Uncovering Transport Mechanisms in Perovskite Materials and Devices with Recombination-Induced Action Spectroscopies

McNamee, Meredith G.; Ouyang, Zhenyu; Yan, Liang; Gan, Zijian; Zhou, Ninghao; Williams, Olivia F.; You, Wei; Moran, Andrew M.

doi:10.1021/acs.jpcc.2c08851

Uncovering Transport Mechanisms in Perovskite Materials and Devices with Recombination-Induced Action Spectroscopies

Journal Article · 01 February 2023 · Journal of Physical Chemistry. C

DOI:https://doi.org/10.1021/acs.jpcc.2c08851· OSTI ID:2424982

^[1]; ^[1]; ^[1]; ^[1]; ^[2]; ^[3]; ^[1]; ^[1]

Department of Chemistry, University of North Carolina at Chapel Hill, Chapel Hill, North Carolina 27599, United States
Shanghai Huawei Technologies Co., Ltd., No. 2222, Xinjinqiao Road, China Pilot Free Trade Zone, Shanghai 200120, China
Edmund Optics, Inc., Barrington, New Jersey 08007, United States

Not provided.

Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Center for Hybrid Organic-Inorganic Semiconductors for Energy (CHOISE)

Sponsoring Organization:: USDOE

OSTI ID:: 2424982

Journal Information:: Journal of Physical Chemistry. C, Journal Name: Journal of Physical Chemistry. C Journal Issue: 6 Vol. 127; ISSN 1932-7447

Publisher:: American Chemical Society

Country of Publication:: United States

Language:: English

References (59)

