Multidimensional spectrometer

Zanni, Martin Thomas; Damrauer, Niels H

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Title: Multidimensional spectrometer

Abstract

A multidimensional spectrometer for the infrared, visible, and ultraviolet regions of the electromagnetic spectrum, and a method for making multidimensional spectroscopic measurements in the infrared, visible, and ultraviolet regions of the electromagnetic spectrum. The multidimensional spectrometer facilitates measurements of inter- and intra-molecular interactions.

Inventors:

Zanni, Martin Thomas ^[1]; Damrauer, Niels H ^[2]

Madison, WI
Boulder, CO

Issue Date:: 2010-07-20

Research Org.:: Wisconsin Alumni Research Foundation (Madison, WI); The Regents of the University of Colorado (Denver, CO)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1012815

Patent Number(s):: 7760342

Application Number:: 11/963,123

Assignee:: Wisconsin Alumni Research Foundation (Madison, WI) The Regents of the University of Colorado (Denver, CO)

Patent Classifications (CPCs):: G - PHYSICS G01 - MEASURING G01J - MEASUREMENT OF INTENSITY, VELOCITY, SPECTRAL CONTENT, POLARISATION, PHASE OR PULSE CHARACTERISTICS OF INFRA-RED, VISIBLE OR ULTRA-VIOLET LIGHT

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G - PHYSICS G01 - MEASURING G01J - MEASUREMENT OF INTENSITY, VELOCITY, SPECTRAL CONTENT, POLARISATION, PHASE OR PULSE CHARACTERISTICS OF INFRA-RED, VISIBLE OR ULTRA-VIOLET LIGHT
G01J3/10 - Arrangements of light sources specially adapted for spectrometry or colorimetry
G01J3/433 - Modulation spectrometry

Show less

DOE Contract Number:: FG02-07ER15890

Resource Type:: Patent

Country of Publication:: United States

Language:: English

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                    Zanni, Martin Thomas, and Damrauer, Niels H. Multidimensional spectrometer.  United States: N. p., 2010. 
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                    Zanni, Martin Thomas, & Damrauer, Niels H. Multidimensional spectrometer.  United States.

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                    Zanni, Martin Thomas, and Damrauer, Niels H. Tue .  
        "Multidimensional spectrometer".  United States.  https://www.osti.gov/servlets/purl/1012815.

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@article{osti_1012815,

  title        = {Multidimensional spectrometer},

  author       = {Zanni, Martin Thomas and Damrauer, Niels H},

  abstractNote = {A multidimensional spectrometer for the infrared, visible, and ultraviolet regions of the electromagnetic spectrum, and a method for making multidimensional spectroscopic measurements in the infrared, visible, and ultraviolet regions of the electromagnetic spectrum. The multidimensional spectrometer facilitates measurements of inter- and intra-molecular interactions.},

  doi          = {},

  journal      = {},
number       = ,

  volume       = ,

  place        = {United States},

  year         = {2010},

  month        = {7}

}

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In response to a user request, a computer generates a graphical user interface on a computer display. A schema information region of the graphical user interface includes multiple operand names, each operand name associated with one or more fields of a multi-dimensional database. A data visualization region of the graphical user interface includes multiple shelves. Upon detecting a user selection of the operand names and a user request to associate each user-selected operand name with a respective shelf in the data visualization region, the computer generates a visual table in the data visualization region in accordance with the associations betweenmore » « less
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Multidimensional bioseparation with modular microfluidics

Patent Chirica, Gabriela S.; Renzi, Ronald F.

A multidimensional chemical separation and analysis system is described including a prototyping platform and modular microfluidic components capable of rapid and convenient assembly, alteration and disassembly of numerous candidate separation systems. Partial or total computer control of the separation system is possible. Single or multiple alternative processing trains can be tested, optimized and/or run in parallel. Examples related to the separation and analysis of human bodily fluids are given.
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Title: Multidimensional spectrometer

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Local structure and dynamics of liquid acetone by heterodyned 2D IR spectroscopy conference, January 2002

The two-dimensional IR nonlinear spectroscopy of a cyclic penta-peptide in relation to its three-dimensional structure journal, March 1999

Inter-peptide interaction and delocalization of amide I vibrational excitons in myoglobin and flavodoxin journal, October 2002

Coherently Controlled Ultrafast Four-Wave Mixing Spectroscopy journal, June 2007

Site-specific vibrational dynamics of the CD3ζ membrane peptide using heterodyned two-dimensional infrared photon echo spectroscopy journal, June 2004

Conformational Preferences and Vibrational Frequency Distributions of Short Peptides in Relation to Multidimensional Infrared Spectroscopy journal, December 2001

