Single-reactor process for producing liquid-phase organic compounds from biomass

Dumesic, James A.; Simonetti, Dante A.; Kunkes, Edward L.

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A - human necessities
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Title: Single-reactor process for producing liquid-phase organic compounds from biomass

Abstract

Disclosed is a method for preparing liquid fuel and chemical intermediates from biomass-derived oxygenated hydrocarbons. The method includes the steps of reacting in a single reactor an aqueous solution of a biomass-derived, water-soluble oxygenated hydrocarbon reactant, in the presence of a catalyst comprising a metal selected from the group consisting of Cr, Mn, Fe, Co, Ni, Cu, Mo, Tc, Ru, Rh, Pd, Ag, W, Re, Os, Ir, Pt, and Au, at a temperature, and a pressure, and for a time sufficient to yield a self-separating, three-phase product stream comprising a vapor phase, an organic phase containing linear and/or cyclic mono-oxygenated hydrocarbons, and an aqueous phase.

Inventors:: Dumesic, James A.; Simonetti, Dante A.; Kunkes, Edward L.

Issue Date:: 2015-12-08

Research Org.:: Wisconsin Alumni Research Foundation, Madison, WI (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1228377

Patent Number(s):: 9206145

Application Number:: 13/289,076

Assignee:: Wisconsin Alumni Research Foundation

Patent Classifications (CPCs):: C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07D - HETEROCYCLIC COMPOUNDS

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C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07D - HETEROCYCLIC COMPOUNDS
C07D307/06 - with only hydrogen atoms or radicals containing only hydrogen and carbon atoms, directly attached to ring carbon atoms
C07D309/04 - with only hydrogen atoms, hydrocarbon or substituted hydrocarbon radicals, directly attached to ring carbon atoms

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DOE Contract Number:: FG02-84ER13183

Resource Type:: Patent

Resource Relation:: Patent File Date: 2011 Nov 04

Country of Publication:: United States

Language:: English

Subject:: 21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS

Citation Formats


                    Dumesic, James A., Simonetti, Dante A., and Kunkes, Edward L. Single-reactor process for producing liquid-phase organic compounds from biomass.  United States: N. p., 2015. 
        Web.

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                    Dumesic, James A., Simonetti, Dante A., & Kunkes, Edward L. Single-reactor process for producing liquid-phase organic compounds from biomass.  United States.

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                    Dumesic, James A., Simonetti, Dante A., and Kunkes, Edward L. Tue .  
        "Single-reactor process for producing liquid-phase organic compounds from biomass".  United States.  https://www.osti.gov/servlets/purl/1228377.

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@article{osti_1228377,

  title        = {Single-reactor process for producing liquid-phase organic compounds from biomass},

  author       = {Dumesic, James A. and Simonetti, Dante A. and Kunkes, Edward L.},

  abstractNote = {Disclosed is a method for preparing liquid fuel and chemical intermediates from biomass-derived oxygenated hydrocarbons. The method includes the steps of reacting in a single reactor an aqueous solution of a biomass-derived, water-soluble oxygenated hydrocarbon reactant, in the presence of a catalyst comprising a metal selected from the group consisting of Cr, Mn, Fe, Co, Ni, Cu, Mo, Tc, Ru, Rh, Pd, Ag, W, Re, Os, Ir, Pt, and Au, at a temperature, and a pressure, and for a time sufficient to yield a self-separating, three-phase product stream comprising a vapor phase, an organic phase containing linear and/or cyclic mono-oxygenated hydrocarbons, and an aqueous phase.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2015},

  month        = {12}

}

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Works referenced in this record:

Process for conversion of light paraffins to alkylate in the production of tertiary alkyl ether rich gasoline
patent, April 1992

Harandi, Mohsen N.; Owen, Hartley
US Patent Document 5,106,389
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/5106389

Low-temperature hydrocarbon production from oxygenated hydrocarbons
patent, October 2005

Cortright, Randy D.; Dumesic, James A.
US Patent Document 6,953,873
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6953873

Methods and systems for generating polyols
patent, August 2010

Cortright, Randy D.
US Patent Document 7,767,867
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7767867