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Title: Cryogenic Neutron Spectrometer Development

Abstract

Cryogenic microcalorimeter detectors operating at temperatures around {approx}0.1 K have been developed for the last two decades, driven mostly by the need for ultra-high energy resolution (<0.1%) in X-ray astrophysics and dark matter searches [1]. The Advanced Detector Group at Lawrence Livermore National Laboratory has developed different cryogenic detector technologies for applications ranging from X-ray astrophysics to nuclear science and non-proliferation. In particular, we have adapted cryogenic detector technologies for ultra-high energy resolution gamma-spectroscopy [2] and, more recently, fast-neutron spectroscopy [3]. Microcalorimeters are essentially ultra-sensitive thermometers that measure the energy of the radiation from the increase in temperature upon absorption. They consist of a sensitive superconducting thermometer operated at the transition between its superconducting and its normal state, where its resistance changes very rapidly with temperature such that even the minute energies deposited by single radiation quanta are sufficient to be detectable with high precision. The energy resolution of microcalorimeters is fundamentally limited by thermal fluctuations to {Delta}E{sub FWHM} {approx} 2.355 (k{sub B}T{sup 2}C{sub abs}){sup 1/2}, and thus allows an energy below 1 keV for neutron spectrometers for an operating temperature of T {approx} 0.1 K . The {Delta}E{sub FWHM} does not depend on the energy of the incident photonmore » or particle. This expression is equivalent to the familiar (F{var_epsilon}E{sub {gamma}}){sup 1/2} considering that an absorber at temperature T contains a total energy C{sub abs}T, and the associated fluctuation are due to variations in uncorrelated (F=1) phonons ({var_epsilon} = k{sub B}T) dominated by the background energy C{sub abs}T >> E{gamma}. The rationale behind developing a cryogenic neutron spectrometer is the very high energy resolution combined with the high efficiency. Additionally, the response function is simple and the instrument is transportable. We are currently developing a fast neutron spectrometer with 0.1% energy resolution at 1 MeV neutron energy with an efficiency of > 1%. Our fast-neutron spectrometers use boron-based and {sup 6}LiF absorber crystals with Mo/Cu thermistors readout. They have achieved an energy resolution of 5.5 keV FWHM for 2.79 MeV deposited in {sup 10}B by thermal neutron capture (fig. 1), and 46 keV FWHM for fast (MeV) neutrons absorbed in {sup 6}LiF (fig. 2). Since the energy resolution does not depend on the neutron energy, we expect a similar energy resolution for MeV neutron energies. The response function is given simply by the cross section of the capture reaction, offset from zero by the Q-value of the capture reaction. This allows straightforward discrimination against gamma-events, most of which deposit less that Q{sub 6Li} = 4.79 MeV in the {sup 6}LiF absorber, and easy deconvolution of the neutron spectrum, since there is only a single capture reaction in {sup 6}Li and the spectrum is not affected by edge effects or geometric broadening. The current challenge for microcalorimeters is their necessarily small effective pixel area, {approx}1cm{sup 3} for neutron spectrometer pixels, and their slow decay time, {approx}10ms for neutron spectrometers. The pixel size is limited by the requirement for low Cabs for high energy resolution; the decay time is set by the intrinsically weak thermal coupling between materials at low temperatures. Both issues can be addressed by fabricating large detector arrays. This will enable high-precision neutron spectrometry with high statistics, such as simulated for Pu analysis in fig 3.« less

Authors:
; ; ; ; ;
Publication Date:
Research Org.:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
928539
Report Number(s):
UCRL-CONF-219829
TRN: US0803283
DOE Contract Number:
W-7405-ENG-48
Resource Type:
Conference
Resource Relation:
Conference: Presented at: The 11th Symposium on Radiation Measurements and Applications, Ann Arbor, MI, United States, May 23 - May 25, 2006
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; ASTROPHYSICS; CROSS SECTIONS; CRYOGENICS; ENERGY RESOLUTION; FAST NEUTRONS; GAMMA SPECTROSCOPY; LAWRENCE LIVERMORE NATIONAL LABORATORY; NEUTRON SPECTROMETERS; NEUTRON SPECTROSCOPY; NEUTRONS; NONLUMINOUS MATTER; RADIATIONS; RESPONSE FUNCTIONS; SPECTROMETERS; THERMAL NEUTRONS