Inter and Intrastrand Vibrational Coupling in DNA Studied with Heterodyned 2D-IR Spectroscopy journal, September 2003

Correlation between electronic and molecular structure distortions and vibrational properties. II. Amide I modes of NMA–nD2O complexes journal, February 2003

Correlated line broadening in multidimensional vibrational spectroscopy journal, December 2002

Linear and nonlinear infrared signatures of local α- and 310-helical structures in alanine polypeptides journal, February 2003

Vibrational Coupling, Isotopic Editing, and β-Sheet Structure in a Membrane-Bound Polypeptide journal, May 2004

Two-dimensional spectroscopy at infrared and optical frequencies journal, July 2007

Two-Dimensional Electronic Correlation and Relaxation Spectra: Theory and Model Calculations journal, December 1999

Dual-frequency 2D-IR spectroscopy heterodyned photon echo of the peptide bond journal, April 2003

The hammerhead ribozyme journal, November 2002

Ultrafast vibrational spectroscopy in condensed phases journal, January 2002

Two-dimensional IR spectroscopy can be designed to eliminate the diagonal peaks and expose only the crosspeaks needed for structure determination journal, September 2001

Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide journal, May 2007

Characteristics of the two-dimensional infrared spectroscopy of helices from approximate simulations and analytic models journal, February 2004

Passively correcting phase drift in two-dimensional infrared spectroscopy journal, January 2006

Multidimensional femtosecond spectroscopies of molecular aggregates and semiconductor nanostructures: The nonlinear exciton equations journal, December 1998

Obtaining Absorptive Line Shapes in Two-Dimensional Infrared Vibrational Correlation Spectra journal, January 2003

Noise in homodyne and heterodyne detection journal, January 1983

Whither the Future of Controlling Quantum Phenomena? journal, May 2000

Facile collection of two-dimensional electronic spectra using femtosecond pulse-shaping Technology journal, January 2007

Rate of unwinding small DNA journal, November 1971

Determination of the Secondary Structure and Conformation of Puroindolines by Infrared and Raman Spectroscopy † journal, January 1996

Disentangling multidimensional femtosecond spectra of excitons by pulse shaping with coherent control journal, May 2004

Structure Determination of Trialanine in Water Using Polarization Sensitive Two-Dimensional Vibrational Spectroscopy journal, November 2000

A pulse sequence for directly measuring the anharmonicities of coupled vibrations: Two-quantum two-dimensional infrared spectroscopy journal, May 2004

Femtosecond direct space-to-time pulse with MEMS micromirror arrays conference, January 2003

Femtosecond Phase-Coherent Two-Dimensional Spectroscopy journal, June 2003

Heterodyned 3D IR spectroscopy journal, November 2007

Transient 2D-IR Spectroscopy: Snapshots of the Nonequilibrium Ensemble during the Picosecond Conformational Transition of a Small Peptide journal, August 2003

Design strategies for pulse sequences in multidimensional optical spectroscopies journal, September 2001

Vibrational Spectroscopy and Conformation of Peptides, Polypeptides, and Proteins book, January 1986

Vibrational Anharmonicities Revealed by Coherent Two-Dimensional Infrared Spectroscopy journal, March 2001

Ultrafast heterodyne detected infrared multidimensional vibrational stimulated echo studies of hydrogen bond dynamics journal, June 2003

Nature of structural inhomogeneities on folding a helix and their influence on spectral measurements journal, June 2004

Two-dimensional circularly polarized pump–probe spectroscopy journal, October 2003

General Method for the Dimension Reduction of Adaptive Control Experiments journal, May 2006

Structure of the Amide I Band of Peptides Measured by Femtosecond Nonlinear-Infrared Spectroscopy journal, July 1998

Controlling Vibrational Excitation with Shaped Mid-IR Pulses journal, July 2007

Infrared analogs of heteronuclear nuclear magnetic resonance coherence transfer experiments in peptides journal, April 2002

Nonlinear response functions for the three-dimensional spectroscopies journal, September 2001

Two-dimensional infrared spectroscopy of peptides by phase-controlled femtosecond vibrational photon echoes journal, July 2000

Coupling of the Amide I Modes of the Glycine Dipeptide journal, May 2002

Algorithms for the synthesis of complex-value spectral filters with an array of micromechanical mirrors journal, January 2006

The origin of vibrational mode couplings in various secondary structural motifs of polypeptides journal, January 2004

Hydrogen-bond dynamics in water explored by heterodyne-detected photon echo journal, February 2003

Amide I modes in the N -methylacetamide dimer and glycine dipeptide analog: Diagonal force constants journal, April 2003

Mid infrared pulse shaping by optical parametric amplification and its application to optical free induction decay measurement journal, January 2003

Vibrational coherence transfer characterized with Fourier-transform 2D IR spectroscopy journal, January 2004

