Direct Visualization of Subnanometer Variations in the Excitonic Spectra of 2D/3D Semiconductor/Metal Heterostructures

Reidy, Kate; Majchrzak, Paulina Ewa; Haas, Benedikt; Thomsen, Joachim Dahl; Konečná, Andrea; Park, Eugene; Klein, Julian; Jones, Alfred J.  H.; Volckaert, Klara; Biswas, Deepnarayan; Watson, Matthew D.; Cacho, Cephise; Narang, Prineha; Koch, Christoph T.; Ulstrup, Søren; Ross, Frances M.; Idrobo, Juan Carlos

doi:10.1021/acs.nanolett.2c04749

Direct Visualization of Subnanometer Variations in the Excitonic Spectra of 2D/3D Semiconductor/Metal Heterostructures

Journal Article · 12 January 2023 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.2c04749· OSTI ID:2423985

^[1]; ^[2]; Haas, Benedikt ^[3]; Thomsen, Joachim Dahl ^[1]; ^[4]; Park, Eugene ^[1]; ^[1]; Jones, Alfred J. H. ^[2]; Volckaert, Klara ^[2]; Biswas, Deepnarayan ^[2]; Watson, Matthew D. ^[5]; Cacho, Cephise ^[5]; ^[6]; ^[3]; ^[2]; ^[1]; ^[7]

Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States
Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark
Department of Physics & IRIS Adlershof, Humboldt-Universität zu Berlin, 12489 Berlin, Germany
Central European Institute of Technology, Brno University of Technology, 61200 Brno, Czech Republic
Diamond Light Source, Harwell Campus, Didcot OX11 0DE, United Kingdom
College of Letters and Science, Physical Sciences, UCLA, Los Angeles, California 90095, United States
Materials Science and Engineering Department, University of Washington, Seattle, Washington 98195, United States

Not provided.

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)

Sponsoring Organization:: USDOE

DOE Contract Number:: AC05-00OR22725

OSTI ID:: 2423985

Journal Information:: Nano Letters, Journal Name: Nano Letters Journal Issue: 3 Vol. 23; ISSN 1530-6984

Publisher:: American Chemical Society

Country of Publication:: United States

Language:: English

References (48)

