Succinic anhydrides from epoxides

Coates, Geoffrey W; Rowley, John M

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Title: Succinic anhydrides from epoxides

Abstract

Catalysts and methods for the double carbonylation of epoxides are disclosed. Each epoxide molecule reacts with two molecules of carbon monoxide to produce a succinic anhydride. The reaction is facilitated by catalysts combining a Lewis acidic species with a transition metal carbonyl complex. The double carbonylation is achieved in single process by using reaction conditions under which both carbonylation reactions occur without the necessity of isolating or purifying the product of the first carbonylation.

Inventors:: Coates, Geoffrey W; Rowley, John M

Issue Date:: 2014-12-30

Research Org.:: Cornell Univ., Ithaca, NY (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1166757

Patent Number(s):: 8921581

Application Number:: 13/914,592

Assignee:: Cornell Research Foundation, Inc. (Ithaca, NY)

Patent Classifications (CPCs):: C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07D - HETEROCYCLIC COMPOUNDS

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C - CHEMISTRY C07 - ORGANIC CHEMISTRY C07D - HETEROCYCLIC COMPOUNDS
C07D307/60 - Two oxygen atoms, e.g. succinic anhydride

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DOE Contract Number:: FG02-05ER15687

Resource Type:: Patent

Resource Relation:: Patent File Date: 2013 Jun 10

Country of Publication:: United States

Language:: English

Subject:: 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats


                    Coates, Geoffrey W, and Rowley, John M. Succinic anhydrides from epoxides.  United States: N. p., 2014. 
        Web.

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                    Coates, Geoffrey W, & Rowley, John M. Succinic anhydrides from epoxides.  United States.

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                    Coates, Geoffrey W, and Rowley, John M. Tue .  
        "Succinic anhydrides from epoxides".  United States.  https://www.osti.gov/servlets/purl/1166757.

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@article{osti_1166757,

  title        = {Succinic anhydrides from epoxides},

  author       = {Coates, Geoffrey W and Rowley, John M},

  abstractNote = {Catalysts and methods for the double carbonylation of epoxides are disclosed. Each epoxide molecule reacts with two molecules of carbon monoxide to produce a succinic anhydride. The reaction is facilitated by catalysts combining a Lewis acidic species with a transition metal carbonyl complex. The double carbonylation is achieved in single process by using reaction conditions under which both carbonylation reactions occur without the necessity of isolating or purifying the product of the first carbonylation.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2014},

  month        = {12}

}

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Works referenced in this record:

Polycarbonates made using high activity catalysts
patent, October 2000

Coates, Geoffrey W.; Cheng, Ming
US Patent Document 6,133,402
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6133402

Catalytic carbonylation of three and four membered heterocycles
patent, February 2005

Coates, Geoffrey W.; Getzler, Yutan D. Y. L.; Wolczanski, Peter
US Patent Document 6,852,865
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6852865

Polycarbonates made using highly selective catalysts
patent, December 2007

Coates, Geoffrey W.; Qin, Zengquan; Cohen, Claire
US Patent Document 7,304,172
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7304172

Low pressure carbonylation of heterocycles
patent, August 2009

Coates, Geoffrey W.; Kramer, John W.
US Patent Document 7,569,709
URL: https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7569709