Manipulating Peierls Distortion in van der Waals NbOX 2 Maximizes Second-Harmonic Generation

Fu, Tonghuan; Bu, Kejun; Sun, Xuzhou; Wang, Dong; Feng, Xin; Guo, Songhao; Sun, Zongdong; Fang, Yuqiang; Hu, Qingyang; Ding, Yang; Zhai, Tianyou; Huang, Fuqiang; Lü, Xujie

doi:10.1021/jacs.3c04971

Manipulating Peierls Distortion in van der Waals NbOX ₂ Maximizes Second-Harmonic Generation

Journal Article · 19 July 2023 · Journal of the American Chemical Society

DOI:https://doi.org/10.1021/jacs.3c04971· OSTI ID:2419439

Fu, Tonghuan ^[1]; ^[2]; Sun, Xuzhou ^[3]; ^[2]; Feng, Xin ^[4]; ^[2]; Sun, Zongdong ^[4]; Fang, Yuqiang ^[3]; ^[2]; Ding, Yang ^[2]; ^[4]; ^[3]; ^[2]

Center for High Pressure Science and Technology Advanced Research (HPSTAR), Shanghai 201203, China; OSTI
Center for High Pressure Science and Technology Advanced Research (HPSTAR), Shanghai 201203, China
State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China
State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering, Huazhong University of Science and Technology (HUST), Wuhan 430074, China

Not provided.

Research Organization:: Univ. of Chicago, IL (United States); Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

DOE Contract Number:: FG02-94ER14466; AC02-06CH11357

OSTI ID:: 2419439

Journal Information:: Journal of the American Chemical Society, Journal Name: Journal of the American Chemical Society Journal Issue: 30 Vol. 145; ISSN 0002-7863

Publisher:: American Chemical Society (ACS)

Country of Publication:: United States

Language:: English

References (31)

