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Title: Strong-field laser ionization of alkali atoms using two-dimensional cylindrical and three-dimensional Cartesian time-dependent Hartree--Fock theory

Abstract

The time-dependent Schroedinger equation is solved directly for an alkali atom subject to an arbitrarily strong electromagnetic field. Two methods are compared. A tridiagonal finite-difference method is used to solve Schroedinger's equation on a two-dimensional (2D) cylindrical coordinate lattice, while a finite-element method using odd-order {ital B} splines is used to solve Schroedinger's equation on a three-dimensional (3D) Cartesian coordinate lattice. Multiphoton ionization cross sections are extracted from 2D cylindrical calculations for hydrogen and lithium and then compared with previous perturbation theory results. Single-photon ionization probabilities are compared from 2D cylindrical and 3D Cartesian calculations for hydrogen.

Authors:
 [1]; ;  [2]
  1. Department of Physics, Auburn University, Auburn, Alabama 36849 (USA)
  2. Physics Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830 (USA)
Publication Date:
OSTI Identifier:
6916939
DOE Contract Number:  
AC05-84OR21400
Resource Type:
Journal Article
Journal Name:
Journal of the Optical Society of America, Part B: Optical Physics; (USA)
Additional Journal Information:
Journal Volume: 7:4; Journal ID: ISSN 0740-3224
Country of Publication:
United States
Language:
English
Subject:
74 ATOMIC AND MOLECULAR PHYSICS; ALKALI METALS; MULTI-PHOTON PROCESSES; HYDROGEN; QUANTUM ELECTRONICS; ATOMS; ELECTRIC FIELDS; HARTREE-FOCK METHOD; LASER RADIATION; PHOTOIONIZATION; TIME DEPENDENCE; ELECTROMAGNETIC RADIATION; ELEMENTS; IONIZATION; METALS; NONMETALS; RADIATIONS; 640302* - Atomic, Molecular & Chemical Physics- Atomic & Molecular Properties & Theory

Citation Formats

Pindzola, M S, Bottrell, G J, and Bottcher, C. Strong-field laser ionization of alkali atoms using two-dimensional cylindrical and three-dimensional Cartesian time-dependent Hartree--Fock theory. United States: N. p., 1990. Web. doi:10.1364/JOSAB.7.000659.
Pindzola, M S, Bottrell, G J, & Bottcher, C. Strong-field laser ionization of alkali atoms using two-dimensional cylindrical and three-dimensional Cartesian time-dependent Hartree--Fock theory. United States. https://doi.org/10.1364/JOSAB.7.000659
Pindzola, M S, Bottrell, G J, and Bottcher, C. 1990. "Strong-field laser ionization of alkali atoms using two-dimensional cylindrical and three-dimensional Cartesian time-dependent Hartree--Fock theory". United States. https://doi.org/10.1364/JOSAB.7.000659.
@article{osti_6916939,
title = {Strong-field laser ionization of alkali atoms using two-dimensional cylindrical and three-dimensional Cartesian time-dependent Hartree--Fock theory},
author = {Pindzola, M S and Bottrell, G J and Bottcher, C},
abstractNote = {The time-dependent Schroedinger equation is solved directly for an alkali atom subject to an arbitrarily strong electromagnetic field. Two methods are compared. A tridiagonal finite-difference method is used to solve Schroedinger's equation on a two-dimensional (2D) cylindrical coordinate lattice, while a finite-element method using odd-order {ital B} splines is used to solve Schroedinger's equation on a three-dimensional (3D) Cartesian coordinate lattice. Multiphoton ionization cross sections are extracted from 2D cylindrical calculations for hydrogen and lithium and then compared with previous perturbation theory results. Single-photon ionization probabilities are compared from 2D cylindrical and 3D Cartesian calculations for hydrogen.},
doi = {10.1364/JOSAB.7.000659},
url = {https://www.osti.gov/biblio/6916939}, journal = {Journal of the Optical Society of America, Part B: Optical Physics; (USA)},
issn = {0740-3224},
number = ,
volume = 7:4,
place = {United States},
year = {Sun Apr 01 00:00:00 EST 1990},
month = {Sun Apr 01 00:00:00 EST 1990}
}