Observation of Internal Photoinduced Electron and Hole Separation in Hybrid Two-Dimentional Perovskite Films Liu, Junxue; Leng, Jing; Wu, Kaifeng Journal of the American Chemical Society, Vol. 139, Issue 4 https://doi.org/10.1021/jacs.6b12581	journal	January 2017
Origin of layered perovskite device efficiencies revealed by multidimensional time-of-flight spectroscopy Ouyang, Zhenyu; Zhou, Ninghao; McNamee, Meredith G. The Journal of Chemical Physics, Vol. 156, Issue 8 https://doi.org/10.1063/5.0072976	journal	February 2022
Distinguishing Energy- and Charge-Transfer Processes in Layered Perovskite Quantum Wells with Two-Dimensional Action Spectroscopies Zhou, Ninghao; Ouyang, Zhenyu; Hu, Jun The Journal of Physical Chemistry Letters, Vol. 11, Issue 12 https://doi.org/10.1021/acs.jpclett.0c00844	journal	May 2020
Ultrafast decoherence dynamics govern photocarrier generation efficiencies in polymer solar cells Vella, Eleonora; Li, Hao; Grégoire, Pascal Scientific Reports, Vol. 6, Issue 1 https://doi.org/10.1038/srep29437	journal	July 2016
T WO -D IMENSIONAL F EMTOSECOND S PECTROSCOPY Jonas, David M. Annual Review of Physical Chemistry, Vol. 54, Issue 1 https://doi.org/10.1146/annurev.physchem.54.011002.103907	journal	October 2003
Role of microstructure in the electron–hole interaction of hybrid lead halide perovskites Grancini, Giulia; Srimath Kandada, Ajay Ram; Frost, Jarvist M. Nature Photonics, Vol. 9, Issue 10 https://doi.org/10.1038/nphoton.2015.151	journal	August 2015
Phase-modulated rapid-scanning fluorescence-detected two-dimensional electronic spectroscopy Agathangelou, Damianos; Javed, Ariba; Sessa, Francesco The Journal of Chemical Physics, Vol. 155, Issue 9 https://doi.org/10.1063/5.0057649	journal	September 2021
General Post-annealing Method Enables High-Efficiency Two-Dimensional Perovskite Solar Cells Yan, Liang; Hu, Jun; Guo, Zhenkun ACS Applied Materials & Interfaces, Vol. 10, Issue 39 https://doi.org/10.1021/acsami.8b10230	journal	September 2018
Coherent two-dimensional photocurrent spectroscopy in a PbS quantum dot photocell Karki, Khadga J.; Widom, Julia R.; Seibt, Joachim Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms6869	journal	December 2014
Multidimensional coherent photocurrent spectroscopy of a semiconductor nanostructure Nardin, Gaël; Autry, Travis M.; Silverman, Kevin L. Optics Express, Vol. 21, Issue 23 https://doi.org/10.1364/OE.21.028617	journal	January 2013
Two-dimensional action spectroscopy of excitonic systems: Explicit simulation using a phase-modulation technique Damtie, Fikeraddis A.; Wacker, Andreas; Pullerits, Tõnu Physical Review A, Vol. 96, Issue 5 https://doi.org/10.1103/PhysRevA.96.053830	journal	November 2017
Efficient Energy Funneling in Quasi‐2D Perovskites: From Light Emission to Lasing Lei, Lei; Seyitliyev, Dovletgeldi; Stuard, Samuel Advanced Materials, Vol. 32, Issue 16 https://doi.org/10.1002/adma.201906571	journal	February 2020
Fourier Transform Fluorescence-Encoded Infrared Spectroscopy Mastron, Joseph N.; Tokmakoff, Andrei The Journal of Physical Chemistry A, Vol. 122, Issue 2 https://doi.org/10.1021/acs.jpca.7b10305	journal	January 2018
The Role of Driving Energy and Delocalized States for Charge Separation in Organic Semiconductors Bakulin, A. A.; Rao, A.; Pavelyev, V. G. Science, Vol. 335, Issue 6074 https://doi.org/10.1126/science.1217745	journal	February 2012
Scaling law for excitons in 2D perovskite quantum wells Blancon, J. -C.; Stier, A. V.; Tsai, H. Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-04659-x	journal	June 2018
Femtosecond Phase-Coherent Two-Dimensional Spectroscopy Tian, Peifang; Keusters, Dorine; Suzaki, Yoshifumi Science, Vol. 300, Issue 5625, p. 1553-1555 https://doi.org/10.1126/science.1083433	journal	June 2003
