Solid-state lithium battery

Ihlefeld, Jon; Clem, Paul G; Edney, Cynthia; Ingersoll, David; Nagasubramanian, Ganesan; Fenton, Kyle Ross

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Title: Solid-state lithium battery

Abstract

The present invention is directed to a higher power, thin film lithium-ion electrolyte on a metallic substrate, enabling mass-produced solid-state lithium batteries. High-temperature thermodynamic equilibrium processing enables co-firing of oxides and base metals, providing a means to integrate the crystalline, lithium-stable, fast lithium-ion conductor lanthanum lithium tantalate (La.sub.1/3-xLi.sub.3xTaO.sub.3) directly with a thin metal foil current collector appropriate for a lithium-free solid-state battery.

Inventors:: Ihlefeld, Jon; Clem, Paul G; Edney, Cynthia; Ingersoll, David; Nagasubramanian, Ganesan; Fenton, Kyle Ross

Issue Date:: 2014-11-04

Research Org.:: Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1163202

Patent Number(s):: 8877388

Application Number:: 13/478,766

Assignee:: Sandia Corporation (Albuquerque, NM)

Patent Classifications (CPCs):: C - CHEMISTRY C01 - INORGANIC CHEMISTRY C01G - COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F

C - CHEMISTRY C01 - INORGANIC CHEMISTRY C01P - INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS

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C - CHEMISTRY C01 - INORGANIC CHEMISTRY C01G - COMPOUNDS CONTAINING METALS NOT COVERED BY SUBCLASSES C01D OR C01F
C01G35/006 - {Compounds containing, besides tantalum, two or more other elements, with the exception of oxygen or hydrogen}

C - CHEMISTRY C01 - INORGANIC CHEMISTRY C01P - INDEXING SCHEME RELATING TO STRUCTURAL AND PHYSICAL ASPECTS OF SOLID INORGANIC COMPOUNDS
C01P2002/72 - by d-values or two theta-values, e.g. as X-ray diagram
C01P2004/03 - obtained by SEM
C01P2004/04 - obtained by TEM, STEM, STM or AFM
C01P2006/40 - Electric properties

H - ELECTRICITY H01 - BASIC ELECTRIC ELEMENTS H01M - PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
H01M10/0436 - {Small-sized flat cells or batteries for portable equipment}
H01M10/052 - Li-accumulators
H01M10/0562 - Solid materials
H01M10/058 - Construction or manufacture
H01M2300/0071 - Oxides
H01M6/40 - Printed batteries {, e.g. thin film batteries}

Y - NEW / CROSS SECTIONAL TECHNOLOGIES Y02 - TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE Y02E - REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
Y02E60/10 - Energy storage

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DOE Contract Number:: AC04-94AL85000

Resource Type:: Patent

Resource Relation:: Patent File Date: 2012 May 23

Country of Publication:: United States

Language:: English

Subject:: 25 ENERGY STORAGE

Citation Formats


                    Ihlefeld, Jon, Clem, Paul G, Edney, Cynthia, Ingersoll, David, Nagasubramanian, Ganesan, and Fenton, Kyle Ross. Solid-state lithium battery.  United States: N. p., 2014. 
        Web.

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                    Ihlefeld, Jon, Clem, Paul G, Edney, Cynthia, Ingersoll, David, Nagasubramanian, Ganesan, & Fenton, Kyle Ross. Solid-state lithium battery.  United States.

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                    Ihlefeld, Jon, Clem, Paul G, Edney, Cynthia, Ingersoll, David, Nagasubramanian, Ganesan, and Fenton, Kyle Ross. Tue .  
        "Solid-state lithium battery".  United States.  https://www.osti.gov/servlets/purl/1163202.

