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Title: A time-resolved x-ray scattering technique for observation of non-equilibrium phonons

Journal Article · · Review of Scientific Instruments; (USA)
DOI:https://doi.org/10.1063/1.1141906· OSTI ID:6910112
 [1];  [2];  [3]
  1. National Synchrotron Light Source, Brookhaven National Lab, Upton, New York 11973 (US)
  2. School of Materials Engineering, Purdue University, West Lafayette, Indiana 47907 (USA)
  3. National Synchrotron Light Source, Brookhaven National Lab, Upton, New York 11973 (USA)

We have demonstrated a time-resolved x-ray diffraction technique for observing nonequilibrium phonons. We have used this technique to observe phonons in {alpha}-quartz at low temperatures. Phonons were generated by direct stimulation of near zone center transverse-optical phonons using infrared light from a powerful {ital Q} switched CO{sub 2} laser. We show data taken at a Brillouin zone boundary confirming the presence of nonequilibrium phonons initially generated by the laser and their resulting decay products.

DOE Contract Number:
FG02-85ER45183; AC02-76CH00016
OSTI ID:
6910112
Journal Information:
Review of Scientific Instruments; (USA), Vol. 61:1; ISSN 0034-6748
Country of Publication:
United States
Language:
English