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Title: Plutonium Contamination Issues in Hanford Soils and Sediments: Discharges from the Z-Plant (PFP) Complex

Journal Article · · Physics and Chemistry of the Earth, 35(6-8):292-297

Beginning in 1945, weapons production activities at the Hanford Nuclear Reservation resulted in the discharge of large quantities of Pu and other transuranic elements to the subsurface. The vast majority of the transuranics were disposed in the Hanford central plateau (200 areas) predominately associated with activities at the Z-Plant (Plutonium Finishing Plant) complex. In the past the Pu and Am migrated deep into the subsurface at certain locations, although the Pu and other transuranics are not currently being detected in significant concentration in any associated groundwaters. Evaluation of the chemical form of the transuranics in the subsurface along with determining the mechanism(s) of the past subsurface migration is important in establishing strategies for long-term site management practices. Unfortunately, the chemical form of the transuranics in the deep subsurface sediments and the past mechanism of vertical migration remain largely unknown. This paper present a summary of the different waste types and locations where transuranics were disposed, the factors that could have lead to subsurface migration via different transport vectors, the information currently available on the chemical form of Pu in the subsurface, and a summary of current research needs.

Research Organization:
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC05-76RL01830
OSTI ID:
988617
Report Number(s):
PNNL-SA-69092; KP1702030; TRN: US201018%%577
Journal Information:
Physics and Chemistry of the Earth, 35(6-8):292-297, Vol. 35, Issue 6-8
Country of Publication:
United States
Language:
English