Acousto-optical shaping of ultraviolet femtosecond pulses journal, March 2005

Heterodyned Two-Dimensional Infrared Spectroscopy of Solvent-Dependent Conformations of Acetylproline-NH 2 † journal, July 2001

Frequency Selected Ultrafast Infrared Vibrational Echo Studies of Liquids, Glasses, and Proteins journal, September 2002

Generation, shaping, and characterization of intense femtosecond pulses tunable from 3 to 20 μm journal, January 2000

Pump/probe self heterodyned 2D spectroscopy of vibrational transitions of a small globular peptide journal, January 2000

Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation journal, January 2006

Femtosecond pulse shaping using spatial light modulators journal, May 2000

Amide I Modes of α-Helical Polypeptide in Liquid Water: Conformational Fluctuation, Phase Correlation, and Linear and Nonlinear Vibrational Spectra journal, July 2004

Nonlinear Two-Dimensional Vibrational Spectroscopy journal, July 2000

Vibrational-exciton relaxation probed by three-pulse echoes in polypeptides journal, May 2001

Signatures of β-Peptide Unfolding in Two-Dimensional Vibrational Echo Spectroscopy: A Simulation Study journal, April 2001

Frequency Resolved and Heterodyned Femtosecond Infrared Echoes of Pep tides; Multiple Pulse Coherent Vibrational Analogues ofNMR book, January 2001

Experimental Determinations of Coherent Multidimensional Vibrational Spectroscopy journal, August 2003

Coherent Transients book, January 1991

Ultrafast Hydrogen-Bond Dynamics in the Infrared Spectroscopy of Water journal, September 2003

Doubly Vibrationally Enhanced Four Wave Mixing: The Optical Analog to 2D NMR journal, February 2000

Local structure and dynamics of liquid acetone by heterodyned 2D IR spectroscopy
conference, January 2002

The two-dimensional IR nonlinear spectroscopy of a cyclic penta-peptide in relation to its three-dimensional structure
journal, March 1999

Inter-peptide interaction and delocalization of amide I vibrational excitons in myoglobin and flavodoxin
journal, October 2002

Coherently Controlled Ultrafast Four-Wave Mixing Spectroscopy
journal, June 2007

Site-specific vibrational dynamics of the CD3ζ membrane peptide using heterodyned two-dimensional infrared photon echo spectroscopy
journal, June 2004

Conformational Preferences and Vibrational Frequency Distributions of Short Peptides in Relation to Multidimensional Infrared Spectroscopy
journal, December 2001

Inter and Intrastrand Vibrational Coupling in DNA Studied with Heterodyned 2D-IR Spectroscopy
journal, September 2003

Correlation between electronic and molecular structure distortions and vibrational properties. II. Amide I modes of NMA–nD2O complexes
journal, February 2003

Correlated line broadening in multidimensional vibrational spectroscopy
journal, December 2002

Linear and nonlinear infrared signatures of local α- and 310-helical structures in alanine polypeptides
journal, February 2003

Vibrational Coupling, Isotopic Editing, and β-Sheet Structure in a Membrane-Bound Polypeptide
journal, May 2004

Two-dimensional spectroscopy at infrared and optical frequencies
journal, July 2007

Two-Dimensional Electronic Correlation and Relaxation Spectra: Theory and Model Calculations
journal, December 1999

Dual-frequency 2D-IR spectroscopy heterodyned photon echo of the peptide bond
journal, April 2003

The hammerhead ribozyme
journal, November 2002

Ultrafast vibrational spectroscopy in condensed phases
journal, January 2002

Two-dimensional IR spectroscopy can be designed to eliminate the diagonal peaks and expose only the crosspeaks needed for structure determination
journal, September 2001

Automated 2D IR spectroscopy using a mid-IR pulse shaper and application of this technology to the human islet amyloid polypeptide
journal, May 2007

Characteristics of the two-dimensional infrared spectroscopy of helices from approximate simulations and analytic models
journal, February 2004

Passively correcting phase drift in two-dimensional infrared spectroscopy
journal, January 2006

Multidimensional femtosecond spectroscopies of molecular aggregates and semiconductor nanostructures: The nonlinear exciton equations
journal, December 1998

Obtaining Absorptive Line Shapes in Two-Dimensional Infrared Vibrational Correlation Spectra
journal, January 2003

Noise in homodyne and heterodyne detection
journal, January 1983

Whither the Future of Controlling Quantum Phenomena?
journal, May 2000

Facile collection of two-dimensional electronic spectra using femtosecond pulse-shaping Technology
journal, January 2007

Rate of unwinding small DNA
journal, November 1971

Determination of the Secondary Structure and Conformation of Puroindolines by Infrared and Raman Spectroscopy ^†
journal, January 1996

