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Title: Measurements of the effects of humidity on radio-aerosol penetration through ultrafine capillaries

Abstract

The purpose of this research was to examine the effects of humidity on radio-aerosol penetration through ultrafine capillaries. A number of tests were conducted at relative humidities of 20%, 50%, and 80%, with sampling times of 20, 40, and 60 min. The radio-aerosol consisted of polystyrene particles with a diameter of 0.1 {micro}m. The ultrafine capillaries had a diameter of 250 {micro}m. The data from these tests varied significantly. These results made the identification of radio-aerosol penetration trends inconclusive. The standard deviation for all penetration data ranged from 3% to 30%. The results of this study suggest that a better control of the experimental parameters was needed to obtain more accurate data from experiments associated with radio-aerosol penetration in the presence of moisture. The experimental parameters that may have contributed to the wide variance of data, include aerosol flow, radio-aerosol generation, capillary characteristics, humidity control, and radiation measurements. It was the uncertainty of these parameters that contributed to the poor data which made conclusive deductions about radio-aerosol penetration dependence on humidity difficult. The application of this study is to ultrafine leaks resulting from stress fractures in high-level nuclear waste transportation casks under accident scenarios.

Authors:
Publication Date:
Research Org.:
Missouri Univ., Columbia, MO (United States)
Sponsoring Org.:
USDOE Office of Energy Research, Washington, DC (United States)
OSTI Identifier:
573154
Report Number(s):
DOE/OR/00033-T732
ON: DE97053609; TRN: 98:008597
DOE Contract Number:
AC05-76OR00033
Resource Type:
Technical Report
Resource Relation:
Other Information: TH: Thesis (M.S.); PBD: Aug 1996
Country of Publication:
United States
Language:
English
Subject:
05 NUCLEAR FUELS; RADIOACTIVE AEROSOLS; WASTE TRANSPORTATION; CAPILLARY FLOW; DIFFUSION; CONTAINERS; HUMIDITY; PERMEABILITY; LEAKS; HIGH-LEVEL RADIOACTIVE WASTES; RADIATION ACCIDENTS; EXPERIMENTAL DATA

Citation Formats

Cullen, C. Measurements of the effects of humidity on radio-aerosol penetration through ultrafine capillaries. United States: N. p., 1996. Web. doi:10.2172/573154.
Cullen, C. Measurements of the effects of humidity on radio-aerosol penetration through ultrafine capillaries. United States. doi:10.2172/573154.
Cullen, C. Thu . "Measurements of the effects of humidity on radio-aerosol penetration through ultrafine capillaries". United States. doi:10.2172/573154. https://www.osti.gov/servlets/purl/573154.
@article{osti_573154,
title = {Measurements of the effects of humidity on radio-aerosol penetration through ultrafine capillaries},
author = {Cullen, C.},
abstractNote = {The purpose of this research was to examine the effects of humidity on radio-aerosol penetration through ultrafine capillaries. A number of tests were conducted at relative humidities of 20%, 50%, and 80%, with sampling times of 20, 40, and 60 min. The radio-aerosol consisted of polystyrene particles with a diameter of 0.1 {micro}m. The ultrafine capillaries had a diameter of 250 {micro}m. The data from these tests varied significantly. These results made the identification of radio-aerosol penetration trends inconclusive. The standard deviation for all penetration data ranged from 3% to 30%. The results of this study suggest that a better control of the experimental parameters was needed to obtain more accurate data from experiments associated with radio-aerosol penetration in the presence of moisture. The experimental parameters that may have contributed to the wide variance of data, include aerosol flow, radio-aerosol generation, capillary characteristics, humidity control, and radiation measurements. It was the uncertainty of these parameters that contributed to the poor data which made conclusive deductions about radio-aerosol penetration dependence on humidity difficult. The application of this study is to ultrafine leaks resulting from stress fractures in high-level nuclear waste transportation casks under accident scenarios.},
doi = {10.2172/573154},
journal = {},
number = ,
volume = ,
place = {United States},
year = {Thu Aug 01 00:00:00 EDT 1996},
month = {Thu Aug 01 00:00:00 EDT 1996}
}

Technical Report:

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  • In this report, models are presented for calculating aerosol particle penetration through straight tubes of arbitrary orientation, inlets, and elbows. An expression to calculate effective depositional velocities of particles on tube walls is derived. The concept of maximum penetration'' is introduced, which is the maximum possible penetration through a sampling line connecting any two points in a three-dimensional space. A procedure to predict optimum tube diameter for an existing transport line is developed. An interactive menu driven software entitled DEPOSITION has been developed to perform above said tasks. This code can either be used on a PC or on amore » mainframe. The use and illustration of the software is described in Appendix A of this report.« less
  • User-friendly software (DEPOSITION 2.0) has been developed which permits characterization of aerosol particle losses in transport systems. Tho sub-models which comprise the DEPOSITION code are presented and the limitations of these sub-models are noted. These sub-models have all been previously published in the peer-reviewed literature. The software can be used to determine the penetration aerosol through existing transport systems; it will provide the optimal tube diameter for a transport system operated at a given flow rate and at a given particle size; it will provide a value for the maximum penetration for a transport system that would connect two pointsmore » in three-dimensional space; and it will provide tables of data and create output files for parametric studies on the effects of varying particle size, flow rate and tube diameter. Use of this software for specific examples is given herewith in an Appendix. Reference to this software is included in NRC Regulatory Guide 8.25 (1992) where it is considered to be an acceptable method for calculating the penetration of particles through sampling systems.« less
  • A numerical model is developed to predict particle deposition in aerosol sampling lines due to turbulent diffusion and gravitational settling. Input parameters to the model are particle diameter, air flow rate, tube length, and the inside tube diameter--the latter will be referred to as tube diameter for brevity. The flow rate of air in the sampling lines at WIPP site is in the range of 1--2.5 cfm. Additionally, models developed by others are set up for determining for penetration of aerosol through tube bends and the aspiration of air into the transport tubes. In general, the results of the calculationsmore » show aerosol transmission to the CAM samplers to be most significantly impacted by inlet operational characteristics and by the presence of horizontal tube runs and tube bends. 6 refs., 30 figs., 3 tabs.« less
  • In this report, models are presented for calculating aerosol particle penetration through straight tubes of arbitrary orientation, inlets, and elbows. An expression to calculate effective depositional velocities of particles on tube walls is derived. The concept of ``maximum penetration`` is introduced, which is the maximum possible penetration through a sampling line connecting any two points in a three-dimensional space. A procedure to predict optimum tube diameter for an existing transport line is developed. An interactive menu driven software entitled DEPOSITION has been developed to perform above said tasks. This code can either be used on a PC or on amore » mainframe. The use and illustration of the software is described in Appendix A of this report.« less
  • User-friendly software (DEPOSITION 2.0) has been developed which permits characterization of aerosol particle losses in transport systems. Tho sub-models which comprise the DEPOSITION code are presented and the limitations of these sub-models are noted. These sub-models have all been previously published in the peer-reviewed literature. The software can be used to determine the penetration aerosol through existing transport systems; it will provide the optimal tube diameter for a transport system operated at a given flow rate and at a given particle size; it will provide a value for the maximum penetration for a transport system that would connect two pointsmore » in three-dimensional space; and it will provide tables of data and create output files for parametric studies on the effects of varying particle size, flow rate and tube diameter. Use of this software for specific examples is given herewith in an Appendix. Reference to this software is included in NRC Regulatory Guide 8.25 (1992) where it is considered to be an acceptable method for calculating the penetration of particles through sampling systems.« less