Preliminary analysis of DHLW (Defense High-Level Waste) glass performance as related to the NRC 10CFR60 slow release limit criterion
A preliminary analysis was performed to determine if the dissolution resistance of Defense High-Level Waste (DHLW) glass in silicia-saturated brine is sufficient to meet the Nuclear Regulatory Commission (NRC) fractional release rate requirement for nuclear waste repositories. The sensitivities of fractional release to variations in temperature, surface area, and matrix solubility were also examined. Results indicate that a waste form dissolution resistance strategy is potentially viable for demonstrating compliance with the NRC regulatory requirement. However, major uncertainties exist in two areas: demonstrating that the brine contacting the glass is saturated in silica, and predicting the exposed glass surface area. 12more »