Ultrafast Spectroscopy with Photocurrent Detection: Watching Excitonic Optoelectronic Systems at Work Bakulin, Artem A.; Silva, Carlos; Vella, Eleonora The Journal of Physical Chemistry Letters, Vol. 7, Issue 2 https://doi.org/10.1021/acs.jpclett.5b01955	journal	January 2016
Discerning between Exciton and Free-Carrier Behaviors in Ruddlesden–Popper Perovskite Quantum Wells through Kinetic Modeling of Photoluminescence Dynamics Spitha, Natalia; Kohler, Daniel D.; Hautzinger, Matthew P. The Journal of Physical Chemistry C, Vol. 124, Issue 31 https://doi.org/10.1021/acs.jpcc.0c06345	journal	July 2020
Photocurrent-Detected 2D Electronic Spectroscopy Reveals Ultrafast Hole Transfer in Operating PM6/Y6 Organic Solar Cells Bolzonello, Luca; Bernal-Texca, Francisco; Gerling, Luis G. The Journal of Physical Chemistry Letters, Vol. 12, Issue 16 https://doi.org/10.1021/acs.jpclett.1c00822	journal	April 2021
Imaging Carrier Diffusion in Perovskites with a Diffractive Optic-Based Transient Absorption Microscope Guo, Zhenkun; Zhou, Ninghao; Williams, Olivia F. The Journal of Physical Chemistry C, Vol. 122, Issue 19 https://doi.org/10.1021/acs.jpcc.8b03643	journal	April 2018
Femtosecond photovoltage excitation cross-correlation on a ladder-type polymer Lanzani, G.; Zenz, C.; Cerullo, G. Synthetic Metals, Vol. 111-112 https://doi.org/10.1016/S0379-6779(99)00426-9	journal	June 2000
Long-range exciton transport and slow annihilation in two-dimensional hybrid perovskites Deng, Shibin; Shi, Enzheng; Yuan, Long Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-14403-z	journal	January 2020
Elucidation of Quantum-Well-Specific Carrier Mobilities in Layered Perovskites Zhou, Ninghao; Ouyang, Zhenyu; Yan, Liang The Journal of Physical Chemistry Letters, Vol. 12, Issue 4 https://doi.org/10.1021/acs.jpclett.0c03596	journal	January 2021
2D Homologous Perovskites as Light-Absorbing Materials for Solar Cell Applications Cao, Duyen H.; Stoumpos, Constantinos C.; Farha, Omar K. Journal of the American Chemical Society, Vol. 137, Issue 24 https://doi.org/10.1021/jacs.5b03796	journal	June 2015
Using fluorescence detected two-dimensional spectroscopy to investigate initial exciton delocalization between coupled chromophores Schröter, Marco; Pullerits, Tõnu; Kühn, Oliver The Journal of Chemical Physics, Vol. 149, Issue 11 https://doi.org/10.1063/1.5046645	journal	September 2018
Spectrally Resolved Ultrafast Exciton Transfer in Mixed Perovskite Quantum Wells Proppe, Andrew H.; Elkins, Madeline H.; Voznyy, Oleksandr The Journal of Physical Chemistry Letters, Vol. 10, Issue 3 https://doi.org/10.1021/acs.jpclett.9b00018	journal	January 2019
Inter-phase charge and energy transfer in Ruddlesden–Popper 2D perovskites: critical role of the spacing cations Zheng, Kaibo; Chen, Yani; Sun, Yong Journal of Materials Chemistry A, Vol. 6, Issue 15 https://doi.org/10.1039/C8TA01518J	journal	January 2018
Excitons in 2D Organic–Inorganic Halide Perovskites Mauck, Catherine M.; Tisdale, William A. Trends in Chemistry, Vol. 1, Issue 4 https://doi.org/10.1016/j.trechm.2019.04.003	journal	July 2019
Two-dimensional spectroscopy of electronic couplings in photosynthesis Brixner, Tobias; Stenger, Jens; Vaswani, Harsha M. Nature, Vol. 434, Issue 7033 https://doi.org/10.1038/nature03429	journal	March 2005
Temperature-dependent local conformations and conformational distributions of cyanine dimer labeled single-stranded–double-stranded DNA junctions by 2D fluorescence spectroscopy Heussman, Dylan; Kittell, Justin; von Hippel, Peter H. The Journal of Chemical Physics, Vol. 156, Issue 4 https://doi.org/10.1063/5.0076261	journal	January 2022
Band filling with free charge carriers in organometal halide perovskites Manser, Joseph S.; Kamat, Prashant V. Nature Photonics, Vol. 8, Issue 9 https://doi.org/10.1038/nphoton.2014.171	journal	August 2014