Coulomb engineering of the bandgap and excitons in two-dimensional materials Raja, Archana; Chaves, Andrey; Yu, Jaeeun Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms15251	journal	May 2017
Electronic Structure and Luminescence of Quasi-Freestanding MoS ₂ Nanopatches on Au(111) Krane, Nils; Lotze, Christian; Läger, Julia M. Nano Letters, Vol. 16, Issue 8 https://doi.org/10.1021/acs.nanolett.6b02101	journal	July 2016
Excitonic Linewidth Approaching the Homogeneous Limit in MoS 2 -Based van der Waals Heterostructures Cadiz, F.; Courtade, E.; Robert, C. Physical Review X, Vol. 7, Issue 2 https://doi.org/10.1103/PhysRevX.7.021026	journal	May 2017
Mechanisms of Quasi van der Waals Epitaxy of Three-Dimensional Metallic Nanoislands on Suspended Two-Dimensional Materials Reidy, Kate; Thomsen, Joachim Dahl; Lee, Hae Yeon Nano Letters, Vol. 22, Issue 14 https://doi.org/10.1021/acs.nanolett.2c01682	journal	July 2022
Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS 2 Chernikov, Alexey; Berkelbach, Timothy C.; Hill, Heather M. Physical Review Letters, Vol. 113, Issue 7 https://doi.org/10.1103/PhysRevLett.113.076802	journal	August 2014
Direct exciton emission from atomically thin transition metal dichalcogenide heterostructures near the lifetime limit Wierzbowski, Jakob; Klein, Julian; Sigger, Florian Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-09739-4	journal	September 2017
Diversity of trion states and substrate effects in the optical properties of an MoS2 monolayer Drüppel, Matthias; Deilmann, Thorsten; Krüger, Peter Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/s41467-017-02286-6	journal	December 2017
Two-Dimensional Material Tunnel Barrier for Josephson Junctions and Superconducting Qubits Lee, Kan-Heng; Chakram, Srivatsan; Kim, Shi En Nano Letters, Vol. 19, Issue 11 https://doi.org/10.1021/acs.nanolett.9b03886	journal	October 2019
Electrical Tuning of Exciton–Plasmon Polariton Coupling in Monolayer MoS ₂ Integrated with Plasmonic Nanoantenna Lattice Lee, Bumsu; Liu, Wenjing; Naylor, Carl H. Nano Letters, Vol. 17, Issue 7 https://doi.org/10.1021/acs.nanolett.7b02245	journal	June 2017
Renormalization of Molecular Electronic Levels at Metal-Molecule Interfaces Neaton, J. B.; Hybertsen, Mark S.; Louie, Steven G. Physical Review Letters, Vol. 97, Issue 21 https://doi.org/10.1103/PhysRevLett.97.216405	journal	November 2006
Two-Dimensional Heterojunctions from Nonlocal Manipulations of the Interactions Rösner, M.; Steinke, C.; Lorke, M. Nano Letters, Vol. 16, Issue 4 https://doi.org/10.1021/acs.nanolett.5b05009	journal	March 2016
Hyperspectral imaging of exciton confinement within a moiré unit cell with a subnanometer electron probe Susarla, Sandhya; Naik, Mit H.; Blach, Daria D. Science, Vol. 378, Issue 6625 https://doi.org/10.1126/science.add9294	journal	December 2022
Nanoscale Modification of WS ₂ Trion Emission by Its Local Electromagnetic Environment Bonnet, Noémie; Lee, Hae Yeon; Shao, Fuhui Nano Letters, Vol. 21, Issue 24 https://doi.org/10.1021/acs.nanolett.1c02600	journal	December 2021
Gate-Tunable Semiconductor Heterojunctions from 2D/3D van der Waals Interfaces Miao, Jinshui; Liu, Xiwen; Jo, Kiyoung Nano Letters, Vol. 20, Issue 4 https://doi.org/10.1021/acs.nanolett.0c00741	journal	March 2020
Van der Waals integration before and beyond two-dimensional materials Liu, Yuan; Huang, Yu; Duan, Xiangfeng Nature, Vol. 567, Issue 7748 https://doi.org/10.1038/s41586-019-1013-x	journal	March 2019
Electronic Structure of Epitaxial Single-Layer MoS 2 Miwa, Jill A.; Ulstrup, Søren; Sørensen, Signe G. Physical Review Letters, Vol. 114, Issue 4 https://doi.org/10.1103/PhysRevLett.114.046802	journal	January 2015
Computational Study of Metal Contacts to Monolayer Transition-Metal Dichalcogenide Semiconductors Kang, Jiahao; Liu, Wei; Sarkar, Deblina Physical Review X, Vol. 4, Issue 3 https://doi.org/10.1103/PhysRevX.4.031005	journal	July 2014
