CdS/CdSe/CdS Spherical Quantum Wells with Near-Unity Biexciton Quantum Yield for Light-Emitting-Device Applications

Marder, Andrew A.; Cassidy, James; Harankahage, Dulanjan; Beavon, Jacob; Gutiérrez-Arzaluz, Luis; Mohammed, Omar F.; Mishra, Aditya; Adams, Austen C.; Slinker, Jason. D.; Hu, Zhongjian; Savoy, Stephen; Zamkov, Mikhail; Malko, Anton V.

doi:10.1021/acsmaterialslett.3c00110

CdS/CdSe/CdS Spherical Quantum Wells with Near-Unity Biexciton Quantum Yield for Light-Emitting-Device Applications

Journal Article · 10 April 2023 · ACS Materials Letters

DOI:https://doi.org/10.1021/acsmaterialslett.3c00110· OSTI ID:2420078

^[1]; Cassidy, James ^[2]; Harankahage, Dulanjan ^[2]; Beavon, Jacob ^[2]; ^[3]; ^[3]; Mishra, Aditya ^[4]; Adams, Austen C. ^[5]; ^[6]; Hu, Zhongjian ^[7]; Savoy, Stephen ^[7]; ^[2]; ^[5]

Department of Physics, The University of Texas at Dallas, Richardson, Texas 75080, United States; OSTI
The Center for Photochemical Sciences and Department of Physics, Bowling Green State University, Bowling Green, Ohio 43403, United States
Advanced Membranes and Porous Materials Center and KAUST Catalysis Center, Division of Physical Sciences and Engineering, King Abdullah University of Science and Technology, Thuwal 23955-6900, Kingdom of Saudi Arabia
Department of Materials Science and Engineering, The University of Texas at Dallas, Richardson, Texas 75080, United States
Department of Physics, The University of Texas at Dallas, Richardson, Texas 75080, United States
Department of Physics, The University of Texas at Dallas, Richardson, Texas 75080, United States; Department of Materials Science and Engineering, The University of Texas at Dallas, Richardson, Texas 75080, United States
Nanohmics Inc., 6201 E. Oltorf, Suite 400, Austin, Texas 78741, United States

Not provided.

Research Organization:: Univ. of Texas at Dallas, Richardson, TX (United States); Bowling Green State Univ., OH (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

DOE Contract Number:: SC0010697; SC0016872

OSTI ID:: 2420078

Journal Information:: ACS Materials Letters, Journal Name: ACS Materials Letters Journal Issue: 5 Vol. 5; ISSN 2639-4979

Publisher:: ACS Publications

Country of Publication:: United States

Language:: English

References (43)

