1−x)LiMO₂ (M=Mn, Ni, Co) electrodes by Li–Ni–PO₄ treatment
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Kang, Sun-Ho; Thackeray, Michael M.
Electrochemistry Communications, Vol. 11, Issue 4, p. 748-751
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Layered Li(Li_0.2Ni_0.15+0.5zCo_0.10Mn_0.55−0.5z)O_2−zF_z cathode materials for Li-ion secondary batteries
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Kang, S.-H.; Amine, K.
Journal of Power Sources, Vol. 146, Issue 1-2, p. 654-657
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Synthesis of spherical Li[Ni_(1/3−z)Co_(1/3−z)Mn_(1/3−z)Mg_z]O₂ as positive electrode material for lithium-ion battery
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Kim, Gil-Ho; Myung, Seung-Taek; Kim, Hyun-Soo
Electrochimica Acta, Vol. 51, Issue 12, p. 2447-2453
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Improvement of High-Voltage Cycling Behavior of Surface-Modified Li[Ni[sub 1∕3]Co[sub 1∕3]Mn[sub 1∕3]]O[sub 2] Cathodes by Fluorine Substitution for Li-Ion Batteries
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Kim, G.-H.; Kim, J.-H.; Myung, S.-T.
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High capacity Li[Li_0.2Ni_0.2Mn_0.6]O₂ cathode materials via a carbonate co-precipitation method
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Lee, D.-K.; Park, S.-H.; Amine, K.
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Improvement of cycling stability of Si anode by mechanochemcial reduction and carbon coating
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Liu, Y.; Wen, Z. Y.; Wang, X. Y.
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Electrical transport in doped multiwalled carbon nanotubes
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Liu, K.; Avouris, Ph.; Martel, R.
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Fluoroethylene carbonate electrolyte and its use in lithium ion batteries with graphite anodes
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McMillan, Rod; Slegr, Helen; Shu, Z. X.
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Electrochemical Properties and Chemical Structures of Metal-Doped SiO Anodes for Li-Ion Rechargeable Batteries
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Miyachi, Mariko; Yamamoto, Hironori; Kawai, Hidemasa
Journal of The Electrochemical Society, Vol. 154, Issue 4, p. A376-A380
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Nonflammable Hydrofluoroether for Lithium-Ion Batteries: Enhanced Rate Capability, Cyclability, and Low-Temperature Performance
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Naoi, Katsuhiko; Iwama, Etsuro; Ogihara, Nobuhiro
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Enhanced thermal properties of the solid electrolyte interphase formed on graphite in an electrolyte with fluoroethylene carbonate
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Profatilova, Irina A.; Kim, Sung-Soo; Choi, Nam-Soon
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Nano-SnSb alloy deposited on MCMB as an anode material for lithium ion batteries
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Shi, Lihong; Li, Hong; Wang, Zhaoxiang
Journal of Materials Chemistry, Vol. 11, Issue 5, p. 1502-1505
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AlF₃-Coating to Improve High Voltage Cycling Performance of Li[Ni_1∕3]Co_1∕3]Mn_1∕3]O₂ Cathode Materials for Lithium Secondary Batteries
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Sun, Y.-K.; Cho, S.-W.; Lee, S.-W.
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Sun, Y.; Han, J.; Myung, S.
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Li-doping process for Li_xSiO-negative active material synthesized by chemical method for lithium-ion cells
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Tabuchi, Toru; Yasuda, Hideo; Yamachi, Masanori
Journal of Power Sources, Vol. 146, Issue 1-2, p. 507-509
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Comments on the structural complexity of lithium-rich Li_1+xM_1−xO₂ electrodes (M=Mn, Ni, Co) for lithium batteries
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Thackeray, M. M.; Kang, S.-H.; Johnson, C. S.
Electrochemistry Communications, Vol. 8, Issue 9, p. 1531-1538
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Improvement of cycle behaviour of SiO/C anode composite by thermochemically generated Li₄SiO₄ inert phase for lithium batteries
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Veluchamy, Angathevar; Doh, Chil-Hoon; Kim, Dong-Hun
Journal of Power Sources, Vol. 188, Issue 2, p. 574-577
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Significant Improvement of Electrochemical Performance of AlF₃-Coated Li[Ni_0.8Co_0.1Mn_0.1]O₂ Cathode Materials
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Woo, S.-U.; Yoon, C. S.; Amine, K.
Journal of The Electrochemical Society, Vol. 154, Issue 11, p. A1005-A1009
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Nanosized silicon-based composite derived by in situ mechanochemical reduction for lithium ion batteries
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Yang, Xuelin; Wen, Zhaoyin; Xu, Xiaoxiong
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Electrochemical behaviors of silicon based anode material
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Yoshio, Masaki; Tsumura, Takaaki; Dimov, Nikolay
Journal of Power Sources, Vol. 146, Issue 1-2, p. 10-14
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SiO_x-based anodes for secondary lithium batteries
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Yang, J.; Takeda, Y.; Imanishi, N.
Solid State Ionics, Vol. 152-153, p. 125-129
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Nano-sized SiO_x/C composite anode for lithium ion batteries
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Wang, Jing; Zhao, Hailei; He, Jianchao
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High capacity silicon based anode active materials are described for lithium ion batteries. These materials are shown to be effective in combination with high capacity lithium rich cathode active materials. Supplemental lithium is shown to improve the cycling performance and reduce irreversible capacity loss for at least certain silicon based active materials. In particular silicon based active materials can be formed in composites with electrically conductive coatings, such as pyrolytic carbon coatings or metal coatings, and composites can also be formed with other electrically conductive carbon components, such as carbon nanofibers and carbon nanoparticles. Additional alloys with silicon are explored.
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