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Fabrication of carbon nanotube films from alkyne-transition metal complexes

Patent ·
OSTI ID:913336

A simple method for the production or synthesis of carbon nanotubes as free-standing films or nanotube mats by the thermal decomposition of transition metal complexed alkynes with aryl, alkyl, alkenyl, or alkynyl substituents. In particular, transition metal (e.g. Co, Ni, Fe, Mo) complexes of diarylacetylenes, e.g. diphenylacetylene, and solid mixtures of these complexes with suitable, additional carbon sources are heated in a vessel. More specifically, the heating of the transition metal complex is completed at a temperature between 400-800.degree. C. and more particularly 550-700.degree. C. for between 0.1 to 24 hours and more particularly 0.5-3 hours in a sealed vessel under a partial pressure of argon or helium.

Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA
Sponsoring Organization:
United States Department of Energy
DOE Contract Number:
AC03-76SF00098
Assignee:
The Regents of the University of California (Oakland, CA)
Patent Number(s):
7,261,871
Application Number:
10/261,366
OSTI ID:
913336
Country of Publication:
United States
Language:
English

References (1)

Single-walled nanotubes by the pyrolysis of acetylene-organometallic mixtures journal August 1998

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