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Title: Methods of analyzing composition of aerosol particles

Abstract

An aerosol particle analyzer includes a laser ablation chamber, a gas-filled conduit, and a mass spectrometer. The laser ablation chamber can be operated at a low pressure, which can be from 0.1 mTorr to 30 mTorr. The ablated ions are transferred into a gas-filled conduit. The gas-filled conduit reduces the electrical charge and the speed of ablated ions as they collide and mix with buffer gases in the gas-filled conduit. Preferably, the gas filled-conduit includes an electromagnetic multipole structure that collimates the nascent ions into a beam, which is guided into the mass spectrometer. Because the gas-filled conduit allows storage of vast quantities of the ions from the ablated particles, the ions from a single ablated particle can be analyzed multiple times and by a variety of techniques to supply statistically meaningful analysis of composition and isotope ratios.

Inventors:
Issue Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1083195
Patent Number(s):
8373119
Application Number:
13/561,365
Assignee:
UT-Battelle, LLC (Oak Ridge, TN)
Patent Classifications (CPCs):
H - ELECTRICITY H01 - BASIC ELECTRIC ELEMENTS H01J - ELECTRIC DISCHARGE TUBES OR DISCHARGE LAMPS
DOE Contract Number:  
AC05-00OR22725
Resource Type:
Patent
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION

Citation Formats

Reilly, Peter T.A. Methods of analyzing composition of aerosol particles. United States: N. p., 2013. Web.
Reilly, Peter T.A. Methods of analyzing composition of aerosol particles. United States.
Reilly, Peter T.A. Tue . "Methods of analyzing composition of aerosol particles". United States. https://www.osti.gov/servlets/purl/1083195.
@article{osti_1083195,
title = {Methods of analyzing composition of aerosol particles},
author = {Reilly, Peter T.A.},
abstractNote = {An aerosol particle analyzer includes a laser ablation chamber, a gas-filled conduit, and a mass spectrometer. The laser ablation chamber can be operated at a low pressure, which can be from 0.1 mTorr to 30 mTorr. The ablated ions are transferred into a gas-filled conduit. The gas-filled conduit reduces the electrical charge and the speed of ablated ions as they collide and mix with buffer gases in the gas-filled conduit. Preferably, the gas filled-conduit includes an electromagnetic multipole structure that collimates the nascent ions into a beam, which is guided into the mass spectrometer. Because the gas-filled conduit allows storage of vast quantities of the ions from the ablated particles, the ions from a single ablated particle can be analyzed multiple times and by a variety of techniques to supply statistically meaningful analysis of composition and isotope ratios.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Tue Feb 12 00:00:00 EST 2013},
month = {Tue Feb 12 00:00:00 EST 2013}
}

Works referenced in this record:

Chemical Characterization of Individual, Airborne Sub-10-nm Particles and Molecules
journal, March 2006


Measurement of Individual Particle Atomic Composition by Aerosol Mass Spectrometry
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A Design Tool for Aerodynamic Lens Systems
journal, June 2006


Ultra high mass range mass spectrometer systems
patent, December 2005


Mass spectrometer system including a double ion guide interface and method of operation
patent, February 2009


Sensitive Glow Discharge Ion Source for Aerosol and Gas Analysis
patent-application, February 2007


Laser ablation flowing atmospheric-pressure afterglow for ambient mass spectrometry
patent-application, November 2009


Transverse flow aerodynamic lens
patent, November 1991


Method for producing nanoparticles and nanostructured films
patent-application, December 2005