Disentangling multidimensional femtosecond spectra of excitons by pulse shaping with coherent control
journal, May 2004

Structure Determination of Trialanine in Water Using Polarization Sensitive Two-Dimensional Vibrational Spectroscopy
journal, November 2000

A pulse sequence for directly measuring the anharmonicities of coupled vibrations: Two-quantum two-dimensional infrared spectroscopy
journal, May 2004

Femtosecond direct space-to-time pulse with MEMS micromirror arrays
conference, January 2003

Femtosecond Phase-Coherent Two-Dimensional Spectroscopy
journal, June 2003

Heterodyned 3D IR spectroscopy
journal, November 2007

Transient 2D-IR Spectroscopy: Snapshots of the Nonequilibrium Ensemble during the Picosecond Conformational Transition of a Small Peptide
journal, August 2003

Design strategies for pulse sequences in multidimensional optical spectroscopies
journal, September 2001

Vibrational Spectroscopy and Conformation of Peptides, Polypeptides, and Proteins
book, January 1986

Vibrational Anharmonicities Revealed by Coherent Two-Dimensional Infrared Spectroscopy
journal, March 2001

Ultrafast heterodyne detected infrared multidimensional vibrational stimulated echo studies of hydrogen bond dynamics
journal, June 2003

Nature of structural inhomogeneities on folding a helix and their influence on spectral measurements
journal, June 2004

Two-dimensional circularly polarized pump–probe spectroscopy
journal, October 2003

General Method for the Dimension Reduction of Adaptive Control Experiments
journal, May 2006

Structure of the Amide I Band of Peptides Measured by Femtosecond Nonlinear-Infrared Spectroscopy
journal, July 1998

Controlling Vibrational Excitation with Shaped Mid-IR Pulses
journal, July 2007

Infrared analogs of heteronuclear nuclear magnetic resonance coherence transfer experiments in peptides
journal, April 2002

Nonlinear response functions for the three-dimensional spectroscopies
journal, September 2001

Two-dimensional infrared spectroscopy of peptides by phase-controlled femtosecond vibrational photon echoes
journal, July 2000

Coupling of the Amide I Modes of the Glycine Dipeptide
journal, May 2002

Algorithms for the synthesis of complex-value spectral filters with an array of micromechanical mirrors
journal, January 2006

The origin of vibrational mode couplings in various secondary structural motifs of polypeptides
journal, January 2004

Hydrogen-bond dynamics in water explored by heterodyne-detected photon echo
journal, February 2003

Amide I modes in the N -methylacetamide dimer and glycine dipeptide analog: Diagonal force constants
journal, April 2003

Mid infrared pulse shaping by optical parametric amplification and its application to optical free induction decay measurement
journal, January 2003

Vibrational coherence transfer characterized with Fourier-transform 2D IR spectroscopy
journal, January 2004

Acousto-optical shaping of ultraviolet femtosecond pulses
journal, March 2005

Heterodyned Two-Dimensional Infrared Spectroscopy of Solvent-Dependent Conformations of Acetylproline-NH ₂ ^†
journal, July 2001

Frequency Selected Ultrafast Infrared Vibrational Echo Studies of Liquids, Glasses, and Proteins
journal, September 2002

Generation, shaping, and characterization of intense femtosecond pulses tunable from 3 to 20 μm
journal, January 2000

Pump/probe self heterodyned 2D spectroscopy of vibrational transitions of a small globular peptide
journal, January 2000

Femtosecond pulse shaping directly in the mid-IR using acousto-optic modulation
journal, January 2006

Femtosecond pulse shaping using spatial light modulators
journal, May 2000

Amide I Modes of α-Helical Polypeptide in Liquid Water: Conformational Fluctuation, Phase Correlation, and Linear and Nonlinear Vibrational Spectra
journal, July 2004

Nonlinear Two-Dimensional Vibrational Spectroscopy
journal, July 2000

Vibrational-exciton relaxation probed by three-pulse echoes in polypeptides
journal, May 2001

Signatures of β-Peptide Unfolding in Two-Dimensional Vibrational Echo Spectroscopy: A Simulation Study
journal, April 2001

Frequency Resolved and Heterodyned Femtosecond Infrared Echoes of Pep tides; Multiple Pulse Coherent Vibrational Analogues ofNMR
book, January 2001

Experimental Determinations of Coherent Multidimensional Vibrational Spectroscopy
journal, August 2003

Coherent Transients
book, January 1991

Ultrafast Hydrogen-Bond Dynamics in the Infrared Spectroscopy of Water
journal, September 2003

Doubly Vibrationally Enhanced Four Wave Mixing: The Optical Analog to 2D NMR
journal, February 2000