Probing dark excitons in atomically thin semiconductors via near-field coupling to surface plasmon polaritons Zhou, You; Scuri, Giovanni; Wild, Dominik S. Nature Nanotechnology, Vol. 12, Issue 9 https://doi.org/10.1038/nnano.2017.106	journal	June 2017
Improved Contacts to MoS ₂ Transistors by Ultra-High Vacuum Metal Deposition English, Chris D.; Shine, Gautam; Dorgan, Vincent E. Nano Letters, Vol. 16, Issue 6 https://doi.org/10.1021/acs.nanolett.6b01309	journal	May 2016
Giant bandgap renormalization and excitonic effects in a monolayer transition metal dichalcogenide semiconductor Ugeda, Miguel M.; Bradley, Aaron J.; Shi, Su-Fei Nature Materials, Vol. 13, Issue 12 https://doi.org/10.1038/nmat4061	journal	August 2014
Exciton Mapping at Subwavelength Scales in Two-Dimensional Materials Tizei, Luiz H. G.; Lin, Yung-Chang; Mukai, Masaki Physical Review Letters, Vol. 114, Issue 10 https://doi.org/10.1103/PhysRevLett.114.107601	journal	March 2015
Strong Exciton–Plasmon Coupling in MoS ₂ Coupled with Plasmonic Lattice Liu, Wenjing; Lee, Bumsu; Naylor, Carl H. Nano Letters, Vol. 16, Issue 2 https://doi.org/10.1021/acs.nanolett.5b04588	journal	January 2016
Strong-coupling of WSe2 in ultra-compact plasmonic nanocavities at room temperature Kleemann, Marie-Elena; Chikkaraddy, Rohit; Alexeev, Evgeny M. Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/s41467-017-01398-3	journal	November 2017
Nanoassembly of quantum emitters in hexagonal boron nitride and gold nanospheres Nguyen, Minh; Kim, Sejeong; Tran, Toan Trong Nanoscale, Vol. 10, Issue 5 https://doi.org/10.1039/C7NR08249E	journal	January 2018
Visualizing Spatial Variations of Plasmon–Exciton Polaritons at the Nanoscale Using Electron Microscopy Yankovich, Andrew B.; Munkhbat, Battulga; Baranov, Denis G. Nano Letters, Vol. 19, Issue 11 https://doi.org/10.1021/acs.nanolett.9b03534	journal	September 2019
The Dielectric Impact of Layer Distances on Exciton and Trion Binding Energies in van der Waals Heterostructures Florian, Matthias; Hartmann, Malte; Steinhoff, Alexander Nano Letters, Vol. 18, Issue 4 https://doi.org/10.1021/acs.nanolett.8b00840	journal	March 2018
Low-temperature photocarrier dynamics in monolayer MoS ₂ Korn, T.; Heydrich, S.; Hirmer, M. Applied Physics Letters, Vol. 99, Issue 10 https://doi.org/10.1063/1.3636402	journal	September 2011
2D materials for spintronic devices Ahn, Ethan C. npj 2D Materials and Applications, Vol. 4, Issue 1 https://doi.org/10.1038/s41699-020-0152-0	journal	June 2020
Smart Align—a new tool for robust non-rigid registration of scanning microscope data Jones, Lewys; Yang, Hao; Pennycook, Timothy J. Advanced Structural and Chemical Imaging, Vol. 1, Issue 1 https://doi.org/10.1186/s40679-015-0008-4	journal	July 2015
Mapping Modified Electronic Levels in the Moiré Patterns in MoS₂/WSe₂ Using Low-Loss EELS Susarla, Sandhya; M. Sassi, Lucas; Zobelli, Alberto Nano Letters, Vol. 21, Issue 9 https://doi.org/10.1021/acs.nanolett.1c00984	journal	April 2021
Image charge effect on two-dimensional excitons in an inorganic-organic quantum-well crystal Tanaka, Kenichiro; Takahashi, Takayuki; Kondo, Takashi Physical Review B, Vol. 71, Issue 4 https://doi.org/10.1103/PhysRevB.71.045312	journal	January 2005
Electrical contacts to two-dimensional semiconductors Allain, Adrien; Kang, Jiahao; Banerjee, Kaustav Nature Materials, Vol. 14, Issue 12 https://doi.org/10.1038/nmat4452	journal	November 2015
Coulomb interaction in monolayer transition-metal dichalcogenides Van Tuan, Dinh; Yang, Min; Dery, Hanan Physical Review B, Vol. 98, Issue 12 https://doi.org/10.1103/PhysRevB.98.125308	journal	September 2018
Heterojunction tunnel triodes based on two-dimensional metal selenide and three-dimensional silicon Miao, Jinshui; Leblanc, Chloe; Wang, Jinjin Nature Electronics, Vol. 5, Issue 11 https://doi.org/10.1038/s41928-022-00849-0	journal	October 2022
