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Title: Synthesis gas method and apparatus

Abstract

A method and apparatus for producing a synthesis gas product having one or more oxygen transport membrane elements thermally coupled to one or more catalytic reactors such that heat generated from the oxygen transport membrane element supplies endothermic heating requirements for steam methane reforming reactions occurring within the catalytic reactor through radiation and convention heat transfer. A hydrogen containing stream containing no more than 20 percent methane is combusted within the oxygen transport membrane element to produce the heat and a heated combustion product stream. The heated combustion product stream is combined with a reactant stream to form a combined stream that is subjected to the reforming within the catalytic reactor. The apparatus may include modules in which tubular membrane elements surround a central reactor tube.

Inventors:
; ; ; ; ; ; ;
Issue Date:
Research Org.:
National Energy Technology Laboratory (NETL), Pittsburgh, PA, Morgantown, WV (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1082901
Patent Number(s):
8349214
Application Number:
13/179,279
Assignee:
Praxair Technology, Inc. (Danbury, CT)
Patent Classifications (CPCs):
B - PERFORMING OPERATIONS B01 - PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL B01J - CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY
C - CHEMISTRY C01 - INORGANIC CHEMISTRY C01B - NON-METALLIC ELEMENTS
DOE Contract Number:  
FC26-07NT43088
Resource Type:
Patent
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION

Citation Formats

Kelly, Sean M., Kromer, Brian R., Litwin, Michael M., Rosen, Lee J., Christie, Gervase Maxwell, Wilson, Jamie R., Kosowski, Lawrence W., and Robinson, Charles. Synthesis gas method and apparatus. United States: N. p., 2013. Web.
Kelly, Sean M., Kromer, Brian R., Litwin, Michael M., Rosen, Lee J., Christie, Gervase Maxwell, Wilson, Jamie R., Kosowski, Lawrence W., & Robinson, Charles. Synthesis gas method and apparatus. United States.
Kelly, Sean M., Kromer, Brian R., Litwin, Michael M., Rosen, Lee J., Christie, Gervase Maxwell, Wilson, Jamie R., Kosowski, Lawrence W., and Robinson, Charles. Tue . "Synthesis gas method and apparatus". United States. https://www.osti.gov/servlets/purl/1082901.
@article{osti_1082901,
title = {Synthesis gas method and apparatus},
author = {Kelly, Sean M. and Kromer, Brian R. and Litwin, Michael M. and Rosen, Lee J. and Christie, Gervase Maxwell and Wilson, Jamie R. and Kosowski, Lawrence W. and Robinson, Charles},
abstractNote = {A method and apparatus for producing a synthesis gas product having one or more oxygen transport membrane elements thermally coupled to one or more catalytic reactors such that heat generated from the oxygen transport membrane element supplies endothermic heating requirements for steam methane reforming reactions occurring within the catalytic reactor through radiation and convention heat transfer. A hydrogen containing stream containing no more than 20 percent methane is combusted within the oxygen transport membrane element to produce the heat and a heated combustion product stream. The heated combustion product stream is combined with a reactant stream to form a combined stream that is subjected to the reforming within the catalytic reactor. The apparatus may include modules in which tubular membrane elements surround a central reactor tube.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Tue Jan 08 00:00:00 EST 2013},
month = {Tue Jan 08 00:00:00 EST 2013}
}

Works referenced in this record:

Production of synthesis gas by mixed conducting membranes
patent, April 2000


Syngas production method utilizing an oxygen transport membrane
patent, February 2004


Synthesis gas and carbon dioxide generation method
patent, September 2008


Hydrogen production method
patent, August 2004


Ceramic membrane for endothermic reactions
patent, October 2001


Synthesis gas process comprising partial oxidation using controlled and optimized temperature profile
patent-application, February 2006


Utilization of synthesis gas produced by mixed conducting membranes
patent, August 2000


Laboratory workstation for providing samples
patent-application, February 2007


Process for producing a syngas
patent, June 2002


Method and apparatus for light internal reforming in a solid oxide fuel cell system
patent-application, March 2007


Synthesis gas and carbon dioxide generation method
patent-application, February 2007


Staged Membrane Oxidation Reactor System
patent-application, December 2008