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Title: Tagging in-stack suspended particles from a coal-fired power plant with an enriched isotopic tracer

Journal Article · · Aerosol Science and Technology; (United States)
; ;  [1]
  1. Univ. of Maryland, College Park (United States)

A device was constructed for tagging coal fly-ash particles with enriched isotopes of Nd for use in atmospheric tracer experiments by thermally degrading vapor of the 2,2,6,6-tetramethyl 3,5-heptanedione chelate of the metal in the presence of fly-ash laden flue gas. Microanalysis measurements of individual fly-ash particles verify the surface residence of the tracer material and show that particle surfaces are devoid of individual Nd particles. The prototype device was used to release {sup 148}Nd- and {sup 145}Nd-tagged fly-ash particles for an urban-scale field test at isotope delivery rates of 25-54 mg/h.

OSTI ID:
5686388
Journal Information:
Aerosol Science and Technology; (United States), Vol. 15:3; ISSN 0278-6826
Country of Publication:
United States
Language:
English