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Title: Dynamics of quantum spin liquid and spin solid phases in IPA-CuCl3 under an applied magnetic field studied with neutron scattering

Abstract

Inelastic and elastic neutron scattering is used to study spin correlations in the quasi-one-dimensional quantum antiferromagnet IPA-CuCl3 in strong applied magnetic fields. A condensation of magnons and commensurate transverse long-range ordering is observe at a critical field Hc=9.5 T. The field dependencies of the energies and polarizations of all magnon branches are investigated both below and above the transition point. Their dispersion is measured across the entire one-dimensional Brillouin zone in magnetic fields up to 14 T. The critical wave vector of magnon spectrum truncation Masuda et al., Phys. Rev. Lett. 96, 047210 2006 is found to shift from hc0,35 at HHC to hc=0.25 for HHC. A drastic reduction of magnon bandwidths in the ordered phase Garlea et al., Phys. Rev. Lett. 98, 167202 2007 is observed and studied in detail. New features of the spectrum, presumably related to this bandwidth collapse, are observed just above the transition field.

Authors:
 [1];  [1];  [2];  [3];  [4];  [4];  [4];  [5];  [5];  [6];  [6];  [7]
  1. ORNL
  2. Yokohama City University, Japan
  3. Kagoshima University, Kagoshima JAPAN
  4. CEA, Grenoble, France
  5. National Institute of Standards and Technology (NIST)
  6. Hahn-Meitner Institut, Berlin, Germany
  7. Institut Laue-Langevin (ILL)
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
931095
DOE Contract Number:
DE-AC05-00OR22725
Resource Type:
Journal Article
Resource Relation:
Journal Name: Physical Review B; Journal Volume: 98
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; BRILLOUIN ZONES; CRITICAL FIELD; MAGNETIC FIELDS; MAGNONS; NEUTRONS; SCATTERING; SPIN; VECTORS

Citation Formats

Zheludev, Andrey I, Garlea, Vasile O, Masuda, T., Manaka, H., Regnault, L.-P., Ressouche, E., Grenier, B., Chung, J.-H., Qiu, Y., Habicht, Klaus, Kiefer, K., and Boehm, Martin. Dynamics of quantum spin liquid and spin solid phases in IPA-CuCl3 under an applied magnetic field studied with neutron scattering. United States: N. p., 2007. Web. doi:10.1103/PhysRevB.76.054450.
Zheludev, Andrey I, Garlea, Vasile O, Masuda, T., Manaka, H., Regnault, L.-P., Ressouche, E., Grenier, B., Chung, J.-H., Qiu, Y., Habicht, Klaus, Kiefer, K., & Boehm, Martin. Dynamics of quantum spin liquid and spin solid phases in IPA-CuCl3 under an applied magnetic field studied with neutron scattering. United States. doi:10.1103/PhysRevB.76.054450.
Zheludev, Andrey I, Garlea, Vasile O, Masuda, T., Manaka, H., Regnault, L.-P., Ressouche, E., Grenier, B., Chung, J.-H., Qiu, Y., Habicht, Klaus, Kiefer, K., and Boehm, Martin. 2007. "Dynamics of quantum spin liquid and spin solid phases in IPA-CuCl3 under an applied magnetic field studied with neutron scattering". United States. doi:10.1103/PhysRevB.76.054450.
@article{osti_931095,
title = {Dynamics of quantum spin liquid and spin solid phases in IPA-CuCl3 under an applied magnetic field studied with neutron scattering},
author = {Zheludev, Andrey I and Garlea, Vasile O and Masuda, T. and Manaka, H. and Regnault, L.-P. and Ressouche, E. and Grenier, B. and Chung, J.-H. and Qiu, Y. and Habicht, Klaus and Kiefer, K. and Boehm, Martin},
abstractNote = {Inelastic and elastic neutron scattering is used to study spin correlations in the quasi-one-dimensional quantum antiferromagnet IPA-CuCl3 in strong applied magnetic fields. A condensation of magnons and commensurate transverse long-range ordering is observe at a critical field Hc=9.5 T. The field dependencies of the energies and polarizations of all magnon branches are investigated both below and above the transition point. Their dispersion is measured across the entire one-dimensional Brillouin zone in magnetic fields up to 14 T. The critical wave vector of magnon spectrum truncation Masuda et al., Phys. Rev. Lett. 96, 047210 2006 is found to shift from hc0,35 at HHC to hc=0.25 for HHC. A drastic reduction of magnon bandwidths in the ordered phase Garlea et al., Phys. Rev. Lett. 98, 167202 2007 is observed and studied in detail. New features of the spectrum, presumably related to this bandwidth collapse, are observed just above the transition field.},
doi = {10.1103/PhysRevB.76.054450},
journal = {Physical Review B},
number = ,
volume = 98,
place = {United States},
year = 2007,
month = 1
}
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