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@article{osti_1163202,

  title        = {Solid-state lithium battery},

  author       = {Ihlefeld, Jon and Clem, Paul G and Edney, Cynthia and Ingersoll, David and Nagasubramanian, Ganesan and Fenton, Kyle Ross},

  abstractNote = {The present invention is directed to a higher power, thin film lithium-ion electrolyte on a metallic substrate, enabling mass-produced solid-state lithium batteries. High-temperature thermodynamic equilibrium processing enables co-firing of oxides and base metals, providing a means to integrate the crystalline, lithium-stable, fast lithium-ion conductor lanthanum lithium tantalate (La.sub.1/3-xLi.sub.3xTaO.sub.3) directly with a thin metal foil current collector appropriate for a lithium-free solid-state battery.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2014},

  month        = {11}

}

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Rechargeable thin film battery and method for making the same
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Method and apparatus for solid-state microbattery photolithographic manufacture, singulation and passivation
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Inaguma, Yoshiyuki; Liquan, Chen; Itoh, Mitsuru
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Mizumoto, K.
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Crystal Structure and Lithium Ion Conductivity of A-Site Deficient Perovskites La1/3-xLi3xTaO3
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Mizumoto, Katsuyoshi; Hayashi, Shinsuke
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Lithium Ion Mobility and Activation Energy for Lithium Ion Conduction in A-Site Deficient Perovskites La1/3-xLi3xTaO3
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Mizumoto, Katsuyoshi; Hayashi, Shinsuke
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Conductivity relaxation in lithium ion conductors with the perovskite-type structure
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Mizumoto, K.
Solid State Ionics, Vol. 127, Issue 3-4
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Synthesis of lanthanum lithium tantalate powders and thin films by the sol–gel method
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Arakawa, Shuichi; Nitta, Hiroaki; Hayashi, Shinsuke
Journal of Crystal Growth, Vol. 231, Issue 1-2, p. 290-294
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Works referencing / citing this record:

Composite electrodes for lithium ion battery and method of making
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Methods of preventing corrosion of surfaces by application of energy storage-conversion devices
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Garnet-type solid electrolyte, secondary battery containing garnet-type solid electrolyte, and method of producing garnet-type solid electrolyte
patent, May 2015

Teshima, Katsuya; Hozumi, Masato
US Patent Document 9,034,526
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Title: Solid-state lithium battery

Abstract

Citation Formats

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Interconnect supported fuel cell assembly, preform and method of fabrication patent-application, December 2003

Method and apparatus for solid-state microbattery photolithographic manufacture, singulation and passivation patent-application, February 2008

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Lithium Ion Conductivity of A-Site Deficient Perovskite Solid Solution La[sub 0.67−x]Li[sub 3x]TiO[sub 3] journal, January 1994

Developments of high-voltage all-solid-state thin-film lithium ion batteries journal, March 2006

High ionic conductivity in lithium lanthanum titanate journal, June 1993

Lithium ion conduction in A-site deficient perovskites R1/4Li1/4TaO3 (R=La, Nd, Sm and Y) journal, January 1999

Crystal Structure and Lithium Ion Conductivity of A-Site Deficient Perovskites La1/3-xLi3xTaO3 journal, January 1997

Lithium Ion Mobility and Activation Energy for Lithium Ion Conduction in A-Site Deficient Perovskites La1/3-xLi3xTaO3 journal, January 1998

Conductivity relaxation in lithium ion conductors with the perovskite-type structure journal, January 2000

Synthesis of lanthanum lithium tantalate powders and thin films by the sol–gel method journal, September 2001

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Lithium Ion Conductivity of A-Site Deficient Perovskite Solid Solution La[sub 0.67−x]Li[sub 3x]TiO[sub 3]
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Developments of high-voltage all-solid-state thin-film lithium ion batteries
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High ionic conductivity in lithium lanthanum titanate
journal, June 1993

Lithium ion conduction in A-site deficient perovskites R1/4Li1/4TaO3 (R=La, Nd, Sm and Y)
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Crystal Structure and Lithium Ion Conductivity of A-Site Deficient Perovskites La1/3-xLi3xTaO3
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Lithium Ion Mobility and Activation Energy for Lithium Ion Conduction in A-Site Deficient Perovskites La1/3-xLi3xTaO3
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Conductivity relaxation in lithium ion conductors with the perovskite-type structure
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High Temperature Vaporization Behavior of Oxides. I. Alkali Metal Binary Oxides
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Garnet-type solid electrolyte, secondary battery containing garnet-type solid electrolyte, and method of producing garnet-type solid electrolyte
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