Electron-hole diffusion lengths > 175 μm in solution-grown CH ₃ NH ₃ PbI ₃ single crystals Dong, Qingfeng; Fang, Yanjun; Shao, Yuchuan Science, Vol. 347, Issue 6225 https://doi.org/10.1126/science.aaa5760	journal	January 2015
Distance Dependence of Förster Resonance Energy Transfer Rates in 2D Perovskite Quantum Wells via Control of Organic Spacer Length Panuganti, Shobhana; Besteiro, Lucas V.; Vasileiadou, Eugenia S. Journal of the American Chemical Society, Vol. 143, Issue 11 https://doi.org/10.1021/jacs.0c12441	journal	March 2021
Multidimensional time-of-flight spectroscopy Ouyang, Zhenyu; Zhou, Ninghao; McNamee, Meredith G. The Journal of Chemical Physics, Vol. 154, Issue 22 https://doi.org/10.1063/5.0047382	journal	June 2021
Fifth-order two-dimensional Raman spectra of CS2 are dominated by third-order cascades Blank, David A.; Kaufman, Laura J.; Fleming, Graham R. The Journal of Chemical Physics, Vol. 111, Issue 7 https://doi.org/10.1063/1.479591	journal	August 1999
Ruddlesden–Popper Hybrid Lead Iodide Perovskite 2D Homologous Semiconductors Stoumpos, Constantinos C.; Cao, Duyen H.; Clark, Daniel J. Chemistry of Materials, Vol. 28, Issue 8, p. 2852-2867 https://doi.org/10.1021/acs.chemmater.6b00847	journal	April 2016
Probing drift velocity dispersion in MAPbI3 photovoltaic cells with nonlinear photocurrent spectroscopy Ouyang, Zhenyu; Yan, Liang; You, Wei The Journal of Chemical Physics, Vol. 157, Issue 17 https://doi.org/10.1063/5.0116789	journal	November 2022
Interpreting Fluorescence Detected Two-Dimensional Electronic Spectroscopy Kühn, Oliver; Mančal, Tomáš; Pullerits, Tõnu The Journal of Physical Chemistry Letters, Vol. 11, Issue 3 https://doi.org/10.1021/acs.jpclett.9b03851	journal	February 2020
Two step charge carrier generation in a ladder-type conjugated polymer Müller, J. G.; Scherf, U.; Lemmer, U. Synthetic Metals, Vol. 119, Issue 1-3 https://doi.org/10.1016/S0379-6779(00)01102-4	journal	March 2001
Spatially segregated free-carrier and exciton populations in individual lead halide perovskite grains Nah, S.; Spokoyny, B.; Stoumpos, C. Nature Photonics, Vol. 11, Issue 5 https://doi.org/10.1038/nphoton.2017.36	journal	March 2017
Fluorescence-detected two-dimensional electronic coherence spectroscopy by acousto-optic phase modulation Tekavec, Patrick F.; Lott, Geoffrey A.; Marcus, Andrew H. The Journal of Chemical Physics, Vol. 127, Issue 21 https://doi.org/10.1063/1.2800560	journal	December 2007
Perovskite energy funnels for efficient light-emitting diodes Yuan, Mingjian; Quan, Li Na; Comin, Riccardo Nature Nanotechnology, Vol. 11, Issue 10 https://doi.org/10.1038/nnano.2016.110	journal	June 2016
Before Förster. Initial excitation in photosynthetic light harvesting Karki, Khadga J.; Chen, Junsheng; Sakurai, Atsunori Chemical Science, Vol. 10, Issue 34 https://doi.org/10.1039/C9SC01888C	journal	January 2019
Fifth-order two-dimensional Raman spectroscopy: A new direct probe of the liquid state Kubarych, Kevin J.; Milne, Chris J.; Miller, R. J. Dwayne International Reviews in Physical Chemistry, Vol. 22, Issue 3 https://doi.org/10.1080/0144235031000121544	journal	July 2003
Imaging Excited State Dynamics in Layered 2D Perovskites with Transient Absorption Microscopy Williams, Olivia F.; Zhou, Ninghao; Hu, Jun The Journal of Physical Chemistry A, Vol. 123, Issue 51 https://doi.org/10.1021/acs.jpca.9b08852	journal	November 2019
Chapter 5 Multidimensional Electronic and Vibrational Spectroscopy Ogilvie, Jennifer P.; Kubarych, Kevin J. Advances In Atomic, Molecular, and Optical Physics https://doi.org/10.1016/S1049-250X(09)57005-X	book	January 2009
Spatially-resolved fluorescence-detected two-dimensional electronic spectroscopy probes varying excitonic structure in photosynthetic bacteria Tiwari, Vivek; Matutes, Yassel Acosta; Gardiner, Alastair T. Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-06619-x	journal	October 2018