Ultrathin PbS Sheets by Two-Dimensional Oriented Attachment Schliehe, C.; Juarez, B. H.; Pelletier, M. Science, Vol. 329, Issue 5991 https://doi.org/10.1126/science.1188035	journal	July 2010
Trion Decay in Colloidal Quantum Dots Jha, Praket P.; Guyot-Sionnest, Philippe ACS Nano, Vol. 3, Issue 4 https://doi.org/10.1021/nn9001177	journal	March 2009
Size-Dependent Biexciton Quantum Yields and Carrier Dynamics of Quasi-Two-Dimensional Core/Shell Nanoplatelets Ma, Xuedan; Diroll, Benjamin T.; Cho, Wooje ACS Nano, Vol. 11, Issue 9 https://doi.org/10.1021/acsnano.7b03943	journal	September 2017
Auger relaxation processes in semiconductor nanocrystals and quantum wells Kharchenko, V. A.; Rosen, M. Journal of Luminescence, Vol. 70, Issue 1-6 https://doi.org/10.1016/0022-2313(96)00052-X	journal	October 1996
Single-photon emission from pyramidal quantum dots: The impact of hole thermalization on photon emission statistics Malko, A.; Oberli, D. Y.; Baier, M. H. Physical Review B, Vol. 72, Issue 19 https://doi.org/10.1103/PhysRevB.72.195332	journal	November 2005
Stable and Bright Electroluminescent Devices utilizing Emissive 0D Perovskite Nanocrystals Incorporated in a 3D CsPbBr₃ Matrix Mishra, Aditya; Bose, Riya; Zheng, Yangzi Advanced Materials, Vol. 34, Issue 31 https://doi.org/10.1002/adma.202203226	journal	June 2022
Colloidal Quantum Shells: An Emerging 2D Semiconductor for Energy Applications Cassidy, James; Harankahage, Dulanjan; Porotnikov, Dmitry ACS Energy Letters, Vol. 7, Issue 3 https://doi.org/10.1021/acsenergylett.2c00153	journal	March 2022
Super color purity green quantum dot light-emitting diodes fabricated by using CdSe/CdS nanoplatelets Zhang, Fengjuan; Wang, Shujie; Wang, Lei Nanoscale, Vol. 8, Issue 24 https://doi.org/10.1039/C6NR02922A	journal	January 2016
Spectral and Dynamical Properties of Multiexcitons in Semiconductor Nanocrystals Klimov, Victor I. Annual Review of Physical Chemistry, Vol. 58, Issue 1 https://doi.org/10.1146/annurev.physchem.58.032806.104537	journal	May 2007
Low-Threshold Stimulated Emission Using Colloidal Quantum Wells She, Chunxing; Fedin, Igor; Dolzhnikov, Dmitriy S. Nano Letters, Vol. 14, Issue 5 https://doi.org/10.1021/nl500775p	journal	April 2014
Picosecond energy transfer and multiexciton transfer outpaces Auger recombination in binary CdSe nanoplatelet solids Rowland, Clare E.; Fedin, Igor; Zhang, Hui Nature Materials, Vol. 14, Issue 5 https://doi.org/10.1038/nmat4231	journal	March 2015
Bright and Grey States in CdSe-CdS Nanocrystals Exhibiting Strongly Reduced Blinking Spinicelli, P.; Buil, S.; Quélin, X. Physical Review Letters, Vol. 102, Issue 13 https://doi.org/10.1103/PhysRevLett.102.136801	journal	March 2009
Challenge to the Charging Model of Semiconductor-Nanocrystal Fluorescence Intermittency from Off-State Quantum Yields and Multiexciton Blinking Zhao, Jing; Nair, Gautham; Fisher, Brent R. Physical Review Letters, Vol. 104, Issue 15 https://doi.org/10.1103/PhysRevLett.104.157403	journal	April 2010
Colloidal Two-Dimensional Systems: CdSe Quantum Shells and Wells Battaglia, David; Li, Jack J.; Wang, Yunjun Angewandte Chemie International Edition, Vol. 42, Issue 41, p. 5035-5039 https://doi.org/10.1002/anie.200352120	journal	October 2003
Colloidal Spherical Quantum Wells with Near-Unity Photoluminescence Quantum Yield and Suppressed Blinking Jeong, Byeong Guk; Park, Young-Shin; Chang, Jun Hyuk ACS Nano, Vol. 10, Issue 10 https://doi.org/10.1021/acsnano.6b03704	journal	October 2016
Sub–single-exciton lasing using charged quantum dots coupled to a distributed feedback cavity Kozlov, Oleg V.; Park, Young-Shin; Roh, Jeongkyun Science, Vol. 365, Issue 6454 https://doi.org/10.1126/science.aax3489	journal	August 2019
Optical Nonlinearities and Ultrafast Carrier Dynamics in Semiconductor Nanocrystals Klimov, Victor I. The Journal of Physical Chemistry B, Vol. 104, Issue 26 https://doi.org/10.1021/jp9944132	journal	July 2000
High-Performance Deep Red Colloidal Quantum Well Light-Emitting Diodes Enabled by the Understanding of Charge Dynamics Hu, Sujuan; Shabani, Farzan; Liu, Baiquan ACS Nano, Vol. 16, Issue 7 https://doi.org/10.1021/acsnano.2c02967	journal	July 2022
Record High External Quantum Efficiency of 19.2% Achieved in Light‐Emitting Diodes of Colloidal Quantum Wells Enabled by Hot‐Injection Shell Growth Liu, Baiquan; Altintas, Yemliha; Wang, Lin Advanced Materials, Vol. 32, Issue 8 https://doi.org/10.1002/adma.201905824	journal	December 2019
Electrolyte-Gated Field Effect Transistor to Probe the Surface Defects and Morphology in Films of Thick CdSe Colloidal Nanoplatelets Lhuillier, Emmanuel; Pedetti, Silvia; Ithurria, Sandrine ACS Nano, Vol. 8, Issue 4 https://doi.org/10.1021/nn500538n	journal	March 2014
Influence of the core size on biexciton quantum yield of giant CdSe/CdS nanocrystals Mangum, Benjamin D.; Sampat, Siddharth; Ghosh, Yagnaseni Nanoscale, Vol. 6, Issue 7 https://doi.org/10.1039/c3nr06558h	journal	January 2014