Electronic Tuning in WSe₂/Au via van der Waals Interface Twisting and Intercalation Wu, Qilong; Bagheri Tagani, Meysam; Zhang, Lijie ACS Nano, Vol. 16, Issue 4 https://doi.org/10.1021/acsnano.2c00916	journal	March 2022
Substrate influence on transition metal dichalcogenide monolayer exciton absorption linewidth broadening Shao, Fuhui; Woo, Steffi Y.; Wu, Nianjheng Physical Review Materials, Vol. 6, Issue 7 https://doi.org/10.1103/PhysRevMaterials.6.074005	journal	July 2022
microARPES and nanoARPES at diffraction-limited light sources: opportunities and performance gains Rotenberg, Eli; Bostwick, Aaron Journal of Synchrotron Radiation, Vol. 21, Issue 5 https://doi.org/10.1107/S1600577514015409	journal	August 2014
Redshift of Excitons in Carbon Nanotubes Caused by the Environment Polarizability Rohlfing, Michael Physical Review Letters, Vol. 108, Issue 8 https://doi.org/10.1103/PhysRevLett.108.087402	journal	February 2012
Plasmonic Pumping of Excitonic Photoluminescence in Hybrid MoS ₂ –Au Nanostructures Najmaei, Sina; Mlayah, Adnen; Arbouet, Arnaud ACS Nano, Vol. 8, Issue 12 https://doi.org/10.1021/nn5056942	journal	November 2014
Single-layer MoS 2 on Au(111): Band gap renormalization and substrate interaction Bruix, Albert; Miwa, Jill A.; Hauptmann, Nadine Physical Review B, Vol. 93, Issue 16 https://doi.org/10.1103/PhysRevB.93.165422	journal	April 2016
Mixed-dimensional van der Waals heterostructures Jariwala, Deep; Marks, Tobin J.; Hersam, Mark C. Nature Materials, Vol. 16, Issue 2 https://doi.org/10.1038/nmat4703	journal	August 2016
Direct imaging and electronic structure modulation of moiré superlattices at the 2D/3D interface Reidy, Kate; Varnavides, Georgios; Thomsen, Joachim Dahl Nature Communications, Vol. 12, Issue 1 https://doi.org/10.1038/s41467-021-21363-5	journal	February 2021
Integration of bulk materials with two-dimensional materials for physical coupling and applications Bae, Sang-Hoon; Kum, Hyun; Kong, Wei Nature Materials, Vol. 18, Issue 6 https://doi.org/10.1038/s41563-019-0335-2	journal	May 2019
Optospintronics in Graphene via Proximity Coupling Avsar, Ahmet; Unuchek, Dmitrii; Liu, Jiawei ACS Nano, Vol. 11, Issue 11 https://doi.org/10.1021/acsnano.7b06800	journal	September 2017
Visualizing electrostatic gating effects in two-dimensional heterostructures Nguyen, Paul V.; Teutsch, Natalie C.; Wilson, Nathan P. Nature, Vol. 572, Issue 7768 https://doi.org/10.1038/s41586-019-1402-1	journal	July 2019
Deterministic Coupling of Quantum Emitters in 2D Materials to Plasmonic Nanocavity Arrays Tran, Toan Trong; Wang, Danqing; Xu, Zai-Quan Nano Letters, Vol. 17, Issue 4 https://doi.org/10.1021/acs.nanolett.7b00444	journal	March 2017
Uncovering the Effects of Metal Contacts on Monolayer MoS ₂ Schauble, Kirstin; Zakhidov, Dante; Yalon, Eilam ACS Nano, Vol. 14, Issue 11 https://doi.org/10.1021/acsnano.0c03515	journal	September 2020
Catalytically mediated epitaxy of 3D semiconductors on van der Waals substrates Periwal, Priyanka; Thomsen, Joachim Dahl; Reidy, Kate Applied Physics Reviews, Vol. 7, Issue 3 https://doi.org/10.1063/5.0006300	journal	September 2020

Similar Records

Valley-polarized exciton dynamics in a 2D semiconductor heterostructure

Journal Article · 2016 · Science · OSTI ID:1355832

Direct Optoelectronic Imaging of 2D Semiconductor–3D Metal Buried Interfaces

Journal Article · 2021 · ACS Nano · OSTI ID:1785940

Establishing charge-transfer excitons in 2D perovskite heterostructures

Journal Article · 2020 · Nature Communications · OSTI ID:1816873

Related Subjects

Chemistry
Materials Science
Physics
Science & Technology - Other Topics

Direct Visualization of Subnanometer Variations in the Excitonic Spectra of 2D/3D Semiconductor/Metal Heterostructures

Citation Formats

References (48)

Similar Records

Related Subjects