Strongly coupled bacteriochlorin dyad studied using phase-modulated fluorescence-detected two-dimensional electronic spectroscopy Tiwari, Vivek; Matutes, Yassel Acosta; Konar, Arkaprabha Optics Express, Vol. 26, Issue 17 https://doi.org/10.1364/OE.26.022327	journal	January 2018
Molecular Coherent Three-Quantum Two-Dimensional Fluorescence Spectroscopy Mueller, Stefan; Brixner, Tobias The Journal of Physical Chemistry Letters, Vol. 11, Issue 13 https://doi.org/10.1021/acs.jpclett.0c00987	journal	June 2020
Signatures of exciton dynamics and interaction in coherently and fluorescence-detected four- and six-wave-mixing two-dimensional electronic spectroscopy Malý, Pavel; Mueller, Stefan; Lüttig, Julian The Journal of Chemical Physics, Vol. 153, Issue 14 https://doi.org/10.1063/5.0022743	journal	October 2020
Ultrafast Exciton Transport with a Long Diffusion Length in Layered Perovskites with Organic Cation Functionalization Xiao, Xun; Wu, Marvin; Ni, Zhenyi Advanced Materials, Vol. 32, Issue 46 https://doi.org/10.1002/adma.202004080	journal	October 2020
Charge-Carrier Dynamics in Organic-Inorganic Metal Halide Perovskites Herz, Laura M. Annual Review of Physical Chemistry, Vol. 67, Issue 1 https://doi.org/10.1146/annurev-physchem-040215-112222	journal	May 2016
Simulating Fluorescence-Detected Two-Dimensional Electronic Spectroscopy of Multichromophoric Systems Kunsel, Tenzin; Tiwari, Vivek; Matutes, Yassel Acosta The Journal of Physical Chemistry B, Vol. 123, Issue 2 https://doi.org/10.1021/acs.jpcb.8b10176	journal	December 2018
Incoherent population mixing contributions to phase-modulation two-dimensional coherent excitation spectra Grégoire, Pascal; Srimath Kandada, Ajay Ram; Vella, Eleonora The Journal of Chemical Physics, Vol. 147, Issue 11 https://doi.org/10.1063/1.4994987	journal	September 2017
Nonlinear fluorescence spectroscopy of layered perovskite quantum wells Ouyang, Zhenyu; Zhou, Ninghao; Hu, Jun The Journal of Chemical Physics, Vol. 153, Issue 13 https://doi.org/10.1063/5.0021759	journal	October 2020
Energy transfer mechanisms in layered 2D perovskites Williams, Olivia F.; Guo, Zhenkun; Hu, Jun The Journal of Chemical Physics, Vol. 148, Issue 13 https://doi.org/10.1063/1.5009663	journal	April 2018
Identifying incoherent mixing effects in the coherent two-dimensional photocurrent excitation spectra of semiconductors Bargigia, Ilaria; Gutiérrez-Meza, Elizabeth; Valverde-Chávez, David A. The Journal of Chemical Physics, Vol. 157, Issue 20 https://doi.org/10.1063/5.0121635	journal	November 2022
Differentiation of True Nonlinear and Incoherent Mixing of Linear Signals in Action-Detected 2D Spectroscopy Kalaee, Alex Arash Sand; Damtie, Fikeraddis; Karki, Khadga Jung The Journal of Physical Chemistry A, Vol. 123, Issue 19 https://doi.org/10.1021/acs.jpca.9b01129	journal	April 2019
Extremely efficient internal exciton dissociation through edge states in layered 2D perovskites Blancon, J. -C.; Tsai, H.; Nie, W. Science, Vol. 355, Issue 6331 https://doi.org/10.1126/science.aal4211	journal	March 2017

Similar Records

Screening Links Transport and Recombination Mechanisms in Lead Halide Perovskites

Journal Article · 2019 · Journal of Physical Chemistry. C · OSTI ID:1612088

Charge exchange recombination spectroscopy on fusion devices

Journal Article · 2012 · AIP Conference Proceedings · OSTI ID:22004066

ON THE MECHANISM OF ULTRAVIOLET-LIGHT ACTION ON ESCHERICHIA COLI RECOMBINATION.

Journal Article · 1967 · Acta Microbiol. Pol., 17: 337-40(1968). · OSTI ID:4785257

Related Subjects

Chemistry
Materials Science
Science & Technology - Other Topics

Uncovering Transport Mechanisms in Perovskite Materials and Devices with Recombination-Induced Action Spectroscopies

Citation Formats

References (59)

Similar Records

Related Subjects