Method of immobilizing carbon dioxide from gas streams
Patent
·
OSTI ID:863394
- Knoxville, TN
- Oliver Springs, TN
This invention is a method for rapidly and continuously immobilizing carbon dioxide contained in various industrial off-gas streams, the carbon dioxide being immobilized as dry, stable, and substantially water-insoluble particulates. Briefly, the method comprises passing the gas stream through a fixed or fluidized bed of hydrated barium hydroxide to remove and immobilize the carbon dioxide by converting the bed to barium carbonate. The method has several important advantages: it can be conducted effectively at ambient temperature; it provides a very rapid reaction rate over a wide range of carbon dioxide concentrations; it provides high decontamination factors; and it has a high capacity for carbon dioxide. The invention is especially well suited for the removal of radioactive carbon dioxide from off-gases generated by nuclear-fuel reprocessing facilities and nuclear power plants.
- Research Organization:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN
- Assignee:
- United States of America as represented by United States (Washington, DC)
- Patent Number(s):
- US 4162298
- OSTI ID:
- 863394
- Country of Publication:
- United States
- Language:
- English
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Related Subjects
/588/376/423/
active carbon
advantages
ambient
ambient temperature
barium
barium hydroxide
bed
briefly
capacity
carbon
carbon dioxide
carbonate
comprises
comprises passing
concentrations
conducted
contained
continuously
converting
decontamination
decontamination factor
dioxide
dry
effectively
especially
facilities
factors
fixed
fluidized
fluidized bed
fuel reprocessing
gas
gas stream
gas streams
gases generated
generated
hydrated
hydroxide
immobilize
immobilized
immobilizing
immobilizing carbon
industrial
method
method comprise
method comprises
nuclear
nuclear power
nuclear-fuel
off-gas
off-gas stream
off-gases
oxide concentration
particulates
passing
plants
power
power plant
power plants
provides
radioactive
range
rapid
rapidly
rate
reaction
reaction rate
removal
remove
reprocessing
stable
stream
streams
substantially
substantially water-insoluble
suited
temperature
various
water-insoluble
wide
wide range
active carbon
advantages
ambient
ambient temperature
barium
barium hydroxide
bed
briefly
capacity
carbon
carbon dioxide
carbonate
comprises
comprises passing
concentrations
conducted
contained
continuously
converting
decontamination
decontamination factor
dioxide
dry
effectively
especially
facilities
factors
fixed
fluidized
fluidized bed
fuel reprocessing
gas
gas stream
gas streams
gases generated
generated
hydrated
hydroxide
immobilize
immobilized
immobilizing
immobilizing carbon
industrial
method
method comprise
method comprises
nuclear
nuclear power
nuclear-fuel
off-gas
off-gas stream
off-gases
oxide concentration
particulates
passing
plants
power
power plant
power plants
provides
radioactive
range
rapid
rapidly
rate
reaction
reaction rate
removal
remove
reprocessing
stable
stream
streams
substantially
substantially water-insoluble
suited
temperature
various
water-insoluble
wide
wide range