From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solids Malko, A. V.; Mikhailovsky, A. A.; Petruska, M. A. Applied Physics Letters, Vol. 81, Issue 7 https://doi.org/10.1063/1.1497708	journal	August 2002
Auger Recombination of Biexcitons and Negative and Positive Trions in Individual Quantum Dots Park, Young-Shin; Bae, Wan Ki; Pietryga, Jeffrey M. ACS Nano, Vol. 8, Issue 7 https://doi.org/10.1021/nn5023473	journal	June 2014
Continuous Distribution of Emission States from Single CdSe/ZnS Quantum Dots Zhang, Kai; Chang, Hauyee; Fu, Aihua Nano Letters, Vol. 6, Issue 4 https://doi.org/10.1021/nl060483q	journal	April 2006
Controlling the influence of Auger recombination on the performance of quantum-dot light-emitting diodes Bae, Wan Ki; Park, Young-Shin; Lim, Jaehoon Nature Communications, Vol. 4, Issue 1 https://doi.org/10.1038/ncomms3661	journal	October 2013
Near-Unity Quantum Yields of Biexciton Emission from CdSe / CdS Nanocrystals Measured Using Single-Particle Spectroscopy Park, Y. -S.; Malko, A. V.; Vela, J. Physical Review Letters, Vol. 106, Issue 18 https://doi.org/10.1103/PhysRevLett.106.187401	journal	May 2011
Quantization of Multiparticle Auger Rates in Semiconductor Quantum Dots Klimov, V. I. Science, Vol. 287, Issue 5455 https://doi.org/10.1126/science.287.5455.1011	journal	February 2000
Sub-single exciton optical gain threshold in colloidal semiconductor quantum wells with gradient alloy shelling Taghipour, Nima; Delikanli, Savas; Shendre, Sushant Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-17032-8	journal	July 2020
Electron–Hole Correlations Govern Auger Recombination in Nanostructures Philbin, John P.; Rabani, Eran Nano Letters, Vol. 18, Issue 12 https://doi.org/10.1021/acs.nanolett.8b03715	journal	November 2018
Template Synthesis of CuInS ₂ Nanocrystals from In ₂ S ₃ Nanoplates and Their Application as Counter Electrodes in Dye-Sensitized Solar Cells Chen, Bingkun; Chang, Shuai; Li, Deyao Chemistry of Materials, Vol. 27, Issue 17 https://doi.org/10.1021/acs.chemmater.5b01971	journal	August 2015
Efficient Solution-Processed Nanoplatelet-Based Light-Emitting Diodes with High Operational Stability in Air Giovanella, Umberto; Pasini, Mariacecilia; Lorenzon, Monica Nano Letters, Vol. 18, Issue 6 https://doi.org/10.1021/acs.nanolett.8b00456	journal	May 2018
Higher-Order Photon Correlation as a Tool To Study Exciton Dynamics in Quasi-2D Nanoplatelets Amgar, Daniel; Yang, Gaoling; Tenne, Ron Nano Letters, Vol. 19, Issue 12 https://doi.org/10.1021/acs.nanolett.9b03442	journal	November 2019
Suppression of Auger Processes in Confined Structures Cragg, George E.; Efros, Alexander L. Nano Letters, Vol. 10, Issue 1 https://doi.org/10.1021/nl903592h	journal	January 2010
Colloidal CdSe Quantum Wells with Graded Shell Composition for Low-Threshold Amplified Spontaneous Emission and Highly Efficient Electroluminescence Kelestemur, Yusuf; Shynkarenko, Yevhen; Anni, Marco ACS Nano, Vol. 13, Issue 12 https://doi.org/10.1021/acsnano.9b05313	journal	November 2019
Emission Intensity Dependence and Single-Exponential Behavior In Single Colloidal Quantum Dot Fluorescence Lifetimes Fisher, Brent R.; Eisler, Hans-Jürgen; Stott, Nathan E. The Journal of Physical Chemistry B, Vol. 108, Issue 1 https://doi.org/10.1021/jp035756+	journal	December 2003
Quantum Shells Boost the Optical Gain of Lasing Media Cassidy, James; Diroll, Benjamin T.; Mondal, Navendu ACS Nano, Vol. 16, Issue 2 https://doi.org/10.1021/acsnano.1c10404	journal	February 2022
Biexciton Quantum Yield of Single Semiconductor Nanocrystals from Photon Statistics Nair, Gautham; Zhao, Jing; Bawendi, Moungi G. Nano Letters, Vol. 11, Issue 3 https://doi.org/10.1021/nl104054t	journal	March 2011
Quantum Optics with Nanocrystal Quantum Dots in Solution: Quantitative Study of Clustering Bussian, David A.; Malko, Anton V.; Htoon, Han The Journal of Physical Chemistry C, Vol. 113, Issue 6 https://doi.org/10.1021/jp806219s	journal	January 2009
Emergence of Nanoplatelet Light-Emitting Diodes Xiao, Peng; Huang, Junhua; Yan, Dong Materials, Vol. 11, Issue 8 https://doi.org/10.3390/ma11081376	journal	August 2018
Giant Modal Gain Coefficients in Colloidal II–VI Nanoplatelets Guzelturk, Burak; Pelton, Matthew; Olutas, Murat Nano Letters, Vol. 19, Issue 1 https://doi.org/10.1021/acs.nanolett.8b03891	journal	December 2018
Optically pumped colloidal-quantum-dot lasing in LED-like devices with an integrated optical cavity Roh, Jeongkyun; Park, Young-Shin; Lim, Jaehoon Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-019-14014-3	journal	January 2020
Multistate Blinking and Scaling of Recombination Rates in Individual Silica-Coated CdSe/CdS Nanocrystals Sampat, Siddharth; Karan, Niladri S.; Guo, Tianle ACS Photonics, Vol. 2, Issue 10 https://doi.org/10.1021/acsphotonics.5b00423	journal	September 2015
One-Dimensional Carrier Confinement in “Giant” CdS/CdSe Excitonic Nanoshells Razgoniaeva, Natalia; Moroz, Pavel; Yang, Mingrui Journal of the American Chemical Society, Vol. 139, Issue 23 https://doi.org/10.1021/jacs.7b02054	journal	June 2017

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