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Title: Integrated High Temperature Coal to Hydrogen System with CO2 Separation: Semi-Annual Progress Report 1

Abstract

This is the first semi-annual progress report for the program "Integrated High Temperature Coal to Hydrogen System with CO2 Separation." The objective of the program is to develop a detailed design for a single high-temperature syngas-cleanup module to produce a pure stream of H2 from a coal-based system and to develop the new high-temperature membrane materials at the core of that design. The novel one-box process combines a shift reactor with a high-temperature CO2-selective membrane to convert CO to CO2, remove sulfur compounds, and remove CO2 in a simple, compact, fully integrated system. In the first six months of the program, a conceptual design for the one-box system was developed in Task 1 and the performance targets for the system and the membrane were evaluated. In Task 2.1 processes were developed for creating pore architectures in ceramics that are applicable to membrane structures. In Task 2.2, candidate materials were identified that have the potential for separation of CO2 and H2S at high temperatures.

Authors:
; ; ;
Publication Date:
Research Org.:
GE Global Research
Sponsoring Org.:
USDOE - Office of Fossil Energy (FE)
OSTI Identifier:
861563
Report Number(s):
DOE-NT-42451-1
DOE Contract Number:  
FC26-05NT42451
Resource Type:
Technical Report
Country of Publication:
United States
Language:
English
Subject:
01 COAL, LIGNITE, AND PEAT; 36 MATERIALS SCIENCE; coal gasification; CO2 separation; syngas cleanup; membrane

Citation Formats

Ruud, J A, Ku, A, Ramaswamy, V, and Wei, W. Integrated High Temperature Coal to Hydrogen System with CO2 Separation: Semi-Annual Progress Report 1. United States: N. p., 2005. Web. doi:10.2172/861563.
Ruud, J A, Ku, A, Ramaswamy, V, & Wei, W. Integrated High Temperature Coal to Hydrogen System with CO2 Separation: Semi-Annual Progress Report 1. United States. doi:10.2172/861563.
Ruud, J A, Ku, A, Ramaswamy, V, and Wei, W. Wed . "Integrated High Temperature Coal to Hydrogen System with CO2 Separation: Semi-Annual Progress Report 1". United States. doi:10.2172/861563. https://www.osti.gov/servlets/purl/861563.
@article{osti_861563,
title = {Integrated High Temperature Coal to Hydrogen System with CO2 Separation: Semi-Annual Progress Report 1},
author = {Ruud, J A and Ku, A and Ramaswamy, V and Wei, W},
abstractNote = {This is the first semi-annual progress report for the program "Integrated High Temperature Coal to Hydrogen System with CO2 Separation." The objective of the program is to develop a detailed design for a single high-temperature syngas-cleanup module to produce a pure stream of H2 from a coal-based system and to develop the new high-temperature membrane materials at the core of that design. The novel one-box process combines a shift reactor with a high-temperature CO2-selective membrane to convert CO to CO2, remove sulfur compounds, and remove CO2 in a simple, compact, fully integrated system. In the first six months of the program, a conceptual design for the one-box system was developed in Task 1 and the performance targets for the system and the membrane were evaluated. In Task 2.1 processes were developed for creating pore architectures in ceramics that are applicable to membrane structures. In Task 2.2, candidate materials were identified that have the potential for separation of CO2 and H2S at high temperatures.},
doi = {10.2172/861563},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Wed Dec 21 00:00:00 EST 2005},
month = {Wed Dec 21 00:00:00 EST 2005}
}

Technical Report:

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