Data-driven discovery of high performance layered van der Waals piezoelectric NbOI2 Wu, Yaze; Abdelwahab, Ibrahim; Kwon, Ki Chang Nature Communications, Vol. 13, Issue 1 https://doi.org/10.1038/s41467-022-29495-y	journal	April 2022
Nonlinear Optics with 2D Layered Materials Autere, Anton; Jussila, Henri; Dai, Yunyun Advanced Materials, Vol. 30, Issue 24 https://doi.org/10.1002/adma.201705963	journal	March 2018
Quantum interference in second-harmonic generation from monolayer WSe2 Lin, Kai-Qiang; Bange, Sebastian; Lupton, John M. Nature Physics, Vol. 15, Issue 3 https://doi.org/10.1038/s41567-018-0384-5	journal	January 2019
Synthesis of paracrystalline diamond Tang, Hu; Yuan, Xiaohong; Cheng, Yong Nature, Vol. 599, Issue 7886 https://doi.org/10.1038/s41586-021-04122-w	journal	November 2021
Giant second-harmonic generation in ferroelectric NbOI2 Abdelwahab, Ibrahim; Tilmann, Benjamin; Wu, Yaze Nature Photonics, Vol. 16, Issue 9 https://doi.org/10.1038/s41566-022-01021-y	journal	June 2022
Nested order-disorder framework containing a crystalline matrix with self-filled amorphous-like innards Bu, Kejun; Hu, Qingyang; Qi, Xiaohuan Nature Communications, Vol. 13, Issue 1 https://doi.org/10.1038/s41467-022-32419-5	journal	August 2022
Anomalous thermal transport under high pressure in boron arsenide Li, Suixuan; Qin, Zihao; Wu, Huan Nature, Vol. 612, Issue 7940 https://doi.org/10.1038/s41586-022-05381-x	journal	November 2022
Layer-Dependent Mechanical Properties and Enhanced Plasticity in the Van der Waals Chromium Trihalide Magnets Cantos-Prieto, Fernando; Falin, Alexey; Alliati, Martin Nano Letters, Vol. 21, Issue 8 https://doi.org/10.1021/acs.nanolett.0c04794	journal	April 2021
Electrical control of second-harmonic generation in a WSe2 monolayer transistor Seyler, Kyle L.; Schaibley, John R.; Gong, Pu Nature Nanotechnology, Vol. 10, Issue 5 https://doi.org/10.1038/nnano.2015.73	journal	April 2015
Second harmonic generation in 2D layered materials Zhang, Jiantian; Zhao, Weina; Yu, Peng 2D Materials, Vol. 7, Issue 4 https://doi.org/10.1088/2053-1583/abaf68	journal	September 2020
Optical modulators with 2D layered materials Sun, Zhipei; Martinez, Amos; Wang, Feng Nature Photonics, Vol. 10, Issue 4 https://doi.org/10.1038/nphoton.2016.15	journal	March 2016
Pressure-Regulated Dynamic Stereochemical Role of Lone-Pair Electrons in Layered Bi ₂ O ₂ S Bu, Kejun; Luo, Hui; Guo, Songhao The Journal of Physical Chemistry Letters, Vol. 11, Issue 22 https://doi.org/10.1021/acs.jpclett.0c02893	journal	November 2020
Ultrathin quantum light source with van der Waals NbOCl2 crystal Guo, Qiangbing; Qi, Xiao-Zhuo; Zhang, Lishu Nature, Vol. 613, Issue 7942 https://doi.org/10.1038/s41586-022-05393-7	journal	January 2023
Broken Local Symmetry in Paraelectric BaTiO 3 Proved by Second Harmonic Generation Pugachev, A. M.; Kovalevskii, V. I.; Surovtsev, N. V. Physical Review Letters, Vol. 108, Issue 24 https://doi.org/10.1103/PhysRevLett.108.247601	journal	June 2012
Pressure-induced robust emission in a zero-dimensional hybrid metal halide (C9NH20)6Pb3Br12 Chen, Mengting; Guo, Songhao; Bu, Kejun Matter and Radiation at Extremes, Vol. 6, Issue 5 https://doi.org/10.1063/5.0058821	journal	August 2021
Enhanced Second-Harmonic Generation of van der Waals CuInP₂S₆ via Pressure-Regulated Cationic Displacement Bu, Kejun; Fu, Tonghuan; Du, Ziwan Chemistry of Materials, Vol. 35, Issue 1 https://doi.org/10.1021/acs.chemmater.2c03066	journal	December 2022
Chiral-perovskite optoelectronics Long, Guankui; Sabatini, Randy; Saidaminov, Makhsud I. Nature Reviews Materials, Vol. 5, Issue 6 https://doi.org/10.1038/s41578-020-0181-5	journal	March 2020
Highly Efficient Sum‐Frequency Generation in Niobium Oxydichloride NbOCl₂ Nanosheets Abdelwahab, Ibrahim; Tilmann, Benjamin; Zhao, Xiaoxu Advanced Optical Materials, Vol. 11, Issue 7 https://doi.org/10.1002/adom.202202833	journal	February 2023
Strong Second Harmonic Generation in a Tungsten Bronze Oxide by Enhancing Local Structural Distortion Lin, Kun; Gong, Pifu; Chu, Shihang Journal of the American Chemical Society, Vol. 142, Issue 16 https://doi.org/10.1021/jacs.0c00133	journal	April 2020
Engineering symmetry breaking in 2D layered materials Du, Luojun; Hasan, Tawfique; Castellanos-Gomez, Andres Nature Reviews Physics, Vol. 3, Issue 3 https://doi.org/10.1038/s42254-020-00276-0	journal	February 2021
Direct electrical modulation of second-order optical susceptibility via phase transitions Wang, Ying; Xiao, Jun; Chung, Ting-Fung Nature Electronics, Vol. 4, Issue 10 https://doi.org/10.1038/s41928-021-00655-0	journal	October 2021
Structural and physical properties of NbO2 and Nb2O5 thin films prepared by magnetron sputtering Hossain, Nazmul; Günes, Ozan; Zhang, Chunzi Journal of Materials Science: Materials in Electronics, Vol. 30, Issue 10 https://doi.org/10.1007/s10854-019-01319-8	journal	April 2019
Reconfiguring band-edge states and charge distribution of organic semiconductor–incorporated 2D perovskites via pressure gating Guo, Songhao; Li, Yahui; Mao, Yuhong Science Advances, Vol. 8, Issue 44 https://doi.org/10.1126/sciadv.add1984	journal	November 2022
Niobium oxide dihalides NbOX ₂ : a new family of two-dimensional van der Waals layered materials with intrinsic ferroelectricity and antiferroelectricity Jia, Yinglu; Zhao, Min; Gou, Gaoyang Nanoscale Horizons, Vol. 4, Issue 5 https://doi.org/10.1039/C9NH00208A	journal	January 2019
Regulating off-centering distortion maximizes photoluminescence in halide perovskites Lü, Xujie; Stoumpos, Constantinos; Hu, Qingyang National Science Review https://doi.org/10.1093/nsr/nwaa288	journal	November 2020
Towards compact phase-matched and waveguided nonlinear optics in atomically layered semiconductors Xu, Xinyi; Trovatello, Chiara; Mooshammer, Fabian Nature Photonics, Vol. 16, Issue 10 https://doi.org/10.1038/s41566-022-01053-4	journal	August 2022
High-pressure structural phase transitions in semiconducting niobium dioxide Haines, J.; Léger, J. M.; Pereira, A. S. Physical Review B, Vol. 59, Issue 21 https://doi.org/10.1103/PhysRevB.59.13650	journal	June 1999
Monitoring Local Strain Vector in Atomic-Layered MoSe ₂ by Second-Harmonic Generation Liang, Jing; Zhang, Jin; Li, Zhenzhu Nano Letters, Vol. 17, Issue 12 https://doi.org/10.1021/acs.nanolett.7b03476	journal	November 2017
Optical Harmonic Generation in 2D Materials Khan, Ahmed Raza; Zhang, Linglong; Ishfaq, Kashif Advanced Functional Materials, Vol. 32, Issue 3 https://doi.org/10.1002/adfm.202105259	journal	December 2021
2D NbOI ₂ : A Chiral Semiconductor with Highly In‐Plane Anisotropic Electrical and Optical Properties Fang, Yuqiang; Wang, Fakun; Wang, Ruiqi Advanced Materials, Vol. 33, Issue 29 https://doi.org/10.1002/adma.202101505	journal	June 2021
Giant enhancement of optical nonlinearity in two-dimensional materials by multiphoton-excitation resonance energy transfer from quantum dots Hong, Hao; Wu, Chunchun; Zhao, Zixun Nature Photonics, Vol. 15, Issue 7 https://doi.org/10.1038/s41566-021-00801-2	journal	April 2021

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