Citation Formats

Niedermayr, T, Hau, I D, Friedrich, S, Burger, A, Roy, U N, and Bell, Z W. Cryogenic Neutron Spectrometer Development. United States: N. p., 2006. Web.
Niedermayr, T, Hau, I D, Friedrich, S, Burger, A, Roy, U N, & Bell, Z W. Cryogenic Neutron Spectrometer Development. United States.
Niedermayr, T, Hau, I D, Friedrich, S, Burger, A, Roy, U N, and Bell, Z W. Wed . "Cryogenic Neutron Spectrometer Development". United States. doi:. https://www.osti.gov/servlets/purl/928539.
@article{osti_928539,
title = {Cryogenic Neutron Spectrometer Development},
author = {Niedermayr, T and Hau, I D and Friedrich, S and Burger, A and Roy, U N and Bell, Z W},
abstractNote = {Cryogenic microcalorimeter detectors operating at temperatures around {approx}0.1 K have been developed for the last two decades, driven mostly by the need for ultra-high energy resolution (<0.1%) in X-ray astrophysics and dark matter searches [1]. The Advanced Detector Group at Lawrence Livermore National Laboratory has developed different cryogenic detector technologies for applications ranging from X-ray astrophysics to nuclear science and non-proliferation. In particular, we have adapted cryogenic detector technologies for ultra-high energy resolution gamma-spectroscopy [2] and, more recently, fast-neutron spectroscopy [3]. Microcalorimeters are essentially ultra-sensitive thermometers that measure the energy of the radiation from the increase in temperature upon absorption. They consist of a sensitive superconducting thermometer operated at the transition between its superconducting and its normal state, where its resistance changes very rapidly with temperature such that even the minute energies deposited by single radiation quanta are sufficient to be detectable with high precision. The energy resolution of microcalorimeters is fundamentally limited by thermal fluctuations to {Delta}E{sub FWHM} {approx} 2.355 (k{sub B}T{sup 2}C{sub abs}){sup 1/2}, and thus allows an energy below 1 keV for neutron spectrometers for an operating temperature of T {approx} 0.1 K . The {Delta}E{sub FWHM} does not depend on the energy of the incident photon or particle. This expression is equivalent to the familiar (F{var_epsilon}E{sub {gamma}}){sup 1/2} considering that an absorber at temperature T contains a total energy C{sub abs}T, and the associated fluctuation are due to variations in uncorrelated (F=1) phonons ({var_epsilon} = k{sub B}T) dominated by the background energy C{sub abs}T >> E{gamma}. The rationale behind developing a cryogenic neutron spectrometer is the very high energy resolution combined with the high efficiency. Additionally, the response function is simple and the instrument is transportable. We are currently developing a fast neutron spectrometer with 0.1% energy resolution at 1 MeV neutron energy with an efficiency of > 1%. Our fast-neutron spectrometers use boron-based and {sup 6}LiF absorber crystals with Mo/Cu thermistors readout. They have achieved an energy resolution of 5.5 keV FWHM for 2.79 MeV deposited in {sup 10}B by thermal neutron capture (fig. 1), and 46 keV FWHM for fast (MeV) neutrons absorbed in {sup 6}LiF (fig. 2). Since the energy resolution does not depend on the neutron energy, we expect a similar energy resolution for MeV neutron energies. The response function is given simply by the cross section of the capture reaction, offset from zero by the Q-value of the capture reaction. This allows straightforward discrimination against gamma-events, most of which deposit less that Q{sub 6Li} = 4.79 MeV in the {sup 6}LiF absorber, and easy deconvolution of the neutron spectrum, since there is only a single capture reaction in {sup 6}Li and the spectrum is not affected by edge effects or geometric broadening. The current challenge for microcalorimeters is their necessarily small effective pixel area, {approx}1cm{sup 3} for neutron spectrometer pixels, and their slow decay time, {approx}10ms for neutron spectrometers. The pixel size is limited by the requirement for low Cabs for high energy resolution; the decay time is set by the intrinsically weak thermal coupling between materials at low temperatures. Both issues can be addressed by fabricating large detector arrays. This will enable high-precision neutron spectrometry with high statistics, such as simulated for Pu analysis in fig 3.},
doi = {},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Wed Mar 08 00:00:00 EST 2006},
month = {Wed Mar 08 00:00:00